Continuous-wave mirrorless lasing at 2.21 µm in sodium vapors.

We demonstrate backward-directed continuous-wave (cw) emission at 2.21 µm generated on the 4P3/2-4S1/2 population-inverted transition in Na vapors that are two-photon excited with resonant laser light at 589 and 569 nm. Our study of power and atom-number-density threshold characteristics shows that lasing occurs at sub-10 mW total power of the applied laser light. The observed 6 mrad divergence is defined mainly by the aspect ratio of the gain region. We find that mirrorless lasing at 2.21 µm is magnetic field and polarization dependent and this may be useful for remote magnetometry. The presented results could help determine the requirements for obtaining directional return from sodium atoms in the mesosphere.

Arithmetic with optical topological charges in stepwise-excited Rb vapor.

We report on experimentally observed addition, subtraction, and cancellation of orbital angular momentum (OAM) in the process of parametric four-wave mixing that results in frequency up- and down-converted emission in Rb vapor. Specific features of OAM transfer from resonant laser fields with different optical topological charges to the spatially and temporally coherent blue light (CBL) have been considered. We have observed the conservation of OAM in nonlinear wave mixing in a wide range of experimental conditions, including a noncollinear geometry of the applied laser beams, and furthermore, that the CBL accumulates the total OAM of the applied laser light. Spectral and power dependences of vortex and plane wavefront blue light beams have been compared.

Distinguishing nonlinear processes in atomic media via orbital angular momentum transfer.

We suggest a technique based on the transfer of topological charge from applied laser radiation to directional and coherent optical fields generated in ladder-type excited atomic media to identify the major processes responsible for their appearance. As an illustration, in Rb vapors, we analyze transverse intensity and phase profiles of the forward-directed collimated blue and near-IR light using self-interference and astigmatic transformation techniques when either or both of two resonant laser beams carry orbital angular momentum. Our observations unambiguously demonstrate that emission at 1.37 µm is the result of a parametric four-wave mixing process involving only one of the two applied laser fields.

Coherent and collimated blue light generated by four-wave mixing in Rb vapour.

We investigate frequency up-conversion of low power cw resonant radiation in Rb vapour as a function of various experimental parameters. We present evidence that the process of four wave mixing is responsible for unidirectional blue light generation and that the phase matching conditions along a light-induced waveguide determine the direction and divergence of the blue light. Velocity-selective excitation to the 5D level via step-wise and two-photon processes results in a Doppler-free dependence on the frequency detuning of the applied laser fields from the respective dipole-allowed transitions. Possible schemes for ultraviolet generation are discussed.