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Phys Chem Chem Phys ; 25(33): 21981-21992, 2023 Aug 23.
Article in English | MEDLINE | ID: mdl-37555236

ABSTRACT

Many diverse technological applications, such as soft robotics and flexible electronics, demand the development of intelligent sensors that can simultaneously detect different physical parameters. Taking advantage of plasmonic structures, which can experience minute variations in physical parameters upon close contact, herein, a dual channel based silver nanostructure of concentric square rings and disks on an SiO2 substrate is proposed for the synchronized detection of magnetic field (H) and temperature (T). The thermometric polydimethylsiloxane (PDMS) and ferromagnetic Fe3O4 were placed in two channels of the nanostructure, forming the sensor. The structure modeling and electromagnetic study were carried out using the finite element method (FEM). The simultaneous detection of H and T was realized through the sensing matrix, which solved the problem of cross-sensitivity caused by a variation in temperature. Furthermore, the impact of structural asymmetry on the performance of the sensor was studied by tuning its geometrical parameters, such as disk length and ring length, separately and together. Asymmetry and the channel size significantly enhanced the performance, where disk optimization increased the temperature and magnetic field sensitivity by about 760 and 8319 times using 70% and 80% asymmetric systems, respectively. Also, the smallest ΔW (5 nm) provided a sufficiently high channel separation factor of about 7.47 µm during multi-parameter sensing. In addition, asymmetric sensing toward a single parameter was tested by placing PDMS/Fe3O4 on both channels. Multiple peaks were displayed with high sensitivity and CH-factor, making the detection more specific. Thus, the system possessing a combination of narrow channels and unique channel asymmetry exhibited excellent multi- and single-sensing for the detection of temperature and magnetic field.

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