ABSTRACT
Isolated attosecond pulse (IAP) generation usually involves the use of short-medium gas cells operated at high pressures. In contrast, long-medium schemes at low pressures are commonly perceived as inherently unsuitable for IAP generation due to the nonlinear phenomena that challenge favourable phase-matching conditions. Here we provide clear experimental evidence on the generation of isolated extreme-ultraviolet attosecond pulses in a semi-infinite gas cell, demonstrating the use of extended-medium geometries for effective production of IAPs. To gain a deeper understanding we develop a simulation method for high-order harmonic generation (HHG), which combines nonlinear propagation with macroscopic HHG solving the 3D time-dependent Schrödinger equation at the single-atom level. Our simulations reveal that the nonlinear spatio-temporal reshaping of the driving field, observed in the experiment as a bright plasma channel, acts as a self-regulating mechanism boosting the phase-matching conditions for the generation of IAPs.
ABSTRACT
The improvement of techniques for the generation of near-infrared (NIR) few-cycle pulses is paving the way for new scenarios in time-resolved spectroscopy and the generation of ultrashort extreme-ultraviolet pulses through high-harmonic generation. In this work, we numerically study how to optimize the self-compression of NIR pulses using decreasing pressure gradients in hollow capillary fibers (HCFs). We identify a moderate nonlinear regime in which sub-cycle pulses are obtained with very good temporal quality from an input 30 fs pulse centered at a 800 nm wavelength and coupled as the fundamental mode of an argon-filled HCF fully evacuated at the output end. Surprisingly, we observe that there is a relatively broad region of parameters for which the optimum self-compression takes place, defined by a simple relation between the input pulse energy and the initial gas pressure.
ABSTRACT
The collapse of a laser beam propagating inside a hollow-core fiber is investigated by numerically solving different nonlinear propagation models. We have identified that the fiber confinement favors the spatial collapse, especially in case of pulses with the input peak power close to the critical value. We have also observed that when using pulses in the femtosecond range, the temporal dynamics plays an important role, activating the spatial collapse even for pulses with input peak powers below the critical value. The complex self-focusing dynamics observed in the region below the critical power depends on the temporal evolution of the pulse and, also, on the interaction between the different spatial modes of the hollow-core fiber.
ABSTRACT
The response of a hydrogen atom submitted to a multiharmonic laser field is studied. The relative phases of the harmonic components are critical both for atomic ionization and high-order harmonic generation. In the phase-locked case under adequate interference conditions, the inhibition of ionization is followed by an increase of the intensities of the generated harmonics.