Terahertz electric-field-driven dynamical multiferroicity in SrTiO3.

The emergence of collective order in matter is among the most fundamental and intriguing phenomena in physics. In recent years, the dynamical control and creation of novel ordered states of matter not accessible in thermodynamic equilibrium is receiving much attention1-6. The theoretical concept of dynamical multiferroicity has been introduced to describe the emergence of magnetization due to time-dependent electric polarization in non-ferromagnetic materials7,8. In simple terms, the coherent rotating motion of the ions in a crystal induces a magnetic moment along the axis of rotation. Here we provide experimental evidence of room-temperature magnetization in the archetypal paraelectric perovskite SrTiO3 due to this mechanism. We resonantly drive the infrared-active soft phonon mode with an intense circularly polarized terahertz electric field and detect the time-resolved magneto-optical Kerr effect. A simple model, which includes two coupled nonlinear oscillators whose forces and couplings are derived with ab initio calculations using self-consistent phonon theory at a finite temperature9, reproduces qualitatively our experimental observations. A quantitatively correct magnitude was obtained for the effect by also considering the phonon analogue of the reciprocal of the Einstein-de Haas effect, which is also called the Barnett effect, in which the total angular momentum from the phonon order is transferred to the electronic one. Our findings show a new path for the control of magnetism, for example, for ultrafast magnetic switches, by coherently controlling the lattice vibrations with light.

Axial Magnetoelectric Effect in Dirac Semimetals.

We propose a mechanism to generate a static magnetization via the "axial magnetoelectric effect" (AMEE). Magnetization M∼E_{5}(ω)×E_{5}^{*}(ω) appears as a result of the transfer of the angular momentum of the axial electric field E_{5}(t) into the magnetic moment in Dirac and Weyl semimetals. We point out similarities and differences between the proposed AMEE and a conventional inverse Faraday effect. As an example, we estimated the AMEE generated by circularly polarized acoustic waves and find it to be on the scale of microgauss for gigahertz frequency sound. In contrast to a conventional inverse Faraday effect, magnetization rises linearly at small frequencies and fixed sound intensity as well as demonstrates a nonmonotonic peak behavior for the AMEE. The effect provides a way to investigate unusual axial electromagnetic fields via conventional magnetometry techniques.

Erratum: Dynamic Multiferroicity of a Ferroelectric Quantum Critical Point [Phys. Rev. Lett. 122, 057208 (2019)].

This corrects the article DOI: 10.1103/PhysRevLett.122.057208.

Interacting Dirac materials.

We investigate the extent to which the class of Dirac materials in two-dimensions provides general statements about the behavior of both fermionic and bosonic Dirac quasiparticles in the interacting regime. For both quasiparticle types, we find common features for the interaction induced renormalization of the conical Dirac spectrum. We perform the perturbative renormalization analysis and compute the self-energy for both quasiparticle types with different interactions and collate previous results from the literature whenever necessary. Guided by the systematic presentation of our results in table 1, we conclude that long-range interactions generically lead to an increase of the slope of the single-particle Dirac cone, whereas short-range interactions lead to a decrease. The quasiparticle statistics does not qualitatively impact the self-energy correction for long-range repulsion but does affect the behavior of short-range coupled systems, giving rise to different thermal power-law contributions. The possibility of a universal description of the Dirac materials based on these features is also mentioned.

Gap-like feature observed in the non-magnetic topological insulators.

Non-magnetic gap at the Dirac point of topological insulators remains an open question in the field. Here, we present angle-resolved photoemission spectroscopy experiments performed on Cr-doped Bi2Se3 and showed that the Dirac point is progressively buried by the bulk bands and a low spectral weight region in the vicinity of the Dirac point appears. These two mechanisms lead to spectral weight suppression region being mistakenly identified as an energy gap in earlier studies. We further calculated the band structure and found that the original Dirac point splits into two nodes due to the impurity resonant states and the energy separation between the nodes is the low density of state region which appears to be like an energy gap in potoemission experiments. We supported our arguments by presenting photoemission experiments carried out with on- and off- resonant photon energies. Our observation resolves the widely debated questions of apparent energy gap opening at the Dirac point without long range ferromagnetic order in topological insulators.

Dynamic Multiferroicity of a Ferroelectric Quantum Critical Point.

Quantum matter hosts a large variety of phases, some coexisting, some competing; when two or more orders occur together, they are often entangled and cannot be separated. Dynamical multiferroicity, where fluctuations of electric dipoles lead to magnetization, is an example where the two orders are impossible to disentangle. Here we demonstrate an elevated magnetic response of a ferroelectric near the ferroelectric quantum critical point (FE QCP), since magnetic fluctuations are entangled with ferroelectric fluctuations. We thus suggest that any ferroelectric quantum critical point is an inherent multiferroic quantum critical point. We calculate the magnetic susceptibility near the FE QCP and find a region with enhanced magnetic signatures near the FE QCP and controlled by the tuning parameter of the ferroelectric phase. The effect is small but observable-we propose quantum paraelectric strontium titanate as a candidate material where the magnitude of the induced magnetic moments can be ∼5×10^{-7} µ_{B} per unit cell near the FE QCP.

Effect of Coenzyme Q10 on Expression of UbiAd1 Gene in Rat Model of Local Cerebral Ischemia.

The study examined the effect of endogenous lipid-soluble antioxidant coenzyme Q10 on the expression of UbiA gene of prenyltransferase domain-containing protein 1 (UbiAd1) involved in synthesis of vitamin K2 (and probably of coenzyme Q10) on a rat model of ischemic stroke provoked by ligation of the middle cerebral artery in the left hemisphere. Ischemia enhanced expression of mRNA of UbiAd1 gene in both cerebral hemispheres, but the effect was significant only in the contralateral one. The study revealed no effect of intraperitoneal injection of coenzyme Q10 (30 mg/kg) on ischemia-produced elevation of mRNA of UbiAd1 gene. Further studies are needed to assess possible neuroprotective effects of antioxidant coenzyme Q10.

Prolonged duration of nonequilibrated Dirac fermions in neutral topological insulators.

Topological insulators (TIs) possess spin-polarized Dirac fermions on their surface but their unique properties are often masked by residual carriers in the bulk. Recently, (Sb1-x Bi x )2Te3 was introduced as a non-metallic TI whose carrier type can be tuned from n to p across the charge neutrality point. By using time- and angle-resolved photoemission spectroscopy, we investigate the ultrafast carrier dynamics in the series of (Sb1-x Bi x )2Te3. The Dirac electronic recovery of ∼10 ps at most in the bulk-metallic regime elongated to >400 ps when the charge neutrality point was approached. The prolonged nonequilibration is attributed to the closeness of the Fermi level to the Dirac point and to the high insulation of the bulk. We also discuss the feasibility of observing excitonic instability of (Sb1-x Bi x )2Te3.

[Single Nucleotide Polymorphisms in T-Cadherin Gene (CDH13) Have Cumulative Effect on Body Mass in Patients With Ischemic Heart Disease].

BACKGROUND: Low adiponectin concentration observed in obese patients is associated with a high risk of metabolic disorders and cardiovascular diseases and could be related to single nucleotide polymorphisms (SNPs) in T-cadherin gene (CDH13). T-cadherin is a receptor for adiponectin and low-density lipoprotein. Aim of this study was to investigate association of CDH13 SNPs with the development of obesity in patients with ischemic heart disease (IHD). RESULTS: We established a statistically significant correlation between the number of minor alleles of rs11646213, rs4783244 and rs12444338 in CDH13 gene with body mass index: patients with smaller number of minor alleles tended to have normal body weight (odds ratio 3.03, 95% confidence interval 1.03-8.87). CONCLUSION: The obtained results are indicative of the cumulative effect of SNPs in CDH13 (rs11646213, rs4783244, rs12444338) on BMI in patients with IHD.

Induced magnetization in La0.7Sr0.3MnO3/BiFeO3 superlattices.

Using polarized neutron reflectometry, we observe an induced magnetization of 75 ± 25 kA/m at 10 K in a La(0.7)Sr(0.3)MnO(3) (LSMO)/BiFeO(3) superlattice extending from the interface through several atomic layers of the BiFeO(3) (BFO). The induced magnetization in BFO is explained by density functional theory, where the size of band gap of BFO plays an important role. Considering a classical exchange field between the LSMO and BFO layers, we further show that magnetization is expected to extend throughout the BFO, which provides a theoretical explanation for the results of the neutron scattering experiment.

Engineering three-dimensional topological insulators in Rashba-type spin-orbit coupled heterostructures.

Topological insulators represent a new class of quantum phase defined by invariant symmetries and spin-orbit coupling that guarantees metallic Dirac excitations at its surface. The discoveries of these states have sparked the hope of realizing non-trivial excitations and novel effects such as a magnetoelectric effect and topological Majorana excitations. Here we develop a theoretical formalism to show that a three-dimensional topological insulator can be designed artificially via stacking bilayers of two-dimensional Fermi gases with opposite Rashba-type spin-orbit coupling on adjacent layers, and with interlayer quantum tunneling. We demonstrate that in the stack of bilayers grown along a (001)-direction, a non-trivial topological phase transition occurs above a critical number of Rashba bilayers. In the topological phase, we find the formation of a single spin-polarized Dirac cone at the -point. This approach offers an accessible way to design artificial topological insulators in a set up that takes full advantage of the atomic layer deposition approach. This design principle is tunable and also allows us to bypass limitations imposed by bulk crystal geometry.

Local electronic structure and Fano interference in tunneling into a Kondo hole system.

Motivated by the recent success of local electron tunneling into heavy-fermion materials, we study the local electronic structure around a single Kondo hole in an Anderson lattice model and the Fano interference pattern relevant to STM experiments. Within the Gutzwiller method, we find that an intragap bound state exists in the heavy Fermi liquid regime. The energy position of the intragap bound state is dependent on the on-site potential scattering strength in the conduction and f-orbital channels. Within the same method, we derive a new dI/dV formulation, which includes explicitly the renormalization effect due to the f-electron correlation. It is found that the Fano interference gives asymmetric coherent peaks separated by the hybridization gap. The intragap peak structure has a lorenzian shape, and the corresponding dI/dV intensity depends on the energy location of the bound state.

Testing the sign-changing superconducting gap in iron-based superconductors with quasiparticle interference and neutron scattering.

We present a phenomenological calculation of the quasiparticle interference (QPI) pattern and inelastic neutron scattering (INS) spectra in iron-pnictide and layered iron-selenide compounds by using material specific band structure and superconducting (SC) gap properties. As both the QPI and the INS spectra arise due to scattering of the Bogolyubov quasiparticles, they exhibit a one-to-one correspondence of the scattering vectors and the energy scales. We show that these two spectroscopies complement each other in such a way that a comparative study allows one to extract quantitative and unambiguous information about the underlying pairing structure and the phase of the SC gap. Due to the nodeless and isotropic nature of the SC gaps, both the QPI and INS maps are concentrated at only two energies in pnictide (two SC gaps) and one energy in iron-selenide, while the associated scattering vectors q for scattering of sign-changing and same sign of the SC gaps change between these spectroscopies. The results presented, particularly for the newly discovered iron-selenide compounds, can be used to test the nodeless d-wave pairing in this class of high temperature superconductor.

Local electronic structure of a single nonmagnetic impurity as a test of the pairing symmetry of electrons in (K,Tl)FexSe2 superconductors.

We study the effect of a single nonmagnetic impurity on the recently discovered (K,Tl)Fe(x)Se(2) superconductors, within both a toy two-band model and a more realistic five-band model. We find that, out of five types of pairing symmetry under consideration, only the d(x(2)-y(2))-wave pairing gives rise to impurity resonance states. The intragap states have energies far away from the Fermi energy. The existence of these intragap states is robust against the presence or absence of interband scattering. However, the interband scattering does tune the relative distribution of local density of states at the resonance states. All these features can readily be accessed by STM experiments, and are proposed as a means to test the pairing symmetry of the new superconductors.

Two energy scales in the magnetic resonance spectrum of electron and hole doped pnictide superconductors.

We argue that a multiband superconductor with sign-changing gaps may have multiple spin resonances. We calculate the RPA-based spin resonance spectra of a pnictide superconductor by using the five-band tight-binding model or angle-resolved photoemission spectroscopy Fermi surface (FS) and experimental values of superconducting gaps. The resonance spectra split in both energy and momenta due to the effects of multiband and multiple gaps in s(±) pairing; the higher energy peak appears around the commensurate momenta due to scattering between α-FS to γ/δ-FS pockets. The second resonance is incommensurate, coming from ß-FS to γ/δ-FS scatterings, and its q vector is doping-dependent and, hence, on the FS topology. Energies of both resonances ω(res)(1,2) are strongly doping-dependent and are proportional to the gap amplitudes at the contributing FSs.

Interplay of rotational, relaxational, and shear dynamics in solid 4He.

Using a high-sensitivity torsional oscillator (TO) technique, we mapped the rotational and relaxational dynamics of solid helium-4 ((4)He) throughout the parameter range of the proposed supersolidity. We found evidence that the same microscopic excitations controlling the torsional oscillator motions are generated independently by thermal and mechanical stimulation. Moreover, a measure for the relaxation times of these excitations diverges smoothly without any indication for a critical temperature or critical velocity of a supersolid transition. Finally, we demonstrated that the combined temperature-velocity dependence of the TO response is indistinguishable from the combined temperature-strain dependence of the solid's shear modulus. This implies that the rotational responses of solid (4)He attributed to supersolidity are associated with generation of the same microscopic excitations as those produced by direct shear strain.

Imaging the Fano lattice to 'hidden order' transition in URu(2)Si(2).

Within a Kondo lattice, the strong hybridization between electrons localized in real space (r-space) and those delocalized in momentum-space (k-space) generates exotic electronic states called 'heavy fermions'. In URu(2)Si(2) these effects begin at temperatures around 55 K but they are suddenly altered by an unidentified electronic phase transition at T(o) = 17.5 K. Whether this is conventional ordering of the k-space states, or a change in the hybridization of the r-space states at each U atom, is unknown. Here we use spectroscopic imaging scanning tunnelling microscopy (SI-STM) to image the evolution of URu(2)Si(2) electronic structure simultaneously in r-space and k-space. Above T(o), the 'Fano lattice' electronic structure predicted for Kondo screening of a magnetic lattice is revealed. Below T(o), a partial energy gap without any associated density-wave signatures emerges from this Fano lattice. Heavy-quasiparticle interference imaging within this gap reveals its cause as the rapid splitting below T(o) of a light k-space band into two new heavy fermion bands. Thus, the URu(2)Si(2) 'hidden order' state emerges directly from the Fano lattice electronic structure and exhibits characteristics, not of a conventional density wave, but of sudden alterations in both the hybridization at each U atom and the associated heavy fermion states.

Detection and cloaking of molecular objects in coherent nanostructures using inelastic electron tunneling spectroscopy.

We address quantum invisibility in the context of electronics in nanoscale quantum structures. We make use of the freedom of design that quantum corrals provide and show that quantum mechanical objects can be hidden inside the corral, with respect to inelastic electron scattering spectroscopy in combination with scanning tunneling microscopy, and we propose a design strategy. A simple illustration of the invisibility is given in terms of an elliptic quantum corral containing a molecule, with a local vibrational mode, at one of the foci. Our work has implications to quantum information technology and presents new tools for nonlocal quantum detection and distinguishing between different molecules.

Tunneling into clean heavy fermion compounds: origin of the Fano line shape.

Recently observed tunneling spectra on clean heavy-fermion compounds show a lattice periodic Fano line shape similar to what is observed in the case of tunneling to a Kondo ion adsorbed at the surface. We show that the translation symmetry of a clean surface in the case of weakly correlated metals leads to a tunneling spectrum which shows a hybridization gap but does not have a Fano line shape. By contrast, in a strongly correlated heavy-fermion metal the heavy quasiparticle states will be broadened by interaction effects. The hybridization gap is completely filled in this way, and an ideal Fano line shape of width ∼2TK results. In addition, we discuss the possible influence of the tunneling tip on the surface, in (i) leading to additional broadening of the Fano line and (ii) enhancing the hybridization locally, hence adding to the impurity type behavior. The latter effects depend on the tip-surface distance.