Background-free imaging of plasmonic structures with cross-polarized apertureless scanning near-field optical microscopy.

We present advances in experimental techniques of apertureless scanning near-field optical microscopy (aSNOM). The rational alignment procedure we outline is based upon a phase singularity that occurs while scanning polarizers around the nominal cross-polarized configuration of s-polarized excitation and p-polarized detection. We discuss the theoretical origin of this topological feature of the setup, which is robust against small deviations, such as minor tip misalignment or shape variations. Setting the polarizers to this singular configuration point eliminates all background signal, allowing for reproducible plasmonic eigenmode mapping with optimal signal-to-noise ratio.

Direct near-field optical imaging of higher order plasmonic resonances.

We map in real space and by purely optical means near-field optical information of localized surface plasmon polariton (LSPP) resonances excited in nanoscopic particles. We demonstrate that careful polarization control enables apertureless scanning near-field optical microscopy (aSNOM) to image dipolar and quadrupolar LSPPs of the bare sample with high fidelity in both amplitude and phase. This establishes a routine method for in situ optical microscopy of plasmonic and other resonant structures under ambient conditions.

Amplitude- and phase-resolved optical near fields of split-ring-resonator-based metamaterials.

We investigate the local optical response of split-ring resonator-(SRR)-based metamaterials with an apertureless scanning near-field optical microscope. By mapping the near fields of suitably resonant micrometer-sized SRRs in the near-infrared spectral region with an uncoated silicon tip, we obtain a spatial resolution of better than lambda/50. The experimental results confirm numerical predictions of the near-field excitations of SRRs. Combining experimental near-field optical studies with near- and far-field optical simulations provides a detailed understanding of resonance mechanisms in subwavelength structures and will facilitate an efficient approach to improved designs.