Two-photon emission from a superlattice-based superconducting light-emitting structure.

Superconductor-semiconductor hybrid devices can bridge the gap between solid-state-based and photonics-based quantum systems, enabling new hybrid computing schemes, offering increased scalability and robustness. One example for a hybrid device is the superconducting light-emitting diode (SLED). SLEDs have been theoretically shown to emit polarization-entangled photon pairs by utilizing radiative recombination of Cooper pairs. However, the two-photon nature of the emission has not been shown experimentally before. We demonstrate two-photon emission in a GaAs/AlGaAs SLED. Measured electroluminescence spectra reveal unique two-photon superconducting features below the critical temperature (Tc), while temperature-dependent photon-pair correlation experiments (g(2)(τ,T)) demonstrate temperature-dependent time coincidences below Tc between photons emitted from the SLED. Our results pave the way for compact and efficient superconducting quantum light sources and open new directions in light-matter interaction studies.

Enhanced Cooper-Pair Injection into a Semiconductor Structure by Resonant Tunneling.

We demonstrate enhanced Andreev reflection in a Nb/InGaAs/InP-based superconductor-semiconductor hybrid device resulting in increased Cooper-pair injection efficiency, achieved by Cooper-pair tunneling into a semiconductor quantum well resonant state. We show this enhancement by investigating the differential conductance spectra of two kinds of samples: one exhibiting resonant states and one which does not. We observe resonant features alongside strong enhancement of Cooper pair injection in the resonant sample, and lack of Cooper pair injection in the nonresonant sample. The theoretical modeling for measured spectra by a numerical approach agrees well with the experimental data. Our findings open a wide range of directions in condensed matter physics and in quantum technologies such as superconducting light-emitting diodes and structures supporting exotic excitations.

High-T c Cooper-pair injection in a semiconductor-superconductor structure.

We observe Andreev reflection in a YBCO-GaN junction through differential conductance spectroscopy. A strong characteristic zero-bias peak was observed and persisted up to the critical temperature of the superconductor with a smaller superconducting order parameter Δ âˆ¼ 1 meV. The presence of Andreev reflection with the small Δ in comparison to its value for high-T c superconductors forms an important milestone toward demonstration of superconducting proximity in high-T c/semiconductor junctions. Experimental results were then compared to the theoretical model with good agreement. Efficient injection of Cooper pairs into direct bandgap semiconducting structures, together with high transition temperature of YBCO, can pave the way to novel optoelectronics and quantum optical studies of high-T c materials.

Enhanced two-photon amplification in superconductor-semiconductor plasmonic waveguides.

We theoretically demonstrate significant enhancement of two-photon amplification by using a superconductor for both a Cooper-pair source and surface plasmon-polariton mode guiding. Cooper-pair-based gain active region restriction to the superconductor-semiconductor interface limits its potentially highly efficient two-photon gain process. Using the superconductor layer for a plasmonic waveguide structure allows strong photon confinement while reducing design and fabrication constraints. This results in three orders of magnitude enhancement of the superconducting two-photon gain (TPG) compared to superconductor-based dielectric waveguides. Moreover, a superconducting TPG produced by a plasmonic waveguide increases with carrier concentration, meeting practical device requirements. Our results pave the way for efficient two-photon amplification realization in nanoscale devices.

Observation of 2D semiconductor P-type dark-exciton lifetime using two-photon ultrafast spectroscopy.

We report direct measurements of intrinsic lifetimes of P-type dark-excitons in MoS2 monolayers. Using sub-gap excitation, we demonstrate two-photon excited direct population of P-type dark excitons, observe their scattering to bright states and decay with femtosecond resolution. In contrast to one-photon excitation schemes, non-monotonic density variation in bright exciton population observed under two-photon excitation shows the indirect nature of its population and competing decay pathways. Detailed modeling of different recombination pathways of bright and dark excitons allows experimental measurement of 2P dark → 1S bright exciton scattering rates. These insights into the dark states in a MoS2 monolayer pave the way for novel devices such as quantum memories and computing.

Andreev Reflection in a Superconducting Light-Emitting Diode.

We experimentally demonstrate Cooper-pair injection into a superconducting light-emitting diode by observing Andreev reflection at the superconductor-semiconductor interface, overcoming the contradicting requirements of an electrically transparent interface and radiative recombination efficiency. The device exhibits electroluminescence enhancement at the quasi-Fermi energy at temperatures below Tc. The theoretically predicted conductance and electroluminescence spectra based on Cooper-pair injection into the semiconductor correspond well to our experimental results. Our findings pave the way for practical superconductor-semiconductor quantum light sources.

Nanoscale High-Tc YBCO/GaN Super-Schottky Diode.

We demonstrate a high-temperature nanoscale super-Schottky diode based on a superconducting tunnel junction of pulsed-laser-deposited YBCO on GaN thin films. A buffer-free direct growth of nanoscale YBCO thin films on heavily doped GaN was performed to realize a direct high-Tc superconductor-semiconductor junction. The junction shows strongly non-linear I-V characteristics, which have practical applications as a low-voltage super-Schottky diode for microwave mixing and detection. The V-shaped differential conductance spectra observed across the junction are characteristic of the c-axis tunneling into a cuprate superconductor with a certain disorder level. This implementation of the super-Schottky diode, supported by the buffer-free direct growth of nanoscale high-Tc thin films on semiconductors, paves the way for practical large-scale fabrication and integration of high-Tc-superconductor devices in future technologies.

Experimental Demonstration of the Effectiveness of Electromagnetically Induced Transparency for Enhancing Cross-Phase Modulation in the Short-Pulse Regime.

We present an experiment using a sample of laser-cooled Rb atoms to show that cross-phase modulation schemes continue to benefit from electromagnetically induced transparency (EIT) even as the transparency window is made narrower than the signal bandwidth (i.e., for signal pulses much shorter than the response time of the EIT system). Addressing concerns that narrow EIT windows might not prove useful for such applications, we show that while the peak phase shift saturates in this regime, it does not drop, and the time-integrated effect continues to scale inversely with EIT window width. This integrated phase shift is an important figure of merit for tasks such as the detection of single-photon-induced cross-phase shifts. Only when the window width approaches the system's dephasing rate γ does the peak phase shift begin to decrease, leading to an integrated phase shift that peaks when the window width is equal to 4γ.

Spin-patterned plasmonics: towards optical access to topological-insulator surface states.

Topological insulators (TI) are new phases of matter with topologically protected surface states (SS) possessing novel physical properties such as spin-momentum locking. Coupling optical angular momentum to the SS is of interest for both fundamental understanding and applications in future spintronic devices. However, due to the nanoscale thickness of the surface states, the light matter interaction is dominated by the bulk. Here we propose and experimentally demonstrate a plasmonic cavity enabling both nanoscale light confinement and control of surface plasmon-polariton (SPP) spin angular momentum (AM)--towards coupling to topological-insulator SS. The resulting SPP field components within the cavity are arranged in a chess-board-like pattern. Each chess-board square exhibits approximately a uniform circular polarization (spin AM) of the local in-plane field interleaved by out-of-plane field vortices (orbital AM). As the first step, we demonstrate the predicted pattern experimentally by near-field measurements on a gold-air interface, with excellent agreement to our theory. Our results pave the way towards efficient optical access to topological-insulator surface states using plasmonics.

Quantum data compression of a qubit ensemble.

Data compression is a ubiquitous aspect of modern information technology, and the advent of quantum information raises the question of what types of compression are feasible for quantum data, where it is especially relevant given the extreme difficulty involved in creating reliable quantum memories. We present a protocol in which an ensemble of quantum bits (qubits) can in principle be perfectly compressed into exponentially fewer qubits. We then experimentally implement our algorithm, compressing three photonic qubits into two. This protocol sheds light on the subtle differences between quantum and classical information. Furthermore, since data compression stores all of the available information about the quantum state in fewer physical qubits, it could allow for a vast reduction in the amount of quantum memory required to store a quantum ensemble, making even today's limited quantum memories far more powerful than previously recognized.

Experimental demonstration of a flexible time-domain quantum channel.

We present an experimental realization of a flexible quantum channel where the Hilbert space dimensionality can be controlled electronically. Using electro-optical modulators (EOM) and narrow-band optical filters, quantum information is encoded and decoded in the temporal degrees of freedom of photons from a long-coherence-time single-photon source. Our results demonstrate the feasibility of a generic scheme for encoding and transmitting multidimensional quantum information over the existing fiber-optical telecommunications infrastructure.

Scalable spatial superresolution using entangled photons.

N00N states-maximally path-entangled states of N photons-exhibit spatial interference patterns sharper than any classical interference pattern. This is known as superresolution. However, even given perfectly efficient number-resolving detectors, the detection efficiency of all previous measurements of such interference would decrease exponentially with the number of photons in the N00N state, often leading to the conclusion that N00N states are unsuitable for spatial measurements. A technique known as the "optical centroid measurement" has been proposed to solve this and has been experimentally verified for photon pairs; here we present the first extension beyond two photons, measuring the superresolution fringes of two-, three-, and four-photon N00N states. Moreover, we compare the N00N-state interference to the corresponding classical superresolution interference. Although both provide the same increase in spatial frequency, the visibility of the classical fringes decreases exponentially with the number of detected photons. Our work represents an essential step forward for quantum-enhanced measurements, overcoming what was believed to be a fundamental challenge to quantum metrology.

Observing the onset of effective mass.

The response of a particle in a periodic potential to an applied force is commonly described by an effective mass, which accounts for the detailed interaction between the particle and the surrounding potential. Using a Bose-Einstein condensate of (87)Rb atoms initially in the ground band of an optical lattice, we experimentally show that the initial response of a particle to an applied force is in fact characterized by the bare mass. Subsequently, the particle response undergoes rapid oscillations and only over time scales that are long compared to those of the interband dynamics is the effective mass observed to be an appropriate description. Our results elucidate the role of the effective mass on short time scales, which is relevant for example in the interaction of few-cycle laser pulses with dielectric and semiconductor materials.

Enhanced coherence between condensates formed resonantly at different times.

We demonstrate coherence between exciton-polariton condensates created resonantly at different times. The coherence persists much longer than the individual particle dephasing time, and this persistence increases as the particle density increases. The observed coherence time exceeds that of the injecting laser pulse by more than an order of magnitude. We show that this significant coherence enhancement relies critically on the many-body particle interactions, as verified by its dependence on particle density, interaction strength, and bath temperature, whereas the mass of the particles plays no role in the condensation of resonantly injected polaritons. Furthermore, we observe a large nonlinear phase shift resulting from intra-condensate interaction energy. Our results provide a new approach for probing ultrafast dynamics of resonantly-created condensates and open new directions in the study of coherence in matter.

Violation of Heisenberg's measurement-disturbance relationship by weak measurements.

While there is a rigorously proven relationship about uncertainties intrinsic to any quantum system, often referred to as "Heisenberg's uncertainty principle," Heisenberg originally formulated his ideas in terms of a relationship between the precision of a measurement and the disturbance it must create. Although this latter relationship is not rigorously proven, it is commonly believed (and taught) as an aspect of the broader uncertainty principle. Here, we experimentally observe a violation of Heisenberg's "measurement-disturbance relationship", using weak measurements to characterize a quantum system before and after it interacts with a measurement apparatus. Our experiment implements a 2010 proposal of Lund and Wiseman to confirm a revised measurement-disturbance relationship derived by Ozawa in 2003. Its results have broad implications for the foundations of quantum mechanics and for practical issues in quantum measurement.

Proximity-induced high-temperature superconductivity in the topological insulators Bi2Se3 and Bi2Te3.

Interest in the superconducting proximity effect has been reinvigorated recently by novel optoelectronic applications as well as by the possible emergence of the elusive Majorana fermion at the interface between topological insulators and superconductors. Here we produce high-temperature superconductivity in Bi(2)Se(3) and Bi(2)Te(3) via proximity to Bi(2)Sr(2)CaCu(2)O(8+δ), to access higher temperature and energy scales for this phenomenon. This was achieved by a new mechanical bonding technique that we developed, enabling the fabrication of high-quality junctions between materials, unobtainable by conventional approaches. We observe proximity-induced superconductivity in Bi(2)Se(3) and Bi(2)Te(3) persisting up to at least 80 K-a temperature an order of magnitude higher than any previous observations. Moreover, the induced superconducting gap in our devices reaches values of 10 mV, significantly enhancing the relevant energy scales. Our results open new directions for fundamental studies in condensed matter physics and enable a wide range of applications in spintronics and quantum computing.

Dynamic Stark effect in strongly coupled microcavity exciton polaritons.

We present experimental observations of a nonresonant dynamic Stark shift in strongly coupled microcavity quantum well exciton polaritons--a system which provides a rich variety of solid-state collective phenomena. The Stark effect is demonstrated in a GaAs/AlGaAs system at 10 K by femtosecond pump-probe measurements, with the blueshift approaching the meV scale for a pump fluence of 2 mJ cm(-2) and 50 meV red detuning, in good agreement with theory. The energy level structure of the strongly coupled polariton Rabi doublet remains unaffected by the blueshift. The demonstrated effect should allow generation of ultrafast density-independent potentials and imprinting well-defined phase profiles on polariton condensates, providing a powerful tool for manipulation of these condensates, similar to dipole potentials in cold-atom systems.

Multidimensional quantum information based on single-photon temporal wavepackets.

We propose a multidimensional quantum information encoding approach based on temporal modulation of single photons, where the Hilbert space can be spanned by an in-principle infinite set of orthonormal temporal profiles. We analyze two specific realizations of such modulation schemes, and show that error rate per symbol can be smaller than 1% for practical implementations. Temporal modulation may enable multidimensional quantum communication over the existing fiber optical infrastructure, as well as provide an avenue for probing high-dimensional entanglement approaching the continuous limit.

Ultrafast three-photon counting in a photomultiplier tube.

We demonstrate experimentally ultrafast three-photon counting by three-photon absorption in a GaAsP photomultiplier tube at the wavelength range of 1800-1900 nm, and analyze its sensitivity and time response. Pulse energy of ∼500 fJ is shown to be detectable for ultrafast 170 fs pulses. The presented three-photon counter may serve as a unique tool for ultrafast quantum state characterization as well as for ultrasensitive third-order temporal measurements.

Indistinguishable photon pairs from independent true chaotic sources.

Indistinguishability of events in quantum mechanics is manifested by interference between their probability amplitudes. We report a unique kind of interference occurring between indistinguishable events of photon-pair emission, where each photon of the pair is emitted from a distinct true chaotic light source and has a different energy. The indistinguishability results in an interference which is observed as an ultrafast modulation of the second-order coherence function, measured on a femtosecond time scale by two-photon absorption in a semiconductor photomultiplier tube.