Highly Resolved Dynamic Emissions of Air Pollutants and Greenhouse Gas CO2during COVID-19 Pandemic in East China

ABSTRACT

The unintentional emission reductions caused by the COVID-19 pandemic provides an opportunity to investigate the impact of energy, industry, and transportation activities on air pollutants and CO2 emissions and their synergy. Here, we constructed an approach to estimate city-level high resolution dynamic emissions of both anthropogenic air pollutants and CO2 by introducing dynamic temporal allocation coefficients based on real-time multisource activity data. We first apply this approach to estimate the spatiotemporal evolution of sectoral emissions in eastern China, focusing on the period around the COVID-19 lockdown. Comparisons with observational data show that our approach can well capture the spatiotemporal changes of both short-lived precursors (NOx and NMVOCs) and CO2 emissions. Our results show that air pollutants (SO2, NOx, and NMVOCs) were reduced by up to 31%-53% during the lockdown period accompanied by simultaneous changes of 40% CO2 emissions. The declines in power and heavy industry sectors dominated regional SO2 and CO2 reductions. NOx reductions were mainly attributed to mobile sources, while NMVOCs emission reductions were mainly from light industry sectors. Our findings suggest that differentiated emission control strategies should be implemented for different source categories to achieve coordinated reduction goals. © 2021 American Chemical Society.