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Methane emissions are predominantly responsible for record-breaking atmospheric methane growth rates in 2020 and 2021
Atmospheric Chemistry and Physics ; 23(8):4863-4880, 2023.
Article Dans Anglais | ProQuest Central | ID: covidwho-2298817
ABSTRACT
The global atmospheric methane growth rates reported by NOAA for 2020 and 2021 are the largest since systematic measurements began in 1983. To explore the underlying reasons for these anomalous growth rates, we use newly available methane data from the Japanese Greenhouse gases Observing SATellite (GOSAT) to estimate methane surface emissions. Relative to baseline values in 2019, we find that a significant global increase in methane emissions of 27.0 ± 11.3 and 20.8 ± 11.4 Tg is needed to reproduce observed atmospheric methane in 2020 and 2021, respectively, assuming fixed climatological values for OH. We see the largest annual increases in methane emissions during 2020 over Eastern Africa (14 ± 3 Tg), tropical Asia (3 ± 4 Tg), tropical South America (5 ± 4 Tg), and temperate Eurasia (3 ± 3 Tg), and the largest reductions are observed over China (-6 ± 3 Tg) and India (-2 ± 3 Tg). We find comparable emission changes in 2021, relative to 2019, except for tropical and temperate South America where emissions increased by 9 ± 4 and 4 ± 3 Tg, respectively, and for temperate North America where emissions increased by 5 ± 2 Tg. The elevated contributions we saw in 2020 over the western half of Africa (-5 ± 3 Tg) are substantially reduced in 2021, compared to our 2019 baseline. We find statistically significant positive correlations between anomalies of tropical methane emissions and groundwater, consistent with recent studies that have highlighted a growing role for microbial sources over the tropics. Emission reductions over India and China are expected in 2020 due to the Covid-19 lockdown but continued in 2021, which we do not currently understand. To investigate the role of reduced OH concentrations during the Covid-19 lockdown in 2020 on the elevated atmospheric methane growth in 2020–2021, we extended our inversion state vector to include monthly scaling factors for OH concentrations over six latitude bands. During 2020, we find that tropospheric OH is reduced by 1.4 ± 1.7 % relative to the corresponding 2019 baseline value. The corresponding revised global growth of a posteriori methane emissions in 2020 decreased by 34 % to 17.9 ± 13.2 Tg, relative to the a posteriori value that we inferred using fixed climatological OH values, consistent with sensitivity tests using the OH climatology inversion using reduced values for OH. The counter statement is that 66 % of the global increase in atmospheric methane during 2020 was due to increased emissions, particularly from tropical regions. Regional flux differences between the joint methane–OH inversion and the OH climatology inversion in 2020 are typically much smaller than 10 %. We find that OH is reduced by a much smaller amount during 2021 than in 2020, representing about 10 % of the growth of atmospheric methane in that year. Therefore, we conclude that most of the observed increase in atmospheric methane during 2020 and 2021 is due to increased emissions, with a significant contribution from reduced levels of OH.
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Texte intégral: Disponible Collection: Bases de données des oragnisations internationales Base de données: ProQuest Central langue: Anglais Revue: Atmospheric Chemistry and Physics Année: 2023 Type de document: Article

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Texte intégral: Disponible Collection: Bases de données des oragnisations internationales Base de données: ProQuest Central langue: Anglais Revue: Atmospheric Chemistry and Physics Année: 2023 Type de document: Article