ABSTRACT
This paper presents experimental results from a pulsed quantum cascade laser based cavity ringdown spectrometer used as a high-throughput detection system. The results were obtained from an optical cavity with 99.8% input and output coupling mirrors that was rapidly swept (0.2s to 7s sweep times) between 1582.25 cm(-1) (6.3201µm) and 1697.00 cm(-1) (5.8928µm). The spectrometer was able to monitor gas species over the pressure range 585 torr to 1µtorr, and the analysis involves a new digital data processing system that optimises the processing speed and minimises the data storage requirements. In this approach we show that is it not necessary to make direct measurements of the ringdown time of the cavity to obtain the system dynamics. Furthermore, we show that correct data processing is crucial for the ultimate implementation of a wideband IR spectrometer that covers a range similar to that of commercial Fourier transform infrared instruments.
ABSTRACT
This paper presents results from a pulsed-laser cavity ring-down spectrometer with novel field programable gate array real-time data collection. We show both theoretically and experimentally that the data extraction can be achieved from a single cavity ringdown event, and that the absorbance can be determined without the need to fit the ringdown time explicitly. This methodology could potentially provide data acquisition rate up to 1 MHz, with the accuracy and precision comparable to nonlinear least squares fitting algorithms.
ABSTRACT
In this paper we report on the development of a Fourier-transform based signal processing method for laser-locked Continuous Wave Cavity Ringdown Spectroscopy (CWCRDS). Rather than analysing single ringdowns, as is the norm in traditional methods, we amplitude modulate the incident light, and analyse the entire waveform output of the optical cavity; our method has more in common with Cavity Attenuated Phase Shift Spectroscopy than with traditional data analysis methods. We have compared our method to Levenburg-Marquardt non linear least squares fitting, and have found that, for signals with a noise level typical of that from a locked CWCRDS instrument, our method has a comparable accuracy and comparable or higher precision. Moreover, the analysis time is approximately 500 times faster (normalised to the same number of time domain points). Our method allows us to analyse any number of periods of the ringdown waveform at once: this allows the method to be optimised for speed and precision for a given spectrometer.
Subject(s)
Algorithms , Lasers , Spectrum Analysis/instrumentation , Spectrum Analysis/methods , Fourier AnalysisABSTRACT
We present the key elements required for continuous variable parallel quantum information protocols based on spatial multimode quantum correlations. We describe techniques for encoding, combining and detecting spatial quantum information with high efficiency in the individual transverse modes. Until now, the missing feature for the implementation of such protocols was the generation of squeezing in higher order transverse Hermite-Gauss modes. We experimentally demonstrate squeezing in selective modes by fine-tuning the phase matching condition of the nonlinear chi(2) material and the cavity resonance condition of an optical parametric amplifier. Combined, these results open the way to practical multimode optical quantum information systems.
ABSTRACT
We experimentally demonstrate the generation of optical squeezing at multiple longitudinal modes and transverse Hermite-Gauss modes of an optical parametric amplifier. We present measurements of approximately 3 dB squeezing at baseband, 1.7 GHz, 3.4 GHz and 5.1 GHz which correspond to the first, second and third resonances of the amplifier. We show that both the magnitude and the bandwidth of the squeezing at the higher longitudinal modes is greater than can be observed at baseband. The squeezing observed is the highest frequency squeezing reported to date.
ABSTRACT
Second harmonic generation (SHG) can be used as a technique for controlling the spatial mode structure of optical beams. We demonstrate experimentally the generation of higher-order spatial modes, and the possibility to use nonlinear phase matching as a predictable and robust technique for the conversion of transverse electric modes of the second harmonic output. The details of this effect are well described by our wave propagation models, which include mode dependent phase shifts. This is, to our knowledge, the first detailed study of spatial mode conversion in SHG. We discuss potential applications of this effect.
ABSTRACT
Cavity ringdown spectra of ammonia at 10 parts in 10(9) by volume (ppbv) and higher concentrations were recorded by use of a 16-mW continuous-wave quantum-casacde distributed-feedback laser at 8.5 mum whose wavelength was continuously temperature tuned over 15 nm. A sensitivity (noise-equivalent absorbance) of 3.4x10(-9) cm(-1) Hz(-1/2) was achieved for ammonia in nitrogen at standard temperature and pressure, which corresponds to a detection limit of 0.25 ppbv.
ABSTRACT
When the frequency of light coupled into a cavity is suddenly shifted, the radiation emanating from the input port of the previously excited cavity can beat with the reflection of the frequency-shifted input on the surface of a photodetector. When the beat frequency is stable, the time decay of the resulting optical heterodyne signal can be used to measure intracavity absorption spectra with near quantum-limited sensitivity.
ABSTRACT
We present measurements of the power noise that is due to optical amplification in a laser-diode-pumped Nd:YAG free-space traveling-wave linear amplifier in a master-oscillator-power-amplifier configuration. The quantum noise behavior of the optical amplifier was demonstrated by use of InGaAs photodetectors in a balanced detection configuration, at a total photocurrent of 100 mA and in a frequency band from 6.25 to 15.625 MHz. The experimental results are in good agreement with predictions.
ABSTRACT
We analyze and test a laboratory benchtop version of a compound interferometric phase sensor, a Michelson interferometer whose output is combined coherently with a phase-modulated local oscillator beam tapped off the Michelson input beam. This configuration models a whole class of external-modulation interferometers designed to shift signals, obscured by low-frequency intensity noise of the light source, into a shot-noise-limited region of the photocurrent spectrum. We find analytically that the shot-noise-limited sensitivity achievable with this system is comparable with that obtained by using internal phase modulation, with both schemes suffering (for different reasons) approximately a 22% sensitivity penalty compared with ideal shot-noise-limited direct detection. Experimentally we achieve true shot-noise-limited sensitivity, and we investigate trade-offs necessitated by commonly encountered nonideal features in any external-modulation system. Our analytic model, which specifically accounts for Michelson fringe contrast, electronic receiver noise, phase-modulation depth, and the local oscillator tap-off fraction, is sufficiently accurate to predict the absolute sensitivity of our benchtop instrument to within 0.5 dB.
