Analogue cosmological particle creation in an ultracold quantum fluid of light.

The rapid expansion of the early universe resulted in the spontaneous production of cosmological particles from vacuum fluctuations, some of which are observable today in the cosmic microwave background anisotropy. The analogue of cosmological particle creation in a quantum fluid was proposed, but the quantum, spontaneous effect due to vacuum fluctuations has not yet been observed. Here we report the spontaneous creation of analogue cosmological particles in the laboratory, using a quenched 3-dimensional quantum fluid of light. We observe acoustic peaks in the density power spectrum, in close quantitative agreement with the quantum-field theoretical prediction. We find that the long-wavelength particles provide a window to early times. This work introduces the quantum fluid of light, as cold as an atomic Bose-Einstein condensate.

Dissipative Phase Transition with Driving-Controlled Spatial Dimension and Diffusive Boundary Conditions.

We investigate theoretically and experimentally a first-order dissipative phase transition, with diffusive boundary conditions and the ability to tune the spatial dimension of the system. The considered physical system is a planar semiconductor microcavity in the strong light-matter coupling regime, where polariton excitations are injected by a quasiresonant optical driving field. The spatial dimension of the system from 1D to 2D is tuned by designing the intensity profile of the driving field. We investigate the emergence of criticality by increasing the spatial size of the driven region. The system is nonlinear due to polariton-polariton interactions and the boundary conditions are diffusive because the polaritons can freely diffuse out of the driven region. We show that no phase transition occurs using a 1D driving geometry, while for a 2D geometry we do observe both in theory and experiments the emergence of a first-order phase transition. The demonstrated technique allows all-optical and in situ control of the system geometry, providing a versatile platform for exploring the many-body physics of photons.

Measurement of the Static Structure Factor in a Paraxial Fluid of Light Using Bragg-like Spectroscopy.

We implement Bragg-like spectroscopy in a paraxial fluid of light by imprinting analogues of short Bragg pulses on the photon fluid using wavefront shaping with a spatial light modulator. We report a measurement of the static structure factor, S(k), and we find a quantitative agreement with the prediction of the Feynman relation revealing indirectly the presence of pair-correlated particles in the fluid. Finally, we improve the resolution over previous methods and obtain the dispersion relation including a linear phononic regime for weakly interacting photons and low sound velocity.

Single Photons Emitted by Nanocrystals Optically Trapped in a Deep Parabolic Mirror.

We investigate the emission of single photons from CdSe/CdS dots-in-rod which are optically trapped in the focus of a deep parabolic mirror. Thanks to this mirror, we are able to image almost the full 4π emission pattern of nanometer-sized elementary dipoles and verify the alignment of the rods within the optical trap. From the motional dynamics of the emitters in the trap, we infer that the single-photon emission occurs from clusters comprising several emitters. We demonstrate the optical trapping of rod-shaped quantum emitters in a configuration suitable for efficiently coupling an ensemble of linear dipoles with the electromagnetic field in free space.

Attenuation-free non-diffracting Bessel beams.

We report on a versatile method to compensate the linear attenuation in a medium, independently of its microscopic origin. The method exploits diffraction-limited Bessel beams and tailored on-axis intensity profiles, which are generated using a phase-only spatial light modulator. This technique for compensating one of the most fundamental limiting processes in linear optics is shown to be efficient for a wide range of experimental conditions (modifying the refractive index and the attenuation coefficient). Finally, we explain how this method can be advantageously exploited in applications ranging from bio-imaging light sheet microscopy to quantum memories for future quantum communication networks.

Exciton Fine Structure of CdSe/CdS Nanocrystals Determined by Polarization Microscopy at Room Temperature.

We present a method that allows determining the band-edge exciton fine structure of CdSe/CdS dot-in-rods samples based on single particle polarization measurements at room temperature. We model the measured emission polarization of such single particles considering the fine structure properties, the dielectric effect induced by the anisotropic shell, and the measurement configuration. We use this method to characterize the band-edge exciton fine structure splitting of various samples of dot-in-rods. We show that, when the diameter of the CdSe core increases, a transition from a spherical like band-edge exciton symmetry to a rod-like band edge exciton symmetry occurs. This explains the often reported large emission polarization of such particles compared to spherical CdSe/CdS emitters.

Two-photon injection of polaritons in semiconductor microstructures.

We experimentally demonstrate that two-photon pumping of "dark" excitons in quantum wells embedded in semiconductor microcavities can result in exciton-polariton injection and photon lasing. In the case of a semiconductor micropillar pumped at half of the exciton frequency, we observe a clear threshold behavior, characteristic of the vertical cavity surface emitting laser transition. These results are interpreted in terms of stimulated emission of terahertz photons, which allows for conversion of "dark" excitons into exciton-polaritons.

Non-blinking single-photon generation with anisotropic colloidal nanocrystals: towards room-temperature, efficient, colloidal quantum sources.

Blinking and single-photon emission can be tailored in CdSe/CdS core/shell colloidal dot-in-rods. By increasing the shell thickness it is possible to obtain almost non-blinking nanocrystals, while the shell length can be used to control single-photon emission probability.

Vacuum squeezed light for atomic memories at the D2 cesium line.

We report the experimental generation of squeezed light at 852 nm, locked on the Cesium D(2) line. 50% of noise reduction down to 50 kHz has been obtained with a doubly resonant optical parametric oscillator operating below threshold, using a periodically-poled KTP crystal. This light is directly utilizable with Cesium atomic ensembles for quantum networking applications.

Optimal intensity noise reduction in multimode vertical-cavity surface-emitting lasers by polarization-selective attenuation.

We study in detail the effect of the anticorrelation of the polarization modes on the total intensity noise of a vertical-cavity surface-emitting laser. We show that small polarization-dependent losses can greatly improve the total intensity noise, and we determine and experimentally demonstrate the conditions necessary for optimal intensity noise reduction.