ABSTRACT
Spontaneous symmetry breaking in physical systems leads to salient phenomena at all scales, from the Higgs mechanism and the emergence of the mass of the elementary particles, to superconductivity and magnetism in solids. The hidden-order state arising below 17.5 K in URu2Si2 is a puzzling example of one of such phase transitions: its associated broken symmetry and gap structure have remained longstanding riddles. Here we directly image how, across the hidden-order transition, the electronic structure of URu2Si2 abruptly reconstructs. We observe an energy gap of 7 meV opening over 70% of a large diamond-like heavy-fermion Fermi surface, resulting in the formation of four small Fermi petals, and a change in the electronic periodicity from body-centred tetragonal to simple tetragonal. Our results explain the large entropy loss in the hidden-order phase, and the similarity between this phase and the high-pressure antiferromagnetic phase found in quantum-oscillation experiments.
ABSTRACT
We study, using high-resolution angle-resolved photoemission spectroscopy, the evolution of the electronic structure in URu2Si2 at the Γ, Z, and X high-symmetry points from the high-temperature Kondo-screened regime to the low-temperature hidden-order (HO) state. At all temperatures and symmetry points, we find structures resulting from the interaction between heavy and light bands related to the Kondo-lattice formation. At the X point, we directly measure a hybridization gap of 11 meV already open at temperatures above the ordered phase. Strikingly, we find that while the HO induces pronounced changes at Γ and Z, the hybridization gap at X does not change, indicating that the hidden-order parameter is anisotropic. Furthermore, at the Γ and Z points, we observe the opening of a gap in momentum in the HO state, and show that the associated electronic structure results from the hybridization of a light electron band with the Kondo-lattice bands characterizing the paramagnetic state.
