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1.
Opt Express ; 31(6): 9437-9447, 2023 Mar 13.
Article in English | MEDLINE | ID: mdl-37157515

ABSTRACT

Quantum key distribution (QKD) allows the distribution of cryptographic keys between multiple users in an information-theoretic secure way, exploiting quantum physics. While current QKD systems are mainly based on attenuated laser pulses, deterministic single-photon sources could give concrete advantages in terms of secret key rate (SKR) and security owing to the negligible probability of multi-photon events. Here, we introduce and demonstrate a proof-of-concept QKD system exploiting a molecule-based single-photon source operating at room temperature and emitting at 785 nm. With an estimated maximum SKR of 0.5 Mbps, our solution paves the way for room-temperature single-photon sources for quantum communication protocols.

2.
ACS Nano ; 12(5): 4295-4303, 2018 05 22.
Article in English | MEDLINE | ID: mdl-29630340

ABSTRACT

Quantum technologies could largely benefit from the control of quantum emitters in sub-micrometric size crystals. These are naturally prone to integration in hybrid devices, including heterostructures and complex photonic devices. Currently available quantum emitters in nanocrystals suffer from spectral instability, preventing their use as single-photon sources for most quantum optics operations. In this work we report on the performances of single-photon emission from organic nanocrystals (average size of hundreds of nm), made of anthracene (Ac) and doped with dibenzoterrylene (DBT) molecules. The source has hours-long photostability with respect to frequency and intensity, both at room and at cryogenic temperature. When cooled to 3 K, the 00-zero phonon line shows linewidth values (50 MHz) close to the lifetime limit. Such optical properties in a nanocrystalline environment recommend the proposed organic nanocrystals as single-photon sources for integrated photonic quantum technologies.

3.
Light Sci Appl ; 6(4): e16245, 2017 Apr.
Article in English | MEDLINE | ID: mdl-30167241

ABSTRACT

The efficient interaction of light with quantum emitters is crucial to most applications in nano and quantum photonics, such as sensing or quantum information processing. Effective excitation and photon extraction are particularly important for the weak signals emitted by a single atom or molecule. Recent works have introduced novel collection strategies, which demonstrate that large efficiencies can be achieved by either planar dielectric antennas combined with high numerical aperture objectives or optical nanostructures that beam emission into a narrow angular distribution. However, the first approach requires the use of elaborate collection optics, while the latter is based on accurate positioning of the quantum emitter near complex nanoscale architectures; hence, sophisticated fabrication and experimental capabilities are needed. Here we present a theoretical and experimental demonstration of a planar optical antenna that beams light emitted by a single molecule, which results in increased collection efficiency at small angles without stringent requirements on the emitter position. The proposed device exhibits broadband performance and is spectrally scalable, and it is simple to fabricate and therefore applies to a wide range of quantum emitters. Our design finds immediate application in spectroscopy, quantum optics and sensing.

4.
Phys Rev Lett ; 104(5): 050403, 2010 Feb 05.
Article in English | MEDLINE | ID: mdl-20366751

ABSTRACT

We present the proposition of an experiment in which the multiphoton quantum superposition consisting of N approximately 10{5} particles generated by a quantum-injected optical parametric amplifier, seeded by a single-photon belonging to an Einstein-Podolsky-Rosen entangled pair, is made to interact with a mirror-Bose-Einstein condensate (BEC) shaped as a Bragg interference structure. The overall process will realize a macroscopic quantum superposition involving a microscopic single-photon state of polarization entangled with the coherent macroscopic transfer of momentum to the BEC structure, acting in spacelike separated distant places.

5.
Phys Rev Lett ; 104(7): 073601, 2010 Feb 19.
Article in English | MEDLINE | ID: mdl-20366880

ABSTRACT

The radiation pressure coupling between a low-mass moving mirror and an incident light field has been experimentally studied in a high-finesse Fabry-Perot cavity. Using classical intensity noise in order to mimic radiation pressure quantum fluctuations, the physics of ponderomotive squeezing comes into play as a result of the opto-mechanical correlations between the field quadratures. The same scheme can be used to probe ponderomotive squeezing at the quantum level, thus opening new routes in quantum optics and high sensitivity measurement experiments.

6.
Phys Rev Lett ; 95(6): 063201, 2005 Aug 05.
Article in English | MEDLINE | ID: mdl-16090948

ABSTRACT

In the present work we demonstrate how to realize a 1D closed optical lattice experimentally, including a tunable boundary phase twist. The latter may induce "persistent currents" visible by studying the atoms' momentum distribution. We show how important phenomena in 1D physics can be studied by physical realization of systems of trapped atoms in ring-shaped optical lattices. A mixture of bosonic and/or fermionic atoms can be loaded into the lattice, realizing a generic quantum system of many interacting particles.

7.
Phys Rev Lett ; 90(19): 197902, 2003 May 16.
Article in English | MEDLINE | ID: mdl-12785986

ABSTRACT

We present here an all-optical scheme for the experimental realization of a quantum phase gate. It is based on the polarization degree of freedom of two traveling single-photon wave packets and exploits giant Kerr nonlinearities that can be attained in coherently driven ultracold atomic media.

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