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1.
Environ Int ; 135: 105404, 2020 02.
Article in English | MEDLINE | ID: mdl-31865278

ABSTRACT

Landfill leachates are identified as a significant source of pharmaceutical and personal care products (PPCPs), which might pose a threat to groundwater and surface water nearby the landfill. However, knowledge of PPCP contamination in the surrounding water environment of landfills is very limited. Here we investigated eighteen PPCPs in water environment near the largest landfill in China, focusing on their occurrences and spatial distribution, as well as the environmental risks. The results showed the concentration of target PPCPs was below the limit of quantification (

Subject(s)
Cosmetics , China , Environmental Monitoring , Groundwater , Pharmaceutical Preparations , Waste Disposal Facilities , Water Pollutants, Chemical
2.
J Hazard Mater ; 323(Pt A): 99-108, 2017 Feb 05.
Article in English | MEDLINE | ID: mdl-27017099

ABSTRACT

Knowledge on the pharmaceuticals and personal care products (PPCPs) in landfill leachates, which are an important source of PPCPs in the environment, was very limited. Hence, four sampling campaigns were conducted to determine eighteen PPCPs in the landfill leachates from a landfill reservoir in Shanghai. Five of the target PPCPs were first included in a landfill leachate study. Additionally, their removal from landfill leachates by a full-scale membrane bioreactor (MBR) was illustrated. The results showed fourteen out of eighteen PPCPs were detectable in at least one sampling campaign and achieved individual concentrations ranging from 0.39 to 349µg/L in the landfill leachates. Some PPCPs exhibited higher contamination levels than those reported in other countries. Good removal of PPCPs by MBR led to a largely reduced contamination level (

Subject(s)
Bioreactors , Cosmetics/analysis , Pharmaceutical Preparations/analysis , Refuse Disposal/methods , Waste Disposal Facilities , Water Pollutants, Chemical/analysis , Biodegradation, Environmental , China , Cities , Feasibility Studies
3.
Environ Sci Pollut Res Int ; 22(8): 6086-94, 2015 Apr.
Article in English | MEDLINE | ID: mdl-25391230

ABSTRACT

Ten pharmaceuticals and two consumer products were investigated in four wastewater treatment plants (WWTPs) in Shanghai, China. The concentrations of target compounds in the wastewater influents ranged from below the limit of quantification (LOQ) to 9340 ng/L, with the frequency of detection of 31-100%, and the removal efficiencies were observed to be -82 to 100% in the four WWTPs. Concentrations of most target compounds (i.e. diclofenac, caffeine, metoprolol, sulpiride) in the wastewater influents were around three to eight times higher in urban WWTPs than in suburb ones, probably due to the different population served and lifestyles. Mean concentrations of target compounds in the wastewater influent generally decreased by 5-76% after rainfall due to the dilution of raw sewage by rainwater, which infiltrated into the sewer system. In the WWTPs located in the suburb area, the increased flow of wastewater influent led to a shortened hydraulic retention time (HRT) and decreased removal efficiencies of some compounds. On the contrary, the influence of rainfall was not significant on the removal efficiencies of investigated compounds in urban WWTPs, probably due to the almost unchanged influent flow, good removal performance, or bypass system employed.


Subject(s)
Bioreactors , Cities , Environmental Monitoring/statistics & numerical data , Wastewater/chemistry , Water Pollutants, Chemical/analysis , Water Purification/methods , China , Chromatography, High Pressure Liquid , Environmental Monitoring/methods , Household Products/analysis , Pharmaceutical Preparations/analysis , Quality Control , Rain , Sewage , Solid Phase Extraction , Tandem Mass Spectrometry , Time Factors
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