ABSTRACT
de Haas-van Alphen oscillations of the organic metal κ-(ET)2Cu(SCN)2 have been measured up to 55 T at liquid helium temperatures. The Fermi surface of this charge transfer salt is a textbook example of a linear chain of orbits coupled by magnetic breakdown. Accordingly, the oscillation spectrum is composed of linear combinations of the frequencies linked to the α and magnetic breakdown-induced ß orbits. The field and temperature dependence of all the observed Fourier components, in particular the 'forbidden frequency' [Formula: see text] which cannot correspond to a classical orbit, are quantitatively accounted for by analytical calculations based on a second order development of the free energy, i.e. beyond the first order Lifshitz-Kosevich formula.
ABSTRACT
According to band structure calculations, the Fermi surface of the quasi-two dimensional metal θ-(ET)4ZnBr4(C6H4Cl2) illustrates the linear chain of coupled orbits model. Accordingly, de Haas-van Alphen oscillations spectra recorded in pulsed magnetic field of up to 55 T evidence many Fourier components, the frequency of which are linear combinations of the frequencies relevant to the closed α and the magnetic breakdown ß orbits. The field and temperature dependence of their amplitude are quantitatively accounted for by analytic calculations including, beyond the Lifshitz-Kosevich formula, second-order terms in damping factors due to the oscillation of the chemical potential as the magnetic field varies. Whereas these second-order terms are negligible for the orbits α, ß and 2ß-α, they are solely responsible for the 'forbidden orbit' ß-α and its harmonic and have a significant influence on Fourier components such as 2α and ß+α, yielding strongly non-Lifshitz-Kosevich behaviour in the latter case.
ABSTRACT
By improving the experimental conditions and extensive data accumulation, we have achieved very high precision in the measurements of the de Haas-van Alphen effect in the underdoped high-temperature superconductor YBa2Cu3O6.5. We find that the main oscillation, so far believed to be single frequency, is composed of three closely spaced frequencies. We attribute this to bilayer splitting and warping of a single quasi-2D Fermi surface, indicating that c axis coherence is restored at low temperature in underdoped cuprates. Our results do not support the existence of a larger frequency of the order of 1650 T reported recently in the same compound [S. E. Sebastian, Nature (London) 454, 200 (2008)].
ABSTRACT
The de Haas-van Alphen effect was observed in the underdoped cuprate YBa2Cu3O6.5 via a torque technique in pulsed magnetic fields up to 59 T. Above a field of approximately 30 T the magnetization exhibits clear quantum oscillations with a single frequency of 540 T and a cyclotron mass of 1.76 times the free electron mass, in excellent agreement with previously observed Shubnikov-de Haas oscillations. The oscillations obey the standard Lifshitz-Kosevich formula of Fermi-liquid theory. This thermodynamic observation of quantum oscillations confirms the existence of a well-defined, closed, and coherent, Fermi surface in the pseudogap phase of cuprates.
