Characterizing laser-plasma ion accelerators driving an intense neutron beam via nuclear signatures.

Compact, bright neutron sources are opening up several emerging applications including detection of nuclear materials for national security applications. At Los Alamos National Laboratory, we have used a short-pulse laser to accelerate deuterons in the relativistic transparency regime. These deuterons impinge on a beryllium converter to generate neutrons. During the initial experiments where these neutrons were used for active interrogation of uranium and plutonium, we observed ß-delayed neutron production from decay of 9Li, formed by the high-energy deuteron bombardment of the beryllium converter. Analysis of the delayed neutrons provides novel evidence of the divergence of the highest energy portion of the deuterons (i.e., above 10 MeV/nucleon) from the laser axis, a documented feature of the breakout afterburner laser-plasma ion acceleration mechanism. These delayed neutrons form the basis of non-intrusive diagnostics for determining the features of deuteron acceleration as well as monitoring neutron production for the next generation of laser-driven neutron sources.

Anomalous material-dependent transport of focused, laser-driven proton beams.

Intense lasers can accelerate protons in sufficient numbers and energy that the resulting beam can heat materials to exotic warm (10 s of eV temperature) states. Here we show with experimental data that a laser-driven proton beam focused onto a target heated it in a localized spot with size strongly dependent upon material and as small as 35 µm radius. Simulations indicate that cold stopping power values cannot model the intense proton beam transport in solid targets well enough to match the large differences observed. In the experiment a 74 J, 670 fs laser drove a focusing proton beam that transported through different thicknesses of solid Mylar, Al, Cu or Au, eventually heating a rear, thin, Au witness layer. The XUV emission seen from the rear of the Au indicated a clear dependence of proton beam transport upon atomic number, Z, of the transport layer: a larger and brighter emission spot was measured after proton transport through the lower Z foils even with equal mass density for supposed equivalent proton stopping range. Beam transport dynamics pertaining to the observed heated spot were investigated numerically with a particle-in-cell (PIC) code. In simulations protons moving through an Al transport layer result in higher Au temperature responsible for higher Au radiant emittance compared to a Cu transport case. The inferred finding that proton stopping varies with temperature in different materials, considerably changing the beam heating profile, can guide applications seeking to controllably heat targets with intense proton beams.

Visualization of expanding warm dense gold and diamond heated rapidly by laser-generated ion beams.

With the development of several novel heating sources, scientists can now heat a small sample isochorically above 10,000 K. Although matter at such an extreme state, known as warm dense matter, is commonly found in astrophysics (e.g., in planetary cores) as well as in high energy density physics experiments, its properties are not well understood and are difficult to predict theoretically. This is because the approximations made to describe condensed matter or high-temperature plasmas are invalid in this intermediate regime. A sufficiently large warm dense matter sample that is uniformly heated would be ideal for these studies, but has been unavailable to date. Here we have used a beam of quasi-monoenergetic aluminum ions to heat gold and diamond foils uniformly and isochorically. For the first time, we visualized directly the expanding warm dense gold and diamond with an optical streak camera. Furthermore, we present a new technique to determine the initial temperature of these heated samples from the measured expansion speeds of gold and diamond into vacuum. We anticipate the uniformly heated solid density target will allow for direct quantitative measurements of equation-of-state, conductivity, opacity, and stopping power of warm dense matter, benefiting plasma physics, astrophysics, and nuclear physics.

On the analysis of inhomogeneous magnetic field spectrometer for laser-driven ion acceleration.

We present a detailed study of the use of a non-parallel, inhomogeneous magnetic field spectrometer for the investigation of laser-accelerated ion beams. Employing a wedged yoke design, we demonstrate the feasibility of an in-situ self-calibration technique of the non-uniform magnetic field and show that high-precision measurements of ion energies are possible in a wide-angle configuration. We also discuss the implications of a stacked detector system for unambiguous identification of different ion species present in the ion beam and explore the feasibility of detection of high energy particles beyond 100 MeV/amu in radiation harsh environments.

Monoenergetic ion beam generation by driving ion solitary waves with circularly polarized laser light.

Experimental data from the Trident Laser facility is presented showing quasimonoenergetic carbon ions from nm-scaled foil targets with an energy spread of as low as ±15% at 35 MeV. These results and high-resolution kinetic simulations show laser acceleration of quasimonoenergetic ion beams by the generation of ion solitons with circularly polarized laser pulses (500 fs, λ=1054 nm). The conversion efficiency into monoenergetic ions is increased by an order of magnitude compared with previous experimental results, representing an important step towards applications such as ion fast ignition.

A novel high resolution ion wide angle spectrometer.

A novel ion wide angle spectrometer (iWASP) has been developed, which is capable of measuring angularly resolved energy distributions of protons and a second ion species, such as carbon C(6 +), simultaneously. The energy resolution for protons and carbon ions is better than 10% at ∼50 MeV/nucleon and thus suitable for the study of novel laser-ion acceleration schemes aiming for ultrahigh particle energies. A wedged magnet design enables an acceptance angle of 30°(∼524 mrad) and high angular accuracy in the µrad range. First, results obtained at the LANL Trident laser facility are presented demonstrating high energy and angular resolution of this novel iWASP.

Development of a high resolution and high dispersion Thomson parabola.

Here, we report on the development of a novel high resolution and high dispersion Thomson parabola for simultaneously resolving protons and low-Z ions of more than 100 MeV/nucleon necessary to explore novel laser ion acceleration schemes. High electric and magnetic fields enable energy resolutions of ΔE∕E < 5% at 100 MeV/nucleon and impede premature merging of different ion species at low energies on the detector plane. First results from laser driven ion acceleration experiments performed at the Trident Laser Facility demonstrate high resolution and superior species and charge state separation of this novel Thomson parabola for ion energies of more than 30 MeV/nucleon.

Pulse shape measurements using single shot-frequency resolved optical gating for high energy (80 J) short pulse (600 fs) laser.

Relevant to laser based electron/ion accelerations, a single shot second harmonic generation frequency resolved optical gating (FROG) system has been developed to characterize laser pulses (80 J, ∼600 fs) incident on and transmitted through nanofoil targets, employing relay imaging, spatial filter, and partially coated glass substrates to reduce spatial nonuniformity and B-integral. The device can be completely aligned without using a pulsed laser source. Variations of incident pulse shape were measured from durations of 613 fs (nearly symmetric shape) to 571 fs (asymmetric shape with pre- or postpulse). The FROG measurements are consistent with independent spectral and autocorrelation measurements.

Phase-contrast imaging using ultrafast x-rays in laser-shocked materials.

High-energy x-rays, >10 keV, can be efficiently produced from ultrafast laser target interactions with many applications to dense target materials in inertial confinement fusion and high-energy density physics. These same x-rays can also be applied to measurements of low-density materials inside high-density Hohlraum environments. In the experiments presented, high-energy x-ray images of laser-shocked polystyrene are produced through phase contrast imaging. The plastic targets are nominally transparent to traditional x-ray absorption but show detailed features in regions of high density gradients due to refractive effects often called phase contrast imaging. The 200 TW Trident laser is used both to produce the x-ray source and to shock the polystyrene target. X-rays at 17 keV produced from 2 ps, 100 J laser interactions with a 12 µm molybdenum wire are used to produce a small source size, required for optimizing refractive effects. Shocks are driven in the 1 mm thick polystyrene target using 2 ns, 250 J, 532 nm laser drive with phase plates. X-ray images of shocks compare well to one-dimensional hydro calculations.

Enhanced laser-driven ion acceleration in the relativistic transparency regime.

We report on the acceleration of ion beams from ultrathin diamondlike carbon foils of thickness 50, 30, and 10 nm irradiated by ultrahigh contrast laser pulses at intensities of approximately 7 x 10;{19} W/cm;{2}. An unprecedented maximum energy of 185 MeV (15 MeV/u) for fully ionized carbon atoms is observed at the optimum thickness of 30 nm. The enhanced acceleration is attributed to self-induced transparency, leading to strong volumetric heating of the classically overdense electron population in the bulk of the target. Our experimental results are supported by both particle-in-cell (PIC) simulations and an analytical model.

Radiochromic film imaging spectroscopy of laser-accelerated proton beams.

This article reports on an experimental method to fully reconstruct laser-accelerated proton beam parameters called radiochromic film imaging spectroscopy (RIS). RIS allows for the characterization of proton beams concerning real and virtual source size, envelope- and microdivergence, normalized transverse emittance, phase space, and proton spectrum. This technique requires particular targets and a high resolution proton detector. Therefore thin gold foils with a microgrooved rear side were manufactured and characterized. Calibrated GafChromic radiochromic film (RCF) types MD-55, HS, and HD-810 in stack configuration were used as spatial and energy resolved film detectors. The principle of the RCF imaging spectroscopy was demonstrated at four different laser systems. This can be a method to characterize a laser system with respect to its proton-acceleration capability. In addition, an algorithm to calculate the spatial and energy resolved proton distribution has been developed and tested to get a better idea of laser-accelerated proton beams and their energy deposition with respect to further applications.

Development and calibration of a Thomson parabola with microchannel plate for the detection of laser-accelerated MeV ions.

This article reports on the development and application of a Thomson parabola (TP) equipped with a (90x70) mm(2) microchannel-plate (MCP) for the analysis of laser-accelerated ions, produced by a high-energy, high-intensity laser system. The MCP allows an online measurement of the produced ions in every single laser shot. An electromagnet instead of permanent magnets is used that allows the tuning of the magnetic field to adapt the field strength to the analyzed ion species and energy. We describe recent experiments at the 100 TW laser facility at the Laboratoire d'Utilization des Lasers Intenses (LULI) in Palaiseau, France, where we have observed multiple ion species and charge states with ions accelerated up to 5 MeV/u (O(+6)), emitted from the rear surface of a laser-irradiated 50 microm Au foil. Within the experiment the TP was calibrated for protons and for the first time conversion efficiencies of MeV protons (2-13 MeV) to primary electrons (electrons immediately generated by an ion impact onto a surface) in the MCP are presented.

Scaling laws for energetic ions from the commissioning of the new Los Alamos National Laboratory 200 TW Trident laser.

The recent Los Alamos National Laboratory Trident laser enhanced from 30 to 200 TW in power allows more than 100 J to be delivered on target in 500 fs with a spot size smaller than 12 microm at full width at half maximum. 15 microm flat-foil targets have been observed to produce proton beams in excess of 50 MeV at an intensity of only approximately 4x10(19) W/cm(2) with efficiencies approaching 5%. The Trident laser beam characteristics are presented along with the data compared to published scaling laws for proton acceleration.

A simple apparatus for quick qualitative analysis of CR39 nuclear track detectors.

Quantifying the ion pits in Columbia Resin 39 (CR39) nuclear track detector from Thomson parabolas is a time consuming and tedious process using conventional microscope based techniques. A simple inventive apparatus for fast screening and qualitative analysis of CR39 detectors has been developed, enabling efficient selection of data for a more detailed analysis. The system consists simply of a green He-Ne laser and a high-resolution digital single-lens reflex camera. The laser illuminates the edge of the CR39 at grazing incidence and couples into the plastic, acting as a light pipe. Subsequently, the laser illuminates all ion tracks on the surface. A high-resolution digital camera is used to photograph the scattered light from the ion tracks, enabling one to quickly determine charge states and energies measured by the Thomson parabola.

High-energy, high-resolution x-ray imaging on the Trident short-pulse laser facility.

With the completion of the Trident laser facility upgrade, 200 TW high-energy laser pulses are now capable of producing x-ray pulses with energies in the range of 15-40 keV, which will be used for high-spatial resolution radiography. A diagnostic suite is being developed on the laser system to investigate and characterize the x-ray emission from high-Z targets. This includes charge coupled device based single-photon counters, imaging plates, a high-energy electronic imager, spectral diagnostics, and optical and x-ray spot size diagnostics. We describe recent x-ray results from a commissioning campaign as well as describe the development and design of a high-energy spectrometer. X-ray radiographs taken at 22 keV with a spatial resolution of 25 mum are a first demonstration on this facility of high-energy, high-spatial resolution capability.

TRIDENT high-energy-density facility experimental capabilities and diagnostics.

The newly upgraded TRIDENT high-energy-density (HED) facility provides high-energy short-pulse laser-matter interactions with powers in excess of 200 TW and energies greater than 120 J. In addition, TRIDENT retains two long-pulse (nanoseconds to microseconds) beams that are available for simultaneous use in either the same experiment or a separate one. The facility's flexibility is enhanced by the presence of two separate target chambers with a third undergoing commissioning. This capability allows the experimental configuration to be optimized by choosing the chamber with the most advantageous geometry and features. The TRIDENT facility also provides a wide range of standard instruments including optical, x-ray, and particle diagnostics. In addition, one chamber has a 10 in. manipulator allowing OMEGA and National Ignition Facility (NIF) diagnostics to be prototyped and calibrated.

A novel backscatter focus diagnostic for the TRIDENT 200 TW laser.

Here we present the first direct focal spot images and analysis of an ultrahigh intensity short-pulse laser focus (>5x10(19) W/cm(2)) on target. Such a focal spot characterization is typically done previous to the shot with a low-power alignment beam using equivalent plane imaging techniques. The resulting intensity of the shot is then inferred from these results. We report on the development of a backscatter focus diagnostic, which enables imaging of the on-target full-power focal spot.

Controlled transport and focusing of laser-accelerated protons with miniature magnetic devices.

This Letter demonstrates the transporting and focusing of laser-accelerated 14 MeV protons by permanent magnet miniature quadrupole lenses providing field gradients of up to 500 T/m. The approach is highly reproducible and predictable, leading to a focal spot of (286 x 173) microm full width at half maximum 50 cm behind the source. It decouples the relativistic laser-proton acceleration from the beam transport, paving the way to optimize both separately. The collimation and the subsequent energy selection obtained are perfectly applicable for upcoming high-energy, high-repetition rate laser systems.