ABSTRACT
Entangled two-photon absorption (ETPA) has recently become a topic of lively debate, mainly due to the apparent inconsistencies in the experimentally reported ETPA cross sections of organic molecules obtained by a number of groups. In this work, we provide a thorough experimental study of ETPA in the organic molecules Rhodamine B (RhB) and zinc tetraphenylporphirin (ZnTPP). Our contribution is 3-fold: first, we reproduce previous results from other groups; second, we on the one hand determine the effects of different temporal correlationsâintroduced as a controllable temporal delay between the signal and idler photons to be absorbedâon the strength of the ETPA signal, and on the other hand, we introduce two concurrent and equivalent detection systems with and without the sample in place as a useful experimental check; third, we introduce, and apply to our data, a novel method to quantify the ETPA rate based on taking into account the full photon-pair behavior rather than focusing on singles or coincidence counts independently. Through this experimental setup we find that, surprisingly, the purported ETPA signal is not suppressed for a temporal delay much greater than the characteristic photon-pair temporal correlation time. While our results reproduce the previous findings from other authors, our full analysis indicates that the signal observed is not actually due to ETPA but simply to linear losses. Interestingly, for higher RhB concentrations, we find a two-photon signal that, contrary to expectations, likewise does not correspond to ETPA.
ABSTRACT
We experimentally observe the stimulated analogue of Hawking radiation produced in a photonic-crystal fiber, with a pulsed pump and a continuous-wave probe. In particular, we propose and demonstrate an innovative method to boost the efficiency and probe the coherence characteristics of the analogue Hawking effect relying on a double pump pulse with a controlled temporal delay. We show that the emitted analogue Hawking radiation corresponds to the coherently-added, interfering Hawking signals resulting from the probe interacting with each pump pulse. We introduce a simple effective Michelson interference model, and demonstrate excellent agreement between our experimental data and the predictions derived from this model. Importantly, while naively increasing the pump power in an attempt to boost the Hawking-radiation generation efficiency results in the distortion of the output signal, we show that at the maxima of the observed Hawking-signal interference pattern, the signal can be increased by a factor of >3 (up to 4 under ideal experimental conditions). This approach could be extended to the use of sequences of m pulses, resulting in a Hawking-signal enhancement of m2.
ABSTRACT
We present spatially-resolved observations of orbital angular momentum (OAM) conservation, via a Laguerre-Gauss (LG) basis decomposition, of spatially-entangled photon pairs produced in type-I collinear spontaneous parametric downconversion (SPDC). These results were obtained with a novel detection system for OAM-entangled photon pairs that combines a projective measurement for the signal photon to a specific value of the azimuthal index ls, with a spatially-resolved measurement for the idler photon using an intensified charge coupled (ICCD) camera. In combination with far-field diffraction of the idler photon through a triangular aperture, we are able to obtain: i) the spatial structure of the heralded idler photon, as governed by the user-selected topological charge of the signal photon; ii) the OAM spectrum; and iii) the topological charge (both magnitude and sign) for the heralded idler photon.
ABSTRACT
We show that an optical vortex beam, implemented classically, can be transferred to the transverse amplitude of a heralded single photon. For this purpose we have relied on the process of spontaneous parametric downconversion (SPDC) for the generation of signal and idler photon pairs, using a pump in the form of a Bessel-Gauss (BG) beam with orbital angular momentum (specifically, with topological charge l = 1 and l = 2). We have designed our source so that it operates within the short SPDC crystal regime for which, the amplitude and phase of the pump may be transferred to a heralded single photon. In order to verify the vortex nature of our heralded single photon, we have shown that the conditional angular spectrum and the transverse intensity at the single-photon level match similar measurements carried out for the pump. In addition, we have shown that when our heralded single photon is diffracted through a triangular aperture, the far-field single-photon transverse intensity exhibits the expected triangular arrangement of intensity lobes associated with the presence of orbital angular momentum.
ABSTRACT
We present an experimental and theoretical study of photon pairs generated by spontaneous four-wave mixing (SFWM), based on birefringent phasematching, in a fiber that supports more than one transverse mode. We present SFWM spectra, obtained through single-channel and coincidence photon counting, which exhibit multiple peaks shown here to be the result of multiple SFWM processes associated with different combinations of transverse modes for the pump, signal, and idler waves.
ABSTRACT
We demonstrate the generation of non-diffracting heralded single photons, i.e. which are characterized by a single-photon transverse intensity distribution which remains essentially unchanged over a significant propagation distance. For this purpose we have relied on the process of spontaneous parametric downconversion (SPDC) for the generation of signal and idler photon pairs, where our SPDC crystal is pumped by a Bessel-Gauss (BG) beam. Our experiment shows that the well-understood non-diffracting behavior of a BG beam may be directly mapped to the signal-mode, single photons heralded by the detection of a single idler photon. In our experiment, the heralded single photon is thus arranged to be non-diffracting without the need for projecting its single-photon transverse amplitude, post-generation, in any manner.
