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1.
J Chem Phys ; 160(24)2024 Jun 28.
Article in English | MEDLINE | ID: mdl-38912628

ABSTRACT

We present the results of a new analysis of the literature data on electron mobility µ in dense helium gas aimed at determining the existence of a threshold density for electron self-trapping in gaseous helium as a function of temperature. We have investigated the density dependence of µ and, when available, its dependence on the electric field. The experimental data are favorably rationalized by minimizing the excess free energy of the self-localized states within the optimum fluctuation model. It is shown that the formation of electron bubbles via the self-trapping phenomenon is determined by the delicate balance between the electron thermal energy, the density dependence of the electron energy at the bottom of the conduction band in the gas, and the work necessary to expand the bubble. We show that the self-trapping phenomenon is not limited to low temperatures but occurs at any temperatures for large enough densities.

2.
J Chem Phys ; 159(10)2023 Sep 14.
Article in English | MEDLINE | ID: mdl-37694752

ABSTRACT

We report the first ever measurements of the thermalization length of low-energy electrons injected into solid para-hydrogen at a temperature T ≈ 2.8 K. The use of the pulsed Townsend photoinjection technique has allowed us to investigate the behavior of quasi-free electrons rather than of massive, slow negative charges, as reported in all previous literature. We have found an average thermalization length ⟨z0⟩ = 26.1 nm, which is three to five times longer than that in liquid helium at the same temperature.

3.
Rev Sci Instrum ; 85(2): 023105, 2014 Feb.
Article in English | MEDLINE | ID: mdl-24593347

ABSTRACT

We report on a novel electro-optic device for the diagnostics of high repetition rate laser systems. It is composed of a microwave receiver and of a second order nonlinear crystal, whose irradiation with a train of short laser pulses produces a time-dependent polarization in the crystal itself as a consequence of optical rectification. This process gives rise to the emission of microwave radiation that is detected by a receiver and is analyzed to infer the repetition rate and intensity of the pulses. We believe that this new method may overcome some of the limitations of photodetection techniques.

4.
Opt Lett ; 38(21): 4465-8, 2013 Nov 01.
Article in English | MEDLINE | ID: mdl-24177120

ABSTRACT

We report measurements of microwave (RF) generation in the centimeter band accomplished by irradiating a nonlinear KTiOPO4 crystal with a home-made, infrared laser at 1064 nm as a result of optical rectification. The laser delivers pulse trains of duration up to 1 µs. Each train consists of several high-intensity pulses at an adjustable repetition rate of approximately 4.6 GHz. The duration of the generated RF pulses is determined by that of the pulse trains. We have investigated both microwave- and second harmonic generation as a function of the laser intensity and of the orientation of the laser polarization with respect to the crystallographic axes of KTP.

5.
J Chem Phys ; 138(3): 034309, 2013 Jan 21.
Article in English | MEDLINE | ID: mdl-23343278

ABSTRACT

Injection of photoelectrons into gaseous or liquid dielectrics is a widely used technique to produce cold plasmas in weakly ionized systems for investigating the transport properties of electrons. We report measurements of the collection efficiency of photoelectrons injected into dense argon gas for T = 152.7 K, close to the critical temperature T(c) ≈ 150.9 K, and for T = 200.0 K. The high-field data agree with the Young-Bradbury model and with previous measurements below T(c) and at an intermediate temperature above T(c). The effective, density-dependent electron-atom momentum transfer scattering cross section can be deduced. However, the weak-field data near T(c) show large deviations from the theoretical model. We show that the electron behavior at weak field is influenced by electrostriction effects that are only important near the critical point.


Subject(s)
Argon/chemistry , Electrons , Gases/chemistry , Temperature
6.
Rev Sci Instrum ; 82(9): 095103, 2011 Sep.
Article in English | MEDLINE | ID: mdl-21974615

ABSTRACT

We report on the design of a new type of hot-filament electron gun delivering fairly high current (a few hundreds of µ A) at high voltage (up to 100 kV) in continuous or pulsed mode. Its novel features are that the filament is heated by means of a pack of rechargeable batteries floated atop the high-voltage power supply in order to get rid of bulky isolation transformers, and that the filament current and, hence, the electron gun current, is controlled by a feedback circuit including a superluminescent diode decoupled from the high voltage by means of an optical fiber. This electron gun is intended for general purposes, although we have especially developed it to meet the needs of our experiment on the infrared emission spectroscopy of rare gas excimers. Our experiment requires that the charge injection into the sample is pulsed and constant and stable in time. The new electron gun can deliver several tens of nC per pulse of electrons of energy up to 100 keV into the sample cell. The new design also eliminates ripples in the emission current and ensures up to 12 h of stable performance.

7.
Phys Rev E Stat Nonlin Soft Matter Phys ; 65(5 Pt 2): 056403, 2002 May.
Article in English | MEDLINE | ID: mdl-12059711

ABSTRACT

We report accurate measurements of the mobility of excess electrons in high-density helium gas in extended ranges of temperature [(26 < or = T < or = 77) K] and density [(0.05 < or = N < or = 10.0) atoms nm(-3)]. The aim is the investigation of the combined effect of temperature and density on the formation and dynamics of localized electron states. The main result of the experiment is that the formation of localized states essentially depends on the relative balance of fluid dilation energy, repulsive electron-atom interaction energy, and thermal energy. As a consequence, the onset of localization depends on the medium disorder through gas temperature and density. The transition from delocalized to localized states shifts to larger densities as temperature is increased. This behavior can be understood in terms of a simple model of electron self-trapping in a spherically symmetric square well.

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