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1.
Sci Rep ; 7(1): 7228, 2017 08 03.
Article in English | MEDLINE | ID: mdl-28775308

ABSTRACT

A strong coupling regime is demonstrated at near infrared between metallic nanoparticle chains (MNP), supporting localized surface plasmons (LSP), and dielectric waveguides (DWGs) having different core materials. MNP chains are deposited on the top of these waveguides in such a way that the two guiding structures are in direct contact with each other. The strong coupling regime implies (i) a strong interpenetration of the bare modes forming two distinct supermodes and (ii) a large power overlap up to the impossibility to distinguish the power quota inside each bare structure. Additionally, since the system involves LSPs, (i) such a strong coupling occurs on a broad band and (ii) the peculiar vortex-like propagation mechanism of the optical power, supported by the MNP chain, leads to a regime where the light is slowed down over a wide wavelength range. Finally, the strong coupling allows the formation of guided supermodes in regions where the bare modes cannot be both guided at the same time. In other words, very high k modes can then be propagated in a dielectric photonic circuit thanks to hybridisation, leading to extremely concentrated propagating wave. Experimental work gives indirect proof of strong coupling regime whatever the waveguide core indexes.

2.
Nat Commun ; 7: 12017, 2016 06 22.
Article in English | MEDLINE | ID: mdl-27328976

ABSTRACT

The advent of metamaterials more than 15 years ago has offered extraordinary new ways of manipulating electromagnetic waves. Yet, progress in this field has been unequal across the electromagnetic spectrum, especially when it comes to finding applications for such artificial media. Optical metamaterials, in particular, are less compatible with active functionalities than their counterparts developed at lower frequencies. One crucial roadblock in the path to devices is the fact that active optical metamaterials are so far controlled by light rather than electricity, preventing them from being integrated in larger electronic systems. Here we introduce electroluminescent metamaterials based on metal nano-inclusions hybridized with colloidal quantum dots. We show that each of these miniature blocks can be individually tuned to exhibit independent optoelectronic properties (both in terms of electrical characteristics, polarization, colour and brightness), illustrate their capabilities by weaving complex light-emitting surfaces and finally discuss their potential for displays and sensors.

3.
Nanoscale Res Lett ; 9(1): 2361, 2014 Dec.
Article in English | MEDLINE | ID: mdl-26089008

ABSTRACT

We report on the use of soft UV nanoimprint lithography (UV-NIL) for the development of reproducible, millimeter-sized, and sensitive substrates for SERS detection. The used geometry for plasmonic nanostructures is the cylinder. Gold nanocylinders (GNCs) showed to be very sensitive and specific sensing surfaces. Indeed, we demonstrated that less than 4 ×10(6) avidin molecules were detected and contributed to the surface-enhanced Raman scattering (SERS) signal. Thus, the soft UV-NIL technique allows to obtain quickly very sensitive substrates for SERS biosensing on surfaces of 1 mm (2).

4.
Opt Express ; 20(16): 17402-10, 2012 Jul 30.
Article in English | MEDLINE | ID: mdl-23038293

ABSTRACT

We demonstrate the integration of short metal nanoparticle chains (L ≈700 nm) supporting localized surface plasmons in Silicon On Insulator (SOI) waveguides at telecom wavelengths. Nanoparticles are deposited on the waveguide top and excited through the evanescent field of the TE waveguide modes. Finite difference time domain calculations and waveguide transmission measurements reveal that almost all the TE mode energy can be transferred to nanoparticle chains at resonance. It is also shown that the transmission spectrum is very sensitive to the molecular environment of nanoparticles, thus opening the way towards ultra-compact sensors in guided plasmonics on SOI. An experimental demonstration is reported with octadecanthiol molecules for a detection volume as small as 0.26 attoliter.


Subject(s)
Biosensing Techniques/instrumentation , Gold/chemistry , Metal Nanoparticles/chemistry , Silicon/chemistry , Computer Simulation , Metal Nanoparticles/ultrastructure , Numerical Analysis, Computer-Assisted , Time Factors
5.
Nano Lett ; 12(2): 1032-7, 2012 Feb 08.
Article in English | MEDLINE | ID: mdl-22251002

ABSTRACT

We demonstrate that the optical energy carried by a TE dielectric waveguide mode can be totally transferred into a transverse plasmon mode of a coupled metal nanoparticle chain. Experiments are performed at 1.5 µm. Mode coupling occurs through the evanescent field of the dielectric waveguide mode. Giant coupling effects are evidenced from record coupling lengths as short as ~560 nm. This result opens the way to nanometer scale devices based on localized plasmons in photonic integrated circuits.


Subject(s)
Gold/chemistry , Metal Nanoparticles/chemistry , Optical Devices , Silicon/chemistry , Surface Plasmon Resonance
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