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1.
Phys Rev Lett ; 117(2): 027001, 2016 Jul 08.
Article in English | MEDLINE | ID: mdl-27447519

ABSTRACT

The nature of the pairing states of superconducting LaNiC_{2} and LaNiGa_{2} has to date remained a puzzling question. Broken time reversal symmetry has been observed in both compounds and a group theoretical analysis implies a nonunitary triplet pairing state. However, all the allowed nonunitary triplet states have nodal gap functions but most thermodynamic and NMR measurements indicate fully gapped superconductivity in LaNiC_{2}. Here we probe the gap symmetry of LaNiGa_{2} by measuring the London penetration depth, specific heat, and upper critical field. These measurements demonstrate two-gap nodeless superconductivity in LaNiGa_{2}, suggesting that this is a common feature of both compounds. These results allow us to propose a novel triplet superconducting state, where the pairing occurs between electrons of the same spin, but on different orbitals. In this case the superconducting wave function has a triplet spin component but isotropic even parity gap symmetry, yet the overall wave function remains antisymmetric under particle exchange. This model leads to a nodeless two-gap superconducting state which breaks time reversal symmetry, and therefore accounts well for the seemingly contradictory experimental results.

2.
J Phys Condens Matter ; 26(27): 274212, 2014 Jul 09.
Article in English | MEDLINE | ID: mdl-24934542

ABSTRACT

The presence of a spin-flip potential at the interface between a superconductor and a ferromagnetic metal allows for the generation of equal-spin spin-triplet Cooper pairs. These Cooper pairs are compatible with the exchange interaction within the ferromagnetic region and hence allow for the long-range proximity effect through a ferromagnet or half-metal. One suitable spin-flip potential is provided by incorporating the conical magnet Holmium (Ho) into the interface. The conical magnetic structure is characterised by an opening angle α with respect to the crystal c-axis and a turning (or pitch) angle ß measuring the rotation of magnetisation with respect to the adjacent layers. Here, we present results showing the influence of conical magnet interface layers with varying α and ß on the efficiency of the generation of equal-spin spin-triplet pairing. The results are obtained by self-consistent solutions of the microscopic Bogoliubov-de Gennes equations in the clean limit within a tight-binding model of the heterostructure. In particular, the dependence of unequal-spin and equal-spin spin-triplet pairing correlations on the conical magnetic angles α and ß are discussed in detail.


Subject(s)
Algorithms , Electric Conductivity , Electromagnetic Fields , Holmium/chemistry , Magnets , Models, Chemical , Computer Simulation
3.
Phys Rev Lett ; 112(10): 107002, 2014 Mar 14.
Article in English | MEDLINE | ID: mdl-24679322

ABSTRACT

We have investigated the superconducting state of the noncentrosymmetric compound Re6Zr using magnetization, heat capacity, and muon-spin relaxation or rotation (µSR) measurements. Re6Zr has a superconducting transition temperature, Tc=6.75±0.05 K. Transverse-field µSR experiments, used to probe the superfluid density, suggest an s-wave character for the superconducting gap. However, zero and longitudinal-field µSR data reveal the presence of spontaneous static magnetic fields below Tc indicating that time-reversal symmetry is broken in the superconducting state and an unconventional pairing mechanism. An analysis of the pairing symmetries identifies the ground states compatible with time-reversal symmetry breaking.

4.
Phys Rev Lett ; 109(9): 097001, 2012 Aug 31.
Article in English | MEDLINE | ID: mdl-23002872

ABSTRACT

Muon spin rotation and relaxation experiments on the centrosymmetric intermetallic superconductor LaNiGa2 are reported. The appearance of spontaneous magnetic fields coincides with the onset of superconductivity, implying that the superconducting state breaks time reversal symmetry, similarly to noncentrosymmetric LaNiC2. Only four triplet states are compatible with this observation, all of which are nonunitary triplets. This suggests that LaNiGa2 is the centrosymmetric analogue of LaNiC2. We argue that these materials are representatives of a new family of paramagnetic nonunitary superconductors.

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