UV 30†fs laser pulse generation using a multi-pass cell.

Ultrashort ultraviolet (UV) pulses are pivotal for resolving ultrafast electron dynamics. However, their efficient generation is strongly impeded by material dispersion and two-photon absorption, in particular, if pulse durations around a few tens of femtoseconds or below are targeted. Here, we present a new (to our knowledge) approach to ultrashort UV pulse generation: using the fourth-harmonic generation output of a commercial ytterbium laser system delivering 220 fs UV pulses, we implement a multi-pass cell (MPC) providing 5.6 µJ pulses at 256 nm, compressed to 30.5 fs. Our results set a short-wavelength record for MPC post-compression while offering attractive options to navigate the trade-off between upconversion efficiency and acceptance bandwidth for UV pulse production.

Free-space quasi-phase matching.

We report a new, to the best of our knowledge, approach to phase matching of nonlinear materials based on the free-space multipass cells. This technique is applicable to noncentrosymmetric nonlinear crystals, including crystals that cannot be birefringent phase-matched or quasi-phase matched by periodic poling. Notably, by using this approach, the crystalline quartz is quasi-phase matched with the demonstrated increase of the second harmonic generation efficiency by a factor of 40. The method can be extended toward UV and THz ranges. This promises to revolutionize experimental nonlinear optics and all applications by increasing the number of available crystals for quasi-phase matching by at least one order of magnitude and brings fresh motivation for developing novel nonlinear materials.

Spectral broadening in convex-concave multipass cells.

Since its first demonstration in 2016, the multi-pass spectral broadening technique has covered impressive ranges of pulse energy (3 µJ - 100 mJ) and peak power (4 MW - 100 GW). Energy scaling of this technique into the joule-level is currently limited by phenomena such as optical damage, gas ionization and spatio-spectral beam inhomogeneity. These limitations can be overcome by the novel multi-pass convex-concave arrangement, which exhibits crucial properties such as large mode size and compactness. In a proof-of-principle experiment, 260 fs, 15 µJ and 200 µJ pulses are broadened and subsequently compressed to approximately 50 fs with 90% efficiency and excellent spatio-spectral homogeneity across the beam profile. We simulate the proposed concept for spectral broadening of 40 mJ and 1.3 ps input pulses and discuss the possibility of further scaling.

Multipass spectral broadening and compression in the green spectral range.

Multipass spectral broadening and compression around 515 nm are experimentally demonstrated. A nonlinear multipass cell with a bulk medium is used to compress 250-fs pulses down to 38 fs. The same input pulses create a sufficient bandwidth for sub-20-fs pulse generation in a multipass cell with gaseous media. In both cases, the efficiency exceeds 85%. Dispersion management by reduction of the cell size and the thickness of the nonlinear medium allows an efficient generation of ultrashort pulses in the visible range and establishes a pathway for ultraviolet spectral broadening by means of multipass cells.

Direct refractive index retrieval from interferometry measurements.

We present an alternative numerical method to the Abel inversion technique, which can be applied to complex non-symmetrical systems. A comparison with the Abel inversion algorithm was conducted. For benchmarking, the method was applied to a synthetic trace representing a plasma waveguide characterized by a constant parabolic density profile. Furthermore, the temperature and refractive index of a plume of hot air surrounding a non-cylindrical soldering iron were retrieved. Temperatures between 50 °C and 200 °C were successfully retrieved within the instrument precision. The proposed method allows robust and fast data retrieval while maintaining the accuracy and resolution of well-known methods, as Abel inversion.