Sensitivity and spectral control of network lasers.

Recently, random lasing in complex networks has shown efficient lasing over more than 50 localised modes, promoted by multiple scattering over the underlying graph. If controlled, these network lasers can lead to fast-switching multifunctional light sources with synthesised spectrum. Here, we observe both in experiment and theory high sensitivity of the network laser spectrum to the spatial shape of the pump profile, with some modes for example increasing in intensity by 280% when switching off 7% of the pump beam. We solve the nonlinear equations within the steady state ab-initio laser theory (SALT) approximation over a graph and we show selective lasing of around 90% of the strongest intensity modes, effectively programming the spectrum of the lasing networks. In our experiments with polymer networks, this high sensitivity enables control of the lasing spectrum through non-uniform pump patterns. We propose the underlying complexity of the network modes as the key element behind efficient spectral control opening the way for the development of optical devices with wide impact for on-chip photonics for communication, sensing, and computation.

Dye Stabilization and Wavelength Tunability in Lasing Fibers Based on DNA.

Lasers based on biological materials are attracting an increasing interest in view of their use in integrated and transient photonics. Deoxyribonucleic acid (DNA) as optical biopolymer in combination with highly emissive dyes has been reported to have excellent potential in this respect. However, achieving miniaturized lasing systems based on solid-state DNA shaped in different geometries to confine and enhance emission is still a challenge, and the physicochemical mechanisms originating fluorescence enhancement are not fully understood. Herein, a class of wavelength-tunable lasers based on DNA nanofibers is demonstrated, for which optical properties are highly controlled through the system morphology. A synergistic effect is highlighted at the basis of lasing action. Through a quantum chemical investigation, it is shown that the interaction of DNA with the encapsulated dye leads to hindered twisting and suppressed channels for the nonradiative decay. This is combined with effective waveguiding, optical gain, and tailored mode confinement to promote morphologically controlled lasing in DNA-based nanofibers. The results establish design rules for the development of bright and tunable nanolasers and optical networks based on DNA nanostructures.

A nanophotonic laser on a graph.

Conventional nanophotonic schemes minimise multiple scattering to realise a miniaturised version of beam-splitters, interferometers and optical cavities for light propagation and lasing. Here instead, we introduce a nanophotonic network built from multiple paths and interference, to control and enhance light-matter interaction via light localisation. The network is built from a mesh of subwavelength waveguides, and can sustain localised modes and mirror-less light trapping stemming from interference over hundreds of nodes. With optical gain, these modes can easily lase, reaching ~100 pm linewidths. We introduce a graph solution to the Maxwell's equation which describes light on the network, and predicts lasing action. In this framework, the network optical modes can be designed via the network connectivity and topology, and lasing can be tailored and enhanced by the network shape. Nanophotonic networks pave the way for new laser device architectures, which can be used for sensitive biosensing and on-chip optical information processing.

Metal-Dielectric Parabolic Antenna for Directing Single Photons.

Quantum emitters radiate light omni-directionally, making it hard to collect and use the generated photons. Here, we propose a three-dimensional metal-dielectric parabolic antenna surrounding an individual quantum dot as a source of collimated single photons, which can then be easily extracted and manipulated. Our fabrication method relies on a single optically induced polymerization step once the selected emitter has been localized by confocal microscopy. Compared to conventional nanoantennas, our geometry does not require near-field coupling, and it is, therefore, very robust against misalignment issues and minimally affected by absorption in the metal. The parabolic antenna provides one of the largest reported experimental directivities ( D = 106) and the lowest beam divergences (Θ1/2 = 13.5°) and a broadband operation over all of the visible and near-infrared range together with extraction efficiency of more than 96%, offering a practical advantage for quantum technological applications.

Modal Coupling of Single Photon Emitters Within Nanofiber Waveguides.

Nanoscale generation of individual photons in confined geometries is an exciting research field aiming at exploiting localized electromagnetic fields for light manipulation. One of the outstanding challenges of photonic systems combining emitters with nanostructured media is the selective channelling of photons emitted by embedded sources into specific optical modes and their transport at distant locations in integrated systems. Here, we show that soft-matter nanofibers, electrospun with embedded emitters, combine subwavelength field localization and large broadband near-field coupling with low propagation losses. By momentum spectroscopy, we quantify the modal coupling efficiency identifying the regime of single-mode coupling. These nanofibers do not rely on resonant interactions, making them ideal for room-temperature operation, and offer a scalable platform for future quantum information technology.

Tuning random lasing in photonic glasses.

We present a detailed numerical investigation of the tunability of a diffusive random laser when Mie resonances are excited. We solve a multimode diffusion model and calculate multiple light scattering in presence of optical gain that includes dispersion in both scattering and gain, without any assumptions about the ß parameter. This allows us to investigate a realistic photonic glass made of latex spheres and rhodamine and to quantify both the lasing wavelength tunability range and the lasing threshold. Beyond what is expected by diffusive monochromatic models, the highest threshold is found when the competition between the lasing modes is strongest and not when the lasing wavelength is furthest from the maximum of the gain curve.

Percolating plasmonic networks for light emission control.

Optical nanoantennas have revolutionised the way we manipulate single photons emitted by individual light sources in a nanostructured photonic environment. Complex plasmonic architectures allow for multiscale light control by shortening or stretching the light wavelength for a fixed operating frequency, meeting the size of the emitter and that of propagating modes. Here, we study self-assembled semi-continuous gold films and lithographic gold networks characterised by large local density of optical state (LDOS) fluctuations around the electrical percolation threshold, a regime where the surface is characterised by large metal clusters with fractal topology. We study the formation of plasmonic networks and their effect on light emission from embedded fluorescent probes in these systems. Through fluorescence dynamics experiments we discuss the role of global long-range interactions linked to the degree of percolation and to the network fractality, as well as the local near-field contributions coming from the local electro-magnetic fields and the topology. Our experiments indicate that local properties dominate the fluorescence modification.

Integrated architecture for the electrical detection of plasmonic resonances based on high electron mobility photo-transistors.

We report the design of an integrated platform for on-chip electrical transduction of the surface plasmon resonance supported by a nanostructured metal grating. The latter is fabricated on the active area of a GaAs/AlGaAs photo-HEMT and simultaneously works as the electronic gate of the device. The gold plasmonic crystal has a V-groove profile and has been designed by numerical optical simulations. By showing that the numerical models accurately reproduce the phototransistors experimental response, we demonstrate that the proposed architecture is suitable for the development of a new class of compact and scalable SPR sensors.