Room-Temperature Antiferromagnetic Resonance and Inverse Spin-Hall Voltage in Canted Antiferromagnets.

We study theoretically and experimentally the spin pumping signals induced by the resonance of canted antiferromagnets with Dzyaloshinskii-Moriya interaction and demonstrate that they can generate easily observable inverse spin-Hall voltages. Using a bilayer of hematite/heavy metal as a model system, we measure at room temperature the antiferromagnetic resonance and an associated inverse spin-Hall voltage, as large as in collinear antiferromagnets. As expected for coherent spin pumping, we observe that the sign of the inverse spin-Hall voltage provides direct information about the mode handedness as deduced by comparing hematite, chromium oxide and the ferrimagnet yttrium-iron garnet. Our results open new means to generate and detect spin currents at terahertz frequencies by functionalizing antiferromagnets with low damping and canted moments.

Long-distance spin-transport across the Morin phase transition up to room temperature in ultra-low damping single crystals of the antiferromagnet α-Fe2O3.

Antiferromagnetic materials can host spin-waves with polarizations ranging from circular to linear depending on their magnetic anisotropies. Until now, only easy-axis anisotropy antiferromagnets with circularly polarized spin-waves were reported to carry spin-information over long distances of micrometers. In this article, we report long-distance spin-transport in the easy-plane canted antiferromagnetic phase of hematite and at room temperature, where the linearly polarized magnons are not intuitively expected to carry spin. We demonstrate that the spin-transport signal decreases continuously through the easy-axis to easy-plane Morin transition, and persists in the easy-plane phase through current induced pairs of linearly polarized magnons with dephasing lengths in the micrometer range. We explain the long transport distance as a result of the low magnetic damping, which we measure to be ≤ 10-5 as in the best ferromagnets. All of this together demonstrates that long-distance transport can be achieved across a range of anisotropies and temperatures, up to room temperature, highlighting the promising potential of this insulating antiferromagnet for magnon-based devices.

Current-Driven Dynamics of Magnetic Hopfions.

Topological magnetic textures have attracted considerable interest since they exhibit new properties and might be useful in information technology. Magnetic hopfions are three-dimensional (3D) spatial variations in the magnetization with a nontrivial Hopf index. We find that, in ferromagnetic materials, two types of hopfions, Bloch-type and Néel-type hopfions, can be excited as metastable states in the presence of bulk and interfacial Dzyaloshinskii-Moriya interactions, respectively. We further investigate how hopfions can be driven by currents via spin-transfer torques (STTs) and spin-Hall torques (SHTs). Distinct from 2D ferromagnetic skyrmions, hopfions have a vanishing gyrovector. Consequently, there are no undesirable Hall effects. Néel-type hopfions move along the current direction via both STT and SHT, while Bloch-type hopfions move either transverse to the current direction via SHT or parallel to the current direction via STT. Our findings open the door to utilizing hopfions as information carriers.

Angle Resolved Relaxation of Spin Currents by Antiferromagnets in Spin Valves.

We observe and analyze tunable relaxation of a pure spin current by an antiferromagnet in spin valves. This is achieved by carefully controlling the angle between a resonantly excited ferromagnetic layer pumping the spin current and the Néel vector of the antiferromagnetic layer. The effect is observed as an angle-dependent spin-pumping contribution to the ferromagnetic resonance linewidth. An interplay between spin-mixing conductance and, often disregarded, longitudinal spin conductance is found to underlie our observations, which is in agreement with a recent prediction for related ferromagnetic spin valves.

Tunable long-distance spin transport in a crystalline antiferromagnetic iron oxide.

Spintronics relies on the transport of spins, the intrinsic angular momentum of electrons, as an alternative to the transport of electron charge as in conventional electronics. The long-term goal of spintronics research is to develop spin-based, low-dissipation computing-technology devices. Recently, long-distance transport of a spin current was demonstrated across ferromagnetic insulators1. However, antiferromagnetically ordered materials, the most common class of magnetic materials, have several crucial advantages over ferromagnetic systems for spintronics applications2: antiferromagnets have no net magnetic moment, making them stable and impervious to external fields, and can be operated at terahertz-scale frequencies3. Although the properties of antiferromagnets are desirable for spin transport4-7, indirect observations of such transport indicate that spin transmission through antiferromagnets is limited to only a few nanometres8-10. Here we demonstrate long-distance propagation of spin currents through a single crystal of the antiferromagnetic insulator haematite (α-Fe2O3)11, the most common antiferromagnetic iron oxide, by exploiting the spin Hall effect for spin injection. We control the flow of spin current across a haematite-platinum interface-at which spins accumulate, generating the spin current-by tuning the antiferromagnetic resonance frequency using an external magnetic field12. We find that this simple antiferromagnetic insulator conveys spin information parallel to the antiferromagnetic Néel order over distances of more than tens of micrometres. This mechanism transports spins as efficiently as the most promising complex ferromagnets1. Our results pave the way to electrically tunable, ultrafast, low-power, antiferromagnetic-insulator-based spin-logic devices6,13 that operate without magnetic fields at room temperature.

Asymmetric and Symmetric Exchange in a Generalized 2D Rashba Ferromagnet.

Dzyaloshinskii-Moriya interaction (DMI) is investigated in a 2D ferromagnet (FM) with spin-orbit interaction of Rashba type at finite temperatures. The FM is described in the continuum limit by an effective s-d model with arbitrary dependence of spin-orbit coupling (SOC) and kinetic energy of itinerant electrons on the absolute value of momentum. In the limit of weak SOC, we derive a general expression for the DMI constant D from a microscopic analysis of the electronic grand potential. We compare D with the exchange stiffness A and show that, to the leading order in small SOC strength α_{R}, the conventional relation D=(4mα_{R}/ℏ)A, in general, does not hold beyond the Bychkov-Rashba model. Moreover, in this model, both A and D vanish at zero temperature in the metal regime (i.e., when two spin sub-bands are partly occupied). For nonparabolic bands or nonlinear Rashba coupling, these coefficients are finite and acquire a nontrivial dependence on the chemical potential that demonstrates the possibility to control the size and chirality of magnetic textures by adjusting a gate voltage.

Finite-element theory of transport in ferromagnet-normal metal systems

We formulate a theory of spin dependent transport in an electronic circuit involving ferromagnetic elements with noncollinear magnetization which is based on the conservation of spin and charge current. The theory considerably simplifies the calculation of the transport properties of complicated ferromagnet-normal metal systems. We illustrate the theory by considering a novel three-terminal device.