Radon and thoron concentrations in public workplaces in Brisbane, Australia.

Radon and thoron are radioactive gases that can emanate from soil and building materials, and it can accumulate in indoor environments. The concentrations of radon and thoron in the air from various workplace categories in Brisbane, Australia were measured using an active method. The average radon and thoron concentrations for all workplace categories were 10.5 ± 11.3 and 8.2 ± 1.4 Bq m(-3), respectively. The highest radon concentration was detected in a confined area, 86.6 ± 6.0 Bq m(-3), while the maximum thoron level was found in a storage room, 78.1 ± 14.0 Bq m(-3). At each site, the concentrations of radon and thoron were measured at two heights, 5 cm and 120 cm above the floor. The effect of the measurement heights on the concentration level was significant in the case of thoron. The monitoring of radon and thoron concentrations showed a lower radon concentration during work hours than at other times of the day. This can be attributed to the ventilation systems, including the air conditioner and natural ventilation, which normally operate during work hours. The diurnal variation was less observed in the case of thoron, as the change in its concentration during and after the working hours was insignificant. The study also investigated the influence of the floor level and flooring type on indoor radon and thoron concentrations. The elevated levels of radon and thoron were largely found in basements and ground floor levels and in rooms with concrete flooring.

Radon-222 activity flux measurement using activated charcoal canisters: revisiting the methodology.

The measurement of radon ((222)Rn) activity flux using activated charcoal canisters was examined to investigate the distribution of the adsorbed (222)Rn in the charcoal bed and the relationship between (222)Rn activity flux and exposure time. The activity flux of (222)Rn from five sources of varying strengths was measured for exposure times of one, two, three, five, seven, 10, and 14 days. The distribution of the adsorbed (222)Rn in the charcoal bed was obtained by dividing the bed into six layers and counting each layer separately after the exposure. (222)Rn activity decreased in the layers that were away from the exposed surface. Nevertheless, the results demonstrated that only a small correction might be required in the actual application of charcoal canisters for activity flux measurement, where calibration standards were often prepared by the uniform mixing of radium ((226)Ra) in the matrix. This was because the diffusion of (222)Rn in the charcoal bed and the detection efficiency as a function of the charcoal depth tended to counterbalance each other. The influence of exposure time on the measured (222)Rn activity flux was observed in two situations of the canister exposure layout: (a) canister sealed to an open bed of the material and (b) canister sealed over a jar containing the material. The measured (222)Rn activity flux decreased as the exposure time increased. The change in the former situation was significant with an exponential decrease as the exposure time increased. In the latter case, lesser reduction was noticed in the observed activity flux with respect to exposure time. This reduction might have been related to certain factors, such as absorption site saturation or the back diffusion of (222)Rn gas occurring at the canister-soil interface.

Radon-222 exhalation from open ground on and around a uranium mine in the wet-dry tropics.

Radon-222 exhalation from the ground surface depends upon a number of variables such as the 226Ra activity concentration and its distribution in soil grains; soil grain size; soil porosity, temperature and moisture; atmospheric pressure, rainfall and temperature. In this study, 222Rn exhalation flux density measurements within and around the Ranger uranium mine in northern Australia were performed to investigate the effect of these variables within a tropical region. Measurements were taken at the waste rock dumps, ore stockpiles, mine pits, and at sites where effluent water with elevated 226Ra concentration has been spray irrigated over land, as well as at sites outside the mine. The sites selected represented a variety of geomorphic regions ranging from uranium-bearing rocks to ambient soils. Generally, wet season rains reduced 222Rn exhalation but at a few sites the onset of rains caused a step rise in exhalation flux densities. The results show that parameters such as 226Ra activity concentration, soil grain size and soil porosity have a marked effect on 222Rn flux densities. For similar geomorphic sites, 226Ra activity concentration is a dominant factor, but soil grain size and porosity also influence 222Rn exhalation. Surfaces with vegetation showed higher exhalation flux densities than their barren counterparts, perhaps because the associated root structure increases soil porosity and moisture retention. Repeated measurements over one year at eight sites enabled an analysis of precipitation and soil moisture effects on 222Rn exhalation. Soil moisture depth profiles varied both between seasons and at different times during the wet season, indicating that factors such as duration, intensity and time between precipitation events can influence 222Rn flux densities considerably.