Measurement of radon concentration in soil gas and radon exhalation rate from soil samples along and across the Main Central Thrust of Garhwal Himalaya, India.

The present study focuses on measuring radon concentrations in soil gas at various depths, radon exhalation rate (surface and mass) from soil samples, and gamma dose rate along and across the Main Central Thrust of Garhwal Himalaya, India. Radon concentration in soil gas, surface, and mass exhalation rates was measured using a portable SMART radon monitor (RnDuo). Furthermore, the gamma dose rate was measured using a pocket radiation monitor. The soil gas radon concentration varied from 15 ± 4 to 579 ± 82 Bq m-3 at a depth of 25 cm, 10 ± 2 to 533 ± 75 Bq m-3 at a depth of 30 cm, and 9 ± 1 to 680 ± 95 Bq m-3 at a depth of 35 cm. The surface and mass exhalation rates were found 3 ± 0.7 to 98 ± 3 Bq m-2 h-1 (with AM ± SD = 36 ± 28 Bq m-2 h-1) and 1 ± 0.2 to 95 ± 2 mBq kg-1 h-1 (with AM ± SD = 30 ± 22 mBq kg-1 h-1), respectively. The gamma dose rate for the present study area varies from 0.11 ± 0.05 to 0.28 ± 0.05 µSv h-1 with a mean value of 0.17 ± 0.05 µSv h-1. The correlation analysis between the exhalation rates (mass and surface) and radon concentration of soil gas at various depths was carried out in the current study.

A COMPARATIVE STUDY OF RADIUM CONTENT AND RADON EXHALATION RATE FROM SOIL SAMPLES USING ACTIVE AND PASSIVE TECHNIQUES.

Soil is the most important factor affecting the radon level in the human living environments. It depends not only on uranium and thorium contents but also on the physical and chemical properties of the soil. In this paper, the measurements of radium content and mass exhalation rate of radon from the soil samples collected from Uttarkashi area of Garhwal Himalaya are presented. The correlation between radium content and radon mass exhalation rate from soil has also been obtained. The radium was measured by gamma ray spectrometry, while the mass exhalation rate of radon has been determined by both active and passive methods. The radium activity in the soil of study area was found to vary from 45±7 to 285±29 Bq kg-1 with an average of 99 Bq kg-1 The radon mass exhalation rate was found to vary from 0.59 × 10-5 to 2.2 × 10-5 Bq kg-1 h-1 with an average of 1.4 × 10-5 Bq kg-1 h-1 by passive technique and from 0.8 × 10-5 to 3.2 × 10-5 Bq kg-1 h-1 with an average of 1.5 × 10-5 Bq kg-1 h-1 by active technique. The results suggest that the measured radium value is positively correlated with the radon mass exhalation rate measured with both the active and passive techniques.

MEASUREMENT OF RADON, THORON AND THEIR PROGENY IN DIFFERENT TYPES OF DWELLING IN ALMORA DISTRICT OF KUMAUN HIMALAYAN REGION.

The indoor concentrations of radon (222Rn), thoron (220Rn) and their daughter products were measured in the dwellings of Almora district in Kumaun Himalaya, India using pin-hole dosemeters and deposition progeny sensors. The measurements were made in the residential houses built of mud, stone with cement plaster and cemented house during winter season. Average [geometric mean (GM) values] radon and thoron concentrations for all dwellings were found to be 99.82 and 79.70 Bq m-3, respectively, while average equilibrium equivalent radon concentration and equilibrium equivalent thoron concentration (measured for the first time for this region) were measured at 35.22 and 2.52 Bq m-3, respectively. Radon concentration (GM values) was found to be 110.73, 97.00 and 93.85 Bq m-3 for mud houses, stone with cemented plaster houses and cemented houses, respectively. On the other hand, thoron concentration values were 87.10, 75.79 and 75.68 Bq m-3 for cemented houses, mud houses and stone with cemented plaster houses, respectively. Interpretations have been made on the basis of measured radon/thoron and progeny concentration values with respect to the difference of construction material of the dwellings.

NATURAL RADIOACTIVITY LEVEL AND ELEMENTAL COMPOSITION OF SOIL SAMPLES FROM A HIGH BACKGROUND RADIATION AREA ON EASTERN COAST OF INDIA (ODISHA).

A comprehensive study was carried out to determine the radioactivity concentration of soil samples from different sites of a high background radiation area in the eastern coast of India, Odisha state. The dose rate measured in situ varied from 0.25 to 1.2 µSv h-1 The gamma spectrometry measurements indicated Th series elements as the main contributors to the enhanced level of radiation and allowed the authors to find the mean level of the activity concentration (±SD) for 226Ra, 228Th and 40K as 130±97, 1110±890 and 360±140 Bq kg-1, respectively. Human exposure from radionuclides occurring outdoor was estimated based on the effective dose rate, which ranged from 0.14±0.02 to 2.15±0.26 mSv and was higher than the UNSCEAR annual worldwide average value 0.07 mSv. Additionally, X-ray fluorescence analysis provided information about the content of major elements in samples and indicated the significant amount of Ti (7.4±4.9 %) in soils.

Variability of radon and thoron equilibrium factors in indoor environment of Garhwal Himalaya.

The measurements of radon, thoron and their progeny concentrations have been carried out in the dwellings of Uttarkashi and Tehri districts of Garhwal Himalaya, India using LR-115 detector based pin-hole dosimeter and DRPS/DTPS techniques. The equilibrium factors for radon, thoron and their progeny were calculated by using the values measured with these techniques. The average values of equilibrium factor between radon and its progeny have been found to be 0.44, 0.39, 0.39 and 0.28 for rainy, autumn, winter and summer seasons, respectively. For thoron and its progeny, the average values of equilibrium factor have been found to be 0.04, 0.04, 0.04 and 0.03 for rainy, autumn, winter and summer seasons, respectively. The equilibrium factor between radon and its progeny has been found to be dependent on the seasonal changes. However, the equilibrium factor for thoron and progeny has been found to be same for rainy, autumn and winter seasons but slightly different for summer season. The annual average equilibrium factors for radon and thoron have been found to vary from 0.23 to 0.80 with an average of 0.42 and from 0.01 to 0.29 with an average of 0.07, respectively. The detailed discussion of the measurement techniques and the explanation for the results obtained is given in the paper.

Analysis of natural radionuclides in soil samples of Purola area of Garhwal Himalaya, India.

Naturally occurring radioactive materials are widely spread in the earth's environment, being distributed in soil, rocks, water, air, plants and even within the human body. All of these sources have contributed to an increase in the levels of environmental radioactivity and population radiation doses. This paper presents the activity level due to the presence of (226)Ra, (232)Th and (40)K in soil samples of Purola area in Garhwal Himalaya region. The measured activity of (226)Ra, (232)Th and (40)K in collected soil samples of Purola was found to vary from 13±10 to 55±10 Bq kg(-1) with an average of 31±2 Bq kg(-1), 13±10 to 101±13 Bq kg(-1) with an average 30±3 Bq kg(-1) and 150±81 to 1310±154 Bq kg(-1) with an average 583±30 Bq kg(-1), respectively. The radium equivalent activity in collected soil samples was found to vary from 47 to 221 Bq kg(-1) with an average of 115 Bq kg(-1). The total absorbed gamma dose rate in this area was found to vary from 22 to 93 nGy h(-1) with an average of 55 nGy h(-1). The distribution of these radionuclides in the soil of study area is discussed in details.

Comparative study of various techniques for environmental radon, thoron and progeny measurements.

Long-term average concentrations of radon, thoron and progeny were measured in normal and high background radiation areas in India using different techniques. Radon, thoron and progeny concentrations were measured using Raduet, Pin-Hole dosimeter, deposition-based CR-39 and deposition-based direct radon/thoron progeny sensor (DRPS/DTPS) detector system. All these techniques were used at a same time inside an individual dwelling. Radon concentration was recorded higher than thoron concentration in Garhwal Homes (NBRA) while thoron concentration was found relatively higher in the houses of Chhatarpur area (HBRA) in Odisha, India. The values measured with the CR-39 detector-based technique were found comparable with the values measured with the LR-115 detector-based technique. The comparisons of results using various techniques and their usefulness in radiation measurements are discussed in detail.

Measurements of radon and thoron progeny concentrations in dwellings of Tehri Garhwal, India, using LR-115 deposition-based DTPS/DRPS technique.

This paper presents the values of radon and thoron progeny concentrations for different seasons in the dwellings of Tehri Garhwal, India. The measurements have been carried out using LR-115 solid-state nuclear track detector-based passive time-integrated direct thoron progeny sensor/direct radon progeny sensor technique. In summer, the radon and thoron progeny have been found to vary from 5.7±0.8 to 153.2±4.3 Bq m(-3) with an average of 37.6 Bq m(-3) and 0.3±0.06 to 3.2±0.19 Bq m(-3) with an average of 1.3 Bq m(-3), respectively. In the rainy season, the radon and thoron progeny have been found to vary from 3.2±0.6 to 120±3.7 Bq m(-3) with an average of 58.2 Bq m(-3) and 0.2±0.05 to 11.3±0.37 Bq m(-3) with an average of 3.4 Bq m(-3), respectively. In autumn, the radon and thoron progeny have been found to vary from 4.1±0.7 to 374.4±6.7 Bq m(-3) with an average of 95.6 Bq m(-3) and from 0.3±0.06 to 30.5±0.60 Bq m(-3) with an average of 6.6 Bq m(-3), respectively. In winter, the radon and thoron progeny have been found to vary from 9.8±1.1 to 188.9±4.8 Bq m(-3) with an average of 70.7 Bq m(-3) and 0.1±0.03 to 7.5±0.30 Bq m(-3) with an average of 2.3 Bq m(-3), respectively. It has been observed that the average value of radon and thoron progeny concentrations is maximum for autumn and minimum for summer seasons. The seasonal variations in radon and thoron progeny concentrations in different houses are discussed in detail.

Estimation of past radon exposure to indoor radon from embedded (210)Po in household glass.

In the present investigation, the surface-deposited polonium activities were measured in houses in the Ukhimath region of Garhwal Himalaya, India. The surface-deposited (210)Po activity concentrations were found to vary from 0.7 to 15.40 Bq m(-2) with an average of 5.95 Bq m(-2). The radon concentration estimated on the basis of (210)Po activity was found to vary from 0.29 to 700 Bq m(-3) with an average value 242 Bq m(-3). The contemporary radon concentration in the area was found to vary from 13 to 181 Bq m(-3) with an average of 46 Bq m(-3). The annual effective dose due to (210)Po activity in houses in the Garhwal Himalaya region was found to vary from 0.61 to 13.33 mSv with an average of 5.15 mSv. Some worldwide studies have shown the relation between the increased risk of lung cancer and smoking habits. Data on smoking have also been collected from the same dwellings. The significance of this work is also discussed in detail from a radiation protection point of view.

Distribution of terrestrial gamma radiation dose rate in the eastern coastal area of Odisha, India.

Terrestrial gamma radiation is one of the important radiation exposures on the earth's surface that results from the three primordial radionuclides (226)Ra, (232)Th and (40)K. The elemental concentration of these elements in the earth's crust could result in the anomalous variation of the terrestrial gamma radiation in the environment. The geology of the local area plays an important role in distribution of these radioactive elements. Environmental terrestrial gamma radiation dose rates were measured around the eastern coastal area of Odisha with the objective of establishing baseline data on the background radiation level. The values of the terrestrial gamma radiation dose rate vary significantly at different locations in the study area. The values of the terrestrial gamma dose rate ranged from 77 to 1651 nGy h(-1), with an average of 230 nGy h(-1). During the measurement of the terrestrial gamma dose rate, sand and soil samples were also collected for the assessment of natural radionuclides. The activities of (226)Ra, (232)Th and (40)K from these samples were measured using a gamma-ray spectrometry with a NaI(Tl) detector. Activity concentrations of (226)Ra, (232)Th and (40)K ranged from 15.6 to 69 Bq kg(-1) with an average of 46.7 Bq kg(-1), from 28.9 to 973 Bq kg(-1) with an average of 250 Bq kg(-1) and from 139 to 952 Bq kg(-1) with an average of 429, respectively. The detailed significance of these studies has been discussed from the radiation protection point of view.

Variations in radon concentration in groundwater of Kumaon Himalaya, India.

The radon content in groundwater sources depends on the radium concentration in the rock of the aquifer. Radon was measured in water in many parts of the world, mostly for the risk assessment due to consumption of drinking water. The exposure to radon through drinking water is largely by inhalation and ingestion. Airborne radon can be released during normal household activities and can pose a greater potential health risk than radon ingested with water. Transport of radon through soil and bedrock by water depends mainly on the percolation of water through the pores and along fracture planes of bedrock. In this study, the radon concentration in water from springs and hand pumps of Kumaun Himalaya, India was measured using the radon emanometry technique. Radon concentration was found to vary from 1 to 392 Bq l(-1) with a mean of 50 Bq l(-1) in groundwater in different lithotectonic units. The radon level was found to be higher in the area consisting of granite, quartz porphyry, schist, phyllites and lowest in the area having sedimentary rocks, predominantly dominated by quartzite rocks.

Levels of thoron and progeny in high background radiation area of southeastern coast of Odisha, India.

Exposure to radon, (222)Rn, is assumed to be the most significant source of natural radiation to human beings in most cases. It is thought that radon and its progeny are major factors that cause cancer. The presence of thoron, (220)Rn, was often neglected because it was considered that the quantity of thoron in the environment is less than that of radon. However, recent studies have shown that a high thoron concentration was found in some regions and the exposure to (220)Rn and its progeny can equal or several time exceed that of (220)Rn and its progeny. The results of thoron and its progeny measurements in the houses of high background radiation area (HBRA) of the southeastern coast of Odisha, India presented here. This area is one of the high background radiation areas in India with a large deposit of monazite sand which is the probable source of thoron. Both active and passive methods were employed for the measurement of thoron and its progeny in cement, brick and mud houses in the study area. Thoron concentration was measured using RAD-7 and Raduet. A CR-39 track detector was employed for the measurement of environmental thoron progeny, both in active and passive modes. Thoron and its progeny concentrations were found to be comparatively high in the area. A comparison between the results obtained with various techniques is presented in this paper.

Study of natural radionuclide and absorbed gamma dose in Ukhimath area of Garhwal Himalaya, India.

Natural radiation is the largest contributor to the collective radiation dose of the world population. It is widely distributed in different geological formations such as soil, rocks, air and groundwater. In the present investigation, (226)Ra, (232)Th and (40)K were measured in soil samples of the Ukhimath region of Garhwal Himalaya, India using NaI(Tl) gamma-ray spectrometry. The activity concentrations of naturally occurring radionuclides (226)Ra, (232)Th and (40)K were found to vary from 38.4 ± 6.1 to 141.7 ± 11.9 Bq kg(-1) with an average of 80.5 Bq kg(-1), 57.0 ± 7.5 to 155.9 ± 12.4 Bq kg(-1) with an average of 118.9 Bq kg(-1) and 9.0 ± 3.0 to 672.8 ± 25.9 Bq kg(-1) with an average of 341 Bq kg(-1), respectively. The total absorbed gamma dose rate varies from 70.4 to 169.1 nGy h(-1) with an average of 123.4 nGy h(-1). This study is important to generate a baseline data of radiation exposure in the area. Health hazard effects due to natural radiation exposure are discussed in details.

Estimation of indoor radon concentration based on radon flux from soil and groundwater.

The indoor radon concentration was estimated based on the radon flux in soil and groundwater. The indoor radon concentration in Budhakedar area of Garhwal Himalaya, India is estimated to be 3.0-131.4 Bq/m(3) in summer and 4.6-92.4 Bq/m(3) in winter. Based on the available data from study area, the calculated value of diffusion coefficient for the soil ranges from 0.1×10(-2) to 3.0×10(-2)cm(2) s(-1) in the summer season and 0.1×10(-2) to 0.4×10(-2)cm(2) s(-1) in the winter season. The calculated value of diffusion flux in the study area is found to vary from 0.1×10(-2) to 16.1×10(-2)Bq m(-2) s(-1) in summer season and 0.1×10(-2)-12.2×10(-2)Bq m(-2) s(-1) in winter season. The formulation was tested by comparing the results of radon values from two different seasons of a year.

Preliminary indoor thoron measurements in high radiation background area of southeastern coastal Orissa, India.

This paper presents the preliminary results of radon and thoron measurements in the houses of Chhatrapur area of southeastern coast of Orissa, India. This area is one of the high radiation background radiation areas in India, which consists of monazite sand as the source of thoron. Both active and passive methods were employed for the measurements. Radon and thoron concentrations were measured in the houses of Chhatrapur area using twin cup radon dosemeters, RAD7 and radon-thoron discriminative detector (Raduet). Thoron progeny concentration was also measured in the houses using deposition rate measurements. Radon and thoron concentrations in the houses of study area were found to vary from 8 to 47 Bq m(-3) and the below detection level to 77 Bq m(-3), respectively. While thoron progeny concentration in these houses ranges between 0.17 and 4.24 Bq m(-3), preliminary investigation shows that the thoron concentration is higher than radon concentration in the houses of the study area. The thoron progeny concentration was found to be comparatively higher, which forms a base for further study in the area. The comparison between the results of various techniques is presented in this paper.

(226)Ra, (232)Th and (40)K contents in soil samples from Garhwal Himalaya, India, and its radiological implications.

The exposure of human beings to ionising radiation from natural sources is a continuing and inescapable feature of life on earth. Natural radionuclides are widely distributed in various geological formations and ecosystems such as rocks, soil groundwater and foodstuffs. In the present study, the distribution of (226)Ra, (232)Th and (40)K was measured in soil samples collected from different lithological units of the Thauldhar and Budhakedar regions of Garhwal Himalaya, India. The collected soil samples were analysed using gamma ray spectrometry. The activity concentrations of the naturally occurring radionuclides (226)Ra, (232)Th and (40)K in these soil samples were found to vary from below detection level (BDL) to 131 +/- 18 Bq kg(-1), 9 +/- 6 to 384 +/- 53 Bq kg(-1) and 471 +/- 96 to 1406 +/- 175 Bq kg(-1), respectively. The distribution of radionuclides depends upon the rock formation and chemical properties within the earth. The activity concentrations vary widely depending on the sample origin. The external absorbed gamma dose rates due to (226)Ra, (232)Th and (40)K were found to vary from 49 to 306 nGy h(-1). The average radium equivalent activity from these soil samples was 300 Bq kg(-1).