ABSTRACT
Two-dimensional spectroscopy is performed on a terahertz (THz) frequency quantum cascade laser (QCL) with two broadband THz pulses. Gain switching is used to amplify the first THz pulse and the second THz pulse is used to probe the system. Fourier transforms are taken with respect to the delay time between the two THz pulses and the sampling time of the THz probe pulse. The two-dimensional spectrum consists of three peaks at (ωτ = 0, ωt = ω0), (ωτ = ω0, ωt = ω0), and (ωτ = 2ω0, ωt = ω0) where ω0 denotes the lasing frequency. The peak at ωτ = 0 represents the response of the probe to the zero-frequency (rectified) component of the instantaneous intensity and can be used to measure the gain recovery.
ABSTRACT
Dispersion control is a key objective in the field of photonics and spectroscopy, since it enhances non-linear effects by both enabling phase matching and offering slow light generation. In addition, it is essential for frequency comb generation, which requires a phase-lock mechanism that is provided by broadband compensation of group velocity dispersion (GVD). At optical frequencies, there are several well-established concepts for dispersion control such as prism or grating pairs. However, terahertz dispersion control is still a challenge, thus hindering further progress in the field of terahertz science and technology. In this work, we present a hybrid waveguide with both broadband, tuneable positive and more than octave-spanning negative terahertz GVD on the order of 10-22 s2/m, which is suitable for either intra- or extra cavity operation. This new terahertz device will enable ultra-short pulse compression, allow soliton propagation, improve frequency comb operation and foster the development of novel non-linear applications.
