Generation of macroscopic singlet states in a cold atomic ensemble.

We report the generation of a macroscopic singlet state in a cold atomic sample via quantum nondemolition measurement-induced spin squeezing. We observe 3 dB of spin squeezing and detect entanglement with 5σ statistical significance using a generalized spin-squeezing inequality. The degree of squeezing implies at least 50% of the atoms have formed singlets.

Feedback cooling of an atomic spin ensemble.

We apply entropy removal by measurement and feedback to a cold atomic spin ensemble. Using quantum nondemolition probing by Faraday rotation measurement, and feedback by weak optical pumping, we drive the initially random collective spin variable F toward the origin F=0. We use input-output relations and ensemble quantum noise models to describe this quantum control process and identify an optimal two-round control procedure. We observe 12 dB of spin noise reduction, or a factor-of-63 reduction in phase-space volume. The method offers a nonthermal route to generation of exotic entangled states in ultracold gases, including macroscopic singlet states and strongly correlated states of quantum lattice gases.

Efficient quantification of non-gaussian spin distributions.

We study theoretically and experimentally the quantification of non-gaussian distributions via nondestructive measurements. Using the theory of cumulants, their unbiased estimators, and the uncertainties of these estimators, we describe a quantification which is simultaneously efficient, unbiased by measurement noise, and suitable for hypothesis tests, e.g., to detect nonclassical states. The theory is applied to cold 87Rb spin ensembles prepared in non-gaussian states by optical pumping and measured by nondestructive Faraday rotation probing. We find an optimal use of measurement resources under realistic conditions, e.g., in atomic ensemble quantum memories.

Magnetic sensitivity beyond the projection noise limit by spin squeezing.

We report the generation of spin squeezing and entanglement in a magnetically sensitive atomic ensemble, and entanglement-enhanced field measurements with this system. A maximal m(f) = ± 1 Raman coherence is prepared in an ensemble of 8.5 × 10(5) laser-cooled (87)Rb atoms in the f = 1 hyperfine ground state, and the collective spin is squeezed by synthesized optical quantum nondemolition measurement. This prepares a state with large spin alignment and noise below the projection-noise level in a mixed alignment-orientation variable. 3.2 dB of noise reduction is observed and 2.0 dB of squeezing by the Wineland criterion, implying both entanglement and metrological advantage. Enhanced sensitivity is demonstrated in field measurements using alignment-to-orientation conversion.

Interaction-based quantum metrology showing scaling beyond the Heisenberg limit.

Quantum metrology aims to use entanglement and other quantum resources to improve precision measurement. An interferometer using N independent particles to measure a parameter χ can achieve at best the standard quantum limit of sensitivity, δχ ∝ N(-1/2). However, using N entangled particles and exotic states, such an interferometer can in principle achieve the Heisenberg limit, δχ ∝ N(-1). Recent theoretical work has argued that interactions among particles may be a valuable resource for quantum metrology, allowing scaling beyond the Heisenberg limit. Specifically, a k-particle interaction will produce sensitivity δχ ∝ N(-k) with appropriate entangled states and δχ ∝ N(-(k-1/2)) even without entanglement. Here we demonstrate 'super-Heisenberg' scaling of δχ ∝ N(-3/2) in a nonlinear, non-destructive measurement of the magnetization of an atomic ensemble. We use fast optical nonlinearities to generate a pairwise photon-photon interaction (corresponding to k = 2) while preserving quantum-noise-limited performance. We observe super-Heisenberg scaling over two orders of magnitude in N, limited at large numbers by higher-order nonlinear effects, in good agreement with theory. For a measurement of limited duration, super-Heisenberg scaling allows the nonlinear measurement to overtake in sensitivity a comparable linear measurement with the same number of photons. In other situations, however, higher-order nonlinearities prevent this crossover from occurring, reflecting the subtle relationship between scaling and sensitivity in nonlinear systems. Our work shows that interparticle interactions can improve sensitivity in a quantum-limited measurement, and experimentally demonstrates a new resource for quantum metrology.