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1.
Environ Sci Technol ; 43(3): 743-9, 2009 Feb 01.
Article in English | MEDLINE | ID: mdl-19245011

ABSTRACT

Geological storage of carbon dioxide (CO2) is likely to be an integral component of any realistic plan to reduce anthropogenic greenhouse gas emissions. In conjunction with large-scale deployment of carbon storage as a technology, there is an urgent need for tools which provide reliable and quick assessments of aquifer storage performance. Previously, abandoned wells from over a century of oil and gas exploration and production have been identified as critical potential leakage paths. The practical importance of abandoned wells is emphasized by the correlation of heavy CO2 emitters (typically associated with industrialized areas) to oil and gas producing regions in North America. Herein, we describe a novel framework for predicting the leakage from large numbers of abandoned wells, forming leakage paths connecting multiple subsurface permeable formations. The framework is designed to exploit analytical solutions to various components of the problem and, ultimately, leads to a grid-free approximation to CO2 and brine leakage rates, as well as fluid distributions. We apply our model in a comparison to an established numerical solverforthe underlying governing equations. Thereafter, we demonstrate the capabilities of the model on typical field data taken from the vicinity of Edmonton, Alberta. This data set consists of over 500 wells and 7 permeable formations. Results show the flexibility and utility of the solution methods, and highlight the role that analytical and semianalytical solutions can play in this important problem.


Subject(s)
Carbon Dioxide/chemistry , Geology , Models, Theoretical , Algorithms
2.
Environ Sci Technol ; 39(2): 602-11, 2005 Jan 15.
Article in English | MEDLINE | ID: mdl-15707061

ABSTRACT

Capture and subsequent injection of carbon dioxide into deep geological formations is being considered as a means to reduce anthropogenic emissions of CO2 to the atmosphere. If such a strategy is to be successful, the injected CO2 must remain within the injection formation for long periods of time, at least several hundred years. Because mature continental sedimentary basins have a century-long history of oil and gas exploration and production, they are characterized by large numbers of existing oil and gas wells. For example, more than 1 million such wells have been drilled in the state of Texas in the United States. These existing wells represent potential leakage pathways for injected CO2. To analyze leakage potential, modeling tools are needed that predict leakage rates and patterns in systems with injection and potentially leaky wells. A new semianalytical solution framework allows simple and efficient prediction of leakage rates for the case of injection of supercritical CO2 into a brine-saturated deep aquifer. The solution predicts the extent of the injected CO2 plume, provides leakage rates through an abandoned well located at an arbitrary distance from the injection well, and estimates the CO2 plume extent in the overlying aquifer into which the fluid leaks. Comparison to results from a numerical multiphase flow simulator show excellent agreement. Example calculations show the importance of outer boundary conditions, the influence of both density and viscosity contrasts in the resulting solutions, and the potential importance of local upconing around the leaky well. While several important limiting assumptions are required, the new semianalytical solution provides a simple and efficient procedure for estimation of CO2 leakage for problems involving one injection well, one leaky well, and multiple aquifers separated by impermeable aquitards.


Subject(s)
Carbon Dioxide/analysis , Geology , Models, Theoretical , Petroleum , Equipment Failure , Forecasting , Geological Phenomena , Permeability , Soil , Texas , Volatilization
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