Fluctuation-response relation as a probe of long-range correlations in nonequilibrium quantum and classical fluids.

The absence of a simple fluctuation-dissipation theorem is a major obstacle for studying systems that are not in thermodynamic equilibrium. We show that for a fluid in a nonequilibrium steady state characterized by a constant temperature gradient the commutator correlation functions are still related to response functions; however, the relation is to the bilinear response of products of two observables, rather than to a single linear response function as is the case in equilibrium. This modified fluctuation-response relation holds for both quantum and classical systems. It is both motivated and informed by the long-range correlations that exist in such a steady state and allows for probing them via response experiments. This is of particular interest in quantum fluids, where the direct observation of fluctuations by light scattering would be difficult. In classical fluids it is known that the coupling of the temperature gradient to the diffusive shear velocity leads to correlations of various observables, in particular temperature fluctuations, that do not decay as a function of distance, but rather extend over the entire system. We investigate the nature of these correlations in a fermionic quantum fluid and show that the crucial coupling between the temperature gradient and velocity fluctuations is the same as in the classical case. Accordingly, the nature of the long-ranged correlations in the hydrodynamic regime also is the same. However, as one enters the collisionless regime in the low-temperature limit the nature of the velocity fluctuations changes: they become ballistic rather than diffusive. As a result, correlations of the temperature and other observables are still singular in the long-wavelength limit, but the singularity is weaker than in the hydrodynamic regime.

Fluctuation-Dissipation Relation in a Nonequilibrium Quantum Fluid.

There is no simple fluctuation-dissipation theorem (FDT) for nonequilibrium systems. We show that for a fluid in a nonequilibrium steady state (NESS) characterized by a constant temperature gradient there is a generalized FDT that relates commutator correlation functions to the bilinear response of products of observables. This allows for experimental probes of the long-range correlations in such a system, quantum or classical, via response experiments. We also show that the correlations are not tied to thermal fluctuations but are intrinsic to the NESS and reflect a generalized rigidity.

Nonhydrodynamic initial conditions are not soon forgotten.

Solutions to hydrodynamic equations, which are used for a vast variety of physical problems, are assumed to be specified by boundary conditions and initial conditions on the hydrodynamic variables only. Initial values of other variables are assumed to be irrelevant for a hydrodynamic description. We show that this assumption is not correct because of the existence of long-time-tail effects that are ubiquitous in systems governed by hydrodynamic equations. We illustrate this breakdown of a hydrodynamic description by means of the simple example of diffusion in a disordered electron system.

Rigidity and Superfast Signal Propagation in Fluids and Solids in Non-Equilibrium Steady States.

In the 1980s, it was theoretically predicted that correlations of various observables in a fluid in a non-equilibrium steady state (NESS) are extraordinarily long-ranged, extending, in a well-defined sense, over the size of the system. This is to be contrasted with correlations in an equilibrium fluid, whose range is typically just a few particle diameters. These NESS correlations were later confirmed by numerous experimental studies. Unlike long-ranged correlations at critical points, these correlations are generic in the sense that they exist for any temperature as long as the system is in a NESS. In equilibrium systems, generic long-ranged correlations are caused by spontaneously broken continuous symmetries and are associated with a generalized rigidity, which in turn leads to a new propagating excitation or mode. For example, in a solid, spatial rigidity leads to transverse sound waves, while, in a superfluid, phase rigidity leads to temperature waves known as second sound at finite temperatures and phonons at zero temperature. More generally, long-ranged spatial correlations imply rigidity irrespective of their physical origin. This implies that a fluid in a NESS should also display a type of rigidity and related anomalous transport behavior. Here we show that this is indeed the case. For the particular case of a simple fluid in a constant temperature gradient, the anomalous transport behavior takes the form of a super-diffusive spread of a constant-pressure temperature perturbation. We also discuss the case of an elastic solid, where we predict a spread that is faster than ballistic.

Ferromagnetic Quantum Critical Point in Noncentrosymmetric Systems.

Ferromagnetic quantum criticality in clean metals has proven elusive due to fermionic soft modes that drive the transition first order. We show that noncentrosymmetric metals with a strong spin-orbit interaction provide a promising class of materials for realizing a ferromagnetic quantum critical point in clean systems. The spin-orbit interaction renders massive the soft modes that interfere with quantum criticality in most materials, while the absence of spatial inversion symmetry precludes the existence of new classes of soft modes that could have the same effect.

Quantum Triple Point and Quantum Critical End Points in Metallic Magnets.

In low-temperature metallic magnets, ferromagnetic (FM) and antiferromagnetic (AFM) orders can exist, adjacent to one another or concurrently, in the phase diagram of a single system. We show that universal quantum effects qualitatively alter the known phase diagrams for classical magnets. They shrink the region of concurrent FM and AFM order, change various transitions from second to first order, and, in the presence of a magnetic field, lead to either a quantum triple point where the FM, AFM, and paramagnetic phases all coexist or a quantum critical end point.

Scaling Theory of a Compressibility-Driven Metal-Insulator Transition in a Two-Dimensional Electron Fluid.

We present a scaling description of a metal-insulator transition in two-dimensional electron systems that is driven by a vanishing compressibility rather than a vanishing diffusion coefficient. A small set of basic assumptions leads to a consistent theoretical framework that is compatible with existing transport and compressibility measurements, and allows us to make predictions for other observables. We also discuss connections between these ideas and other theories of transitions to an incompressible quantum fluid.

Third Law of Thermodynamics and The Shape of the Phase Diagram for Systems With a First-Order Quantum Phase Transition.

The third law of thermodynamics constrains the phase diagram of systems with a first-order quantum phase transition. For a zero conjugate field, the coexistence curve has an infinite slope at T=0. If a tricritical point exists at T>0, then the associated tricritical wings are perpendicular to the T=0 plane, but not to the zero-field plane. These results are based on the third law and basic thermodynamics only, and are completely general. As an explicit example we consider the ferromagnetic quantum phase transition in clean metals, where a first-order quantum phase transition is commonly observed.

Disorder dependence of the ferromagnetic quantum phase transition.

We quantitatively discuss the influence of quenched disorder on the ferromagnetic quantum phase transition in metals, using a theory that describes the coupling of the magnetization to gapless fermionic excitations. In clean systems, the transition is first order below a tricritical temperature T_{tc}. Quenched disorder is predicted to suppress T_{tc} until it vanishes for residual resistivities ρ_{0} on the order of several µΩ cm for typical quantum ferromagnets. We discuss experiments that allow us to distinguish the mechanism considered from other possible realizations of a first-order transition.

Preasymptotic critical behavior and effective exponents in disordered metallic quantum ferromagnets.

We determine the preasymptotic critical behavior at the quantum ferromagnetic transition in strongly disordered metals. We find that it is given by effective power laws, in contrast to the previously analyzed asymptotic critical behavior, which is valid only in an unobservably small region. The consequences for analyzing experiments are discussed, in particular, ways to distinguish between critical behavior and Griffiths-phase effects.

Quantum phase transition in a clean two-dimensional electron system.

A quantum phase transition that was recently observed in a high-mobility silicon metal-oxide-semiconductor field-effect transistor is analyzed in terms of a scaling theory. The most striking characteristic of the transition is a divergence of the thermopower, according to an inverse linear law, as a critical value of the electron density is approached. A scaling description of this transition yields predictions about the critical behavior of other observables, e.g., the specific heat. We also explore the possibility that this transition realizes a recently predicted transition from a Fermi liquid to a non-Fermi-liquid state.

Theory of a Fermi-liquid to non-Fermi-liquid quantum phase transition in dimensions d>1.

We develop a theory for a generic instability of a Fermi liquid in dimension d>1 against the formation of a Luttinger-liquid-like state. The density of states at the Fermi level is the order parameter for the ensuing quantum phase transition, which is driven by the effective interaction strength. A scaling theory in conjunction with an effective field theory for clean electrons is used to obtain the critical behavior of observables. In the Fermi-liquid phase the order-parameter susceptibility, which is measurable by tunneling, is predicted to diverge for 1

Nature of the quantum phase transition to a spin-nematic phase.

It is shown that the quantum phase transition in metallic non-s-wave ferromagnets, or spin nematics, is generically of first order. This is due to a coupling of the order parameter to soft electronic modes that play a role analogous to that of the electromagnetic vector potential in a superconductor, which leads to a fluctuation-induced first-order transition. A generalized mean-field theory for the p-wave case is constructed that explicitly shows this effect. Tricritical wings are predicted to appear in the phase diagram in a spatially varying magnetic field, but not in a homogeneous one.

Columnar fluctuations as a source of non-Fermi-liquid behavior in weak metallic magnets.

It is shown that columnar fluctuations, in conjunction with weak quenched disorder, lead to a T{3/2} temperature dependence of the electrical resistivity. This is proposed as an explanation of the observed non-Fermi-liquid behavior in the helimagnet MnSi, with one possible realization of the columnar fluctuations provided by Skyrmion lines that have independently been proposed to be present in this material.

Criticality in inhomogeneous magnetic systems: application to quantum ferromagnets.

We consider a phi4 theory with a position-dependent distance from the critical point. One realization of this model is a classical ferromagnet subject to nonuniform mechanical stress. We find a sharp phase transition where the envelope of the local magnetization vanishes uniformly. The first-order transition in a quantum ferromagnet also remains sharp. The universal mechanism leading to a tricritical point in an itinerant quantum ferromagnet is suppressed, and in principle, one can recover a quantum critical point with mean-field exponents. Observable consequences of these results are discussed.

Elasticity and melting of skyrmion flux lattices in p-wave superconductors.

We analytically calculate the energy, magnetization curves [B(H)], and elasticity of Skyrmions flux lattices in p-wave superconductors near the lower critical field H(c1), and we use these results with the Lindemann criterion to predict their melting curve. In striking contrast to vortex flux lattices, which always melt at an external field H>H(c1), Skyrmion flux lattices never melt near H(c1). This provides a simple and unambiguous test for the presence of Skyrmions.

Blue quantum fog: chiral condensation in quantum helimagnets.

It is shown that a condensation transition involving a chiral order parameter can occur in itinerant helimagnets, in analogy to the transition between the isotropic phase and the phase known as blue fog or blue phase III in cholesteric liquid crystals. It is proposed that such a transition is the explanation for recent neutron scattering results in MnSi. Predictions are made that will allow for experimental tests of this proposal.

Breakdown of hydrodynamic transport theory in the ordered phase of helimagnets.

It is shown that strong fluctuations preclude a hydrodynamic description of transport phenomena in helimagnets, such as MnSi, at T>0. This breakdown of hydrodynamics is analogous to the one in chiral liquid crystals. Mode-mode coupling effects lead to infinite renormalizations of various transport coefficients, and the actual macroscopic description is nonlocal. At T=0 these effects are weakened due to the fluctuation-dissipation theorem, and the renormalizations remain finite. Observable consequences of these results, as manifested in the neutron scattering cross section, are discussed.

Breakdown of the perturbative renormalization group at certain quantum critical points.

It is shown that the presence of multiple time scales at a quantum critical point can lead to a breakdown of the loop expansion for critical exponents, since coefficients in the expansion diverge. Consequently, results obtained from finite-order perturbative renormalization-group treatments may not be an approximation in any sense to the true asymptotic critical behavior. This problem manifests itself as a nonrenormalizable field theory, or, equivalently, as the presence of a dangerous irrelevant variable. The quantum ferromagnetic transition in disordered metals provides an example.

Spontaneous flux lattices in ferromagnetic spin-triplet superconductors.

A theory is developed for the spontaneous vortex lattice that is expected to occur in the ferromagnetic superconductors ZrZn2, UGe2, and URhGe, where the superconductivity is likely of the spin-triplet nature. The long-wavelength fluctuations of this spontaneous flux lattice are predicted to be huge compared to those of a conventional flux lattice, and to be the same as those for spin-singlet ferromagnetic superconductors. It is shown that these fluctuations lead to unambiguous experimental signatures which may provide the easiest way to observe the spontaneous flux lattice.