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1.
Sci Adv ; 6(13): eaax9480, 2020 Mar.
Article in English | MEDLINE | ID: mdl-32258393

ABSTRACT

Van der Waals materials offer unprecedented control of electronic properties via stacking of different types of two-dimensional materials. A fascinating frontier, largely unexplored, is the stacking of strongly correlated phases of matter. We study 4Hb-TaS2, which naturally realizes an alternating stacking of 1T-TaS2 and 1H-TaS2 structures. The former is a well-known Mott insulator, which has recently been proposed to host a gapless spin-liquid ground state. The latter is a superconductor known to also host a competing charge density wave state. This raises the question of how these two components affect each other when stacked together. We find a superconductor with a T c of 2.7 Kelvin and anomalous properties, of which the most notable one is a signature of time-reversal symmetry breaking, abruptly appearing at the superconducting transition. This observation is consistent with a chiral superconducting state.

2.
Sci Adv ; 3(4): e1602372, 2017 Apr.
Article in English | MEDLINE | ID: mdl-28439547

ABSTRACT

The crossover from Bardeen-Cooper-Schrieffer (BCS) superconductivity to Bose-Einstein condensation (BEC) is difficult to realize in quantum materials because, unlike in ultracold atoms, one cannot tune the pairing interaction. We realize the BCS-BEC crossover in a nearly compensated semimetal, Fe1+y Se x Te1-x , by tuning the Fermi energy εF via chemical doping, which permits us to systematically change Δ/εF from 0.16 to 0.50, where Δ is the superconducting (SC) gap. We use angle-resolved photoemission spectroscopy to measure the Fermi energy, the SC gap, and characteristic changes in the SC state electronic dispersion as the system evolves from a BCS to a BEC regime. Our results raise important questions about the crossover in multiband superconductors, which go beyond those addressed in the context of cold atoms.

3.
Phys Rev Lett ; 92(25 Pt 1): 257007, 2004 Jun 25.
Article in English | MEDLINE | ID: mdl-15245055

ABSTRACT

Using the transverse field muon spin relaxation technique, we measure the temperature dependence of the magnetic field penetration depth lambda, in the NaxCoO2.yH(2)O system. We find that lambda, which is determined by the superfluid density n(s) and the effective mass m*, is very small and on the edge of the TF-microSR sensitivity. Nevertheless, the results indicate that this system obeys the Uemura relation. By comparing lambda with the normal state electron density, we conclude that m* of the superconductivity carrier is 70 times larger than the mass of bare electrons. Finally, the order parameter in this system cannot be described by a complete gap over the entire Fermi surface.

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