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1.
Stud Hist Philos Sci ; 93: 163-174, 2022 06.
Article in English | MEDLINE | ID: mdl-35468532

ABSTRACT

The debate around analogy in modern physics that focuses on its role as a logical inference often correspondingly overlooks its historical dimension and the other equally important functions and aspects that are intertwined with this dimension. Inspired by a close investigation of the primary sources and archival material of a few historical actors, this paper lays out a framework on analogy-making which preserves as much as possible its historical complexity. While not losing sight of the logical role, our framework puts a special emphasis on the heuristic process, and aims at offering to the historian and philosopher of science as well as the physicist some tools to capture the subtle functions of analogical reasoning involved in such a process. After having traced it out theoretically, we make use of this framework to interpret the growth of the ideas of two remarkable physicists dealing with the multifaceted notion of vacuum in 20th century physics. We first consider the trajectory followed by John A. Wheeler, between the 1960s and 1970s, towards (in his own words) a "geology of the vacuum"; and then examine, starting from the hitherto neglected Japanese reception of the idea of Dirac sea in the early 1930s, the pathway that led Yoichiro Nambu to the discovery of spontaneous symmetry breaking.


Subject(s)
Geology , Logic , Physics , Problem Solving , Vacuum
3.
Eur Phys J Plus ; 135(8): 627, 2020.
Article in English | MEDLINE | ID: mdl-32832318

ABSTRACT

SrIrO 3 , the three-dimensional member of the Ruddlesden-Popper iridates, is a paramagnetic semimetal characterised by a the delicate interplay between spin-orbit coupling and Coulomb repulsion. In this work, we study the anisotropic magnetoresistance (AMR) of SrIrO 3 thin films, which is closely linked to spin-orbit coupling and probes correlations between electronic transport, magnetic order and orbital states. We show that the low-temperature negative magnetoresistance is anisotropic with respect to the magnetic field orientation, and its angular dependence reveals the appearance of a fourfold symmetric component above a critical magnetic field. We show that this AMR component is of magnetocrystalline origin, and attribute the observed transition to a field-induced magnetic state in SrIrO 3 .

4.
Entropy (Basel) ; 21(8)2019 Jul 29.
Article in English | MEDLINE | ID: mdl-33267456

ABSTRACT

Since its inception, the concept of entropy has been known under a variety of guises and been used in an increasing number of contexts, achieving an almost rock star-like status in both the sciences and popular culture. The three most prominent "styles" which entropy has been (re)told in and which have determined its popularity are the thermodynamic, statistical and information-theoretic one, owing much to the work of Clausius, Boltzmann and Gibbs, and Shannon, respectively. In the relentless hunt for the core of the concept that spurred this development, connections with irreversibility and emergence of time, nature of probability and information emerged adding to its elusiveness as much as stimulating its proliferation and cross-contextual adoption. In this historical review, we retrace, through primary and secondary sources, the three main perspectives from which entropy has been regarded, emphasising the motivations behind each new version, their ramifications and the bridges that have been constructed to justify them. From this analysis of the foundations a number of characteristic traits of the concept emerge that underline its exceptionality as an engine of conceptual progress.

5.
ACS Nano ; 11(6): 5879-5883, 2017 06 27.
Article in English | MEDLINE | ID: mdl-28494146

ABSTRACT

Embedding a magnetic electroactive molecule in a three-terminal junction allows for the fast and local electric field control of magnetic properties desirable in spintronic devices and quantum gates. Here, we provide an example of this control through the reversible and stable charging of a single all-organic neutral diradical molecule. By means of inelastic electron tunnel spectroscopy we show that the added electron occupies a molecular orbital distinct from those containing the two radical electrons, forming a spin system with three antiferromagnetically coupled spins. Changing the redox state of the molecule therefore switches on and off a parallel exchange path between the two radical spins through the added electron. This electrically controlled gating of the intramolecular magnetic interactions constitutes an essential ingredient of a single-molecule [Formula: see text] quantum gate.

6.
Phys Rev Lett ; 118(11): 117001, 2017 Mar 17.
Article in English | MEDLINE | ID: mdl-28368652

ABSTRACT

Superconductors containing magnetic impurities exhibit intriguing phenomena derived from the competition between Cooper pairing and Kondo screening. At the heart of this competition are the Yu-Shiba-Rusinov (Shiba) states which arise from the pair breaking effects a magnetic impurity has on a superconducting host. Hybrid superconductor-molecular junctions offer unique access to these states but the added complexity in fabricating such devices has kept their exploration to a minimum. Here, we report on the successful integration of a model spin 1/2 impurity, in the form of a neutral and stable all organic radical molecule, in proximity-induced superconducting break junctions. Our measurements reveal excitations which are characteristic of a spin-induced Shiba state due to the radical's unpaired spin strongly coupled to a superconductor. By virtue of a variable molecule-electrode coupling, we access both the singlet and doublet ground states of the hybrid system which give rise to the doublet and singlet Shiba excited states, respectively. Our results show that Shiba states are a robust feature of the interaction between a paramagnetic impurity and a proximity-induced superconductor where the excited state is mediated by correlated electron-hole (Andreev) pairs instead of Cooper pairs.

7.
Nano Lett ; 15(5): 3109-14, 2015 May 13.
Article in English | MEDLINE | ID: mdl-25897770

ABSTRACT

Organic radicals are neutral, purely organic molecules exhibiting an intrinsic magnetic moment due to the presence of an unpaired electron in the molecule in its ground state. This property, added to the low spin-orbit coupling and weak hyperfine interactions, make neutral organic radicals good candidates for molecular spintronics insofar as the radical character is stable in solid state electronic devices. Here we show that the paramagnetism of the polychlorotriphenylmethyl radical molecule in the form of a Kondo anomaly is preserved in two- and three-terminal solid-state devices, regardless of mechanical and electrostatic changes. Indeed, our results demonstrate that the Kondo anomaly is robust under electrodes displacement and changes of the electrostatic environment, pointing to a localized orbital in the radical as the source of magnetism. Strong support to this picture is provided by density functional calculations and measurements of the corresponding nonradical species. These results pave the way toward the use of all-organic neutral radical molecules in spintronics devices and open the door to further investigations into Kondo physics.

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