Measurement of delayed fluorescence in N2 + with a streak camera.

Using a streak camera, we directly measure time- and space-resolved dynamics of N 2 + emission from a self-seeded filament. Fluorescence emission does not start with ionization, but with a delay in the tenth of ps range.

High-resolution remote spectroscopy and plasma dynamics induced with UV filaments.

Spectroscopy is performed on the plume created by a high-power short-pulse laser on a solid surface. It is shown that high resolution (<10 pm) and accurate spectral analysis can be performed using a self-absorption feature appearing within the emission lines. The time-dependent self-absorption study reveals dynamics of a shock wave.

Testing the Role of Recollision in N_{2}

It has been known for many years that during filamentation of femtosecond light pulses in air, gain is observed on the B to X transition in N_{2}^{+}. While the gain mechanism remains unclear, it has been proposed that recollision, a process that is fundamental to much of strong field science, is critical for establishing gain. We probe this hypothesis by directly comparing the influence of the ellipticity of the pump light on gain in air filaments. Then, we decouple filamentation from gain by measuring the gain in a thin gas jet that we also use for high harmonic generation. The latter allows us to compare the dependence of the gain on the ellipticity of the pump with the dependence of the high harmonic signal on the ellipticity of the fundamental. We find that gain and harmonic generation have very different behavior in both filaments and in the jet. In fact, in a jet we even measure gain with circular polarization. Thus, we establish that recollision does not play a significant role in creating the inversion.

Controlling the orbital angular momentum of high harmonic vortices.

Optical vortices, which carry orbital angular momentum (OAM), can be flexibly produced and measured with infrared and visible light. Their application is an important research topic for super-resolution imaging, optical communications and quantum optics. However, only a few methods can produce OAM beams in the extreme ultraviolet (XUV) or X-ray, and controlling the OAM on these beams remains challenging. Here we apply wave mixing to a tabletop high-harmonic source, as proposed in our previous work, and control the topological charge (OAM value) of XUV beams. Our technique enables us to produce first-order OAM beams with the smallest possible central intensity null at XUV wavelengths. This work opens a route for carrier-injected laser machining and lithography, which may reach nanometre or even angstrom resolution. Such a light source is also ideal for space communications, both in the classical and quantum regimes.

Perturbative High Harmonic Wave Front Control.

We pattern the wave front of a high harmonic beam by intersecting the intense driving laser pulse that generates the high harmonic with a weak control pulse. To illustrate the potential of wave-front control, we imprint a Fresnel zone plate pattern on a harmonic beam, causing the harmonics to focus and defocus. The quality of the focus that we achieve is measured using the spectral wave-front optical reconstruction by diffraction method. We will show that it is possible to enhance the peak intensity by orders of magnitude without a physical optical element in the path of the extreme ultraviolet (XUV) beam. Through perturbative wave-front control, XUV beams can be created with a flexibility approaching what technology allows for visible and infrared light.

Dramatic enhancement of supercontinuum generation in elliptically-polarized laser filaments.

Broadband laser sources based on supercontinuum generation in femtosecond laser filamentation have enabled applications from stand-off sensing and spectroscopy to the generation and self-compression of high-energy few-cycle pulses. Filamentation relies on the dynamic balance between self-focusing and plasma defocusing - mediated by the Kerr nonlinearity and multiphoton or tunnel ionization, respectively. The filament properties, including the supercontinuum generation, are therefore highly sensitive to the properties of both the laser source and the propagation medium. Here, we report the anomalous spectral broadening of the supercontinuum for filamentation in molecular gases, which is observed for specific elliptical polarization states of the input laser pulse. The resulting spectrum is accompanied by a modification of the supercontinuum polarization state and a lengthening of the filament plasma column. Our experimental results and accompanying simulations suggest that rotational dynamics of diatomic molecules play an essential role in filamentation-induced supercontinuum generation, which can be controlled with polarization ellipticity.

Impact of resonant dispersion on the sensitivity of intracavity phase interferometry and laser gyros.

Intracavity phase interferometry is a phase sensing technique using mode-locked lasers in which two intracavity pulses circulate. The beat frequency between the two output frequency combs is proportional to a phase shift to be measured. A laser gyro is a particular implementation of this device. The demonstrated sensitivity of 10-8 of these devices could be manipulated by applying a giant dispersion to each tooth of the comb. It is shown that the resonant dispersion of a Fabry-Perot inserted in the cavity couples to the modes of the frequency comb, resulting in a large change in phase response.

Ring-shaped backward stimulated Raman scattering driven by stimulated Brillouin scattering.

Backward stimulated Raman scattering is generated in water, pumped by pre-compressed pulses from a single-cell stimulated Brillouin scattering pulse compressor. The maximum energy efficiency of 9% is achieved by employing a circularly-polarized pump pulse at its energy of 50 mJ, around which point the backward stimulated Raman scattering also exhibits a ring-shaped profile. The correlations between spatial and temporal profiles as well as the intensities of the backward stimulated Raman and the stimulated Brillouin scattering generated from Raman cell indicate that the ring-shaped backward stimulated Raman is driven by intense stimulated Brillouin scattering. We demonstrate the latter process to be much more efficient for the backward Raman generation than the conventional process in which the laser itself pumps a backward stimulated Raman beam. It is shown that a further increase in pump energy leads to a drop in efficiency, combined with a break-up of the ring pattern of backward stimulated Raman. These effects are associated with filament generation above a certain threshold.

Self-induced transparency and coherent population trapping of 87Rb vapor in a mode-locked laser.

Simultaneous self-induced transparency and a dark line resonance are observed inside a mode-locked laser. The circulating pulse, tuned to the 795-nm optical resonance of rubidium, has sufficient intensity to create at each passage a population inversion-return to ground state, typical of self-induced transparency. A drop in fluorescence (dark line resonance), is observed as the repetition rate is tuned to a submultiple of the hyperfine ground-state splitting.

Polarization evolution of ultrashort pulses in air.

Measurements of polarization of filamenting light pulses at 800 nm are presented. Electronic nonlinearity, molecular alignment and nonlinear losses all contribute to modify the polarization of a femtosecond filamenting pulse. The polarization is modified in each stage of preparation, filamentation and divergence after the filament.

The effect of propagation in air on the filament spectrum.

Filamentation studies traditionally start from letting a beam focus in air. We present filament studies with control over the preparation propagation, in air or vacuum, using an aerodynamic window. The spectral content of the filament strongly depends on its preparation medium.

Group and phase velocity coupling of colliding pulses in a nanostructure.

It is generally accepted that, in a laser cavity, the group delay--responsible for the round trip time--and the phase delay both have a linear dependence on the cavity length. We show that nanostructures, such as quantum wells, can create a coupling between phase and group velocities, resulting in a periodic dependence of the repetition rate on the laser cavity length.