Midinfrared frequency comb by difference frequency of erbium and thulium fiber lasers in orientation-patterned gallium phosphide.

We generate over 60 mW of pulses with wavelengths from 6 to 11 micrometers by difference frequency mixing between erbium and thulium fiber amplifiers in orientation-patterned GaP with a photon conversion efficiency of 0.2. By stabilizing the repetition rate of the shared oscillator and adding a frequency shifter to one arm, the output becomes a frequency comb with tunable carrier envelope offset.

Imaging of isolated molecules with ultrafast electron pulses.

Imaging isolated molecules in three dimensions with atomic resolution is important for elucidating complex molecular structures and intermediate states in molecular dynamics. This goal has so far remained elusive due to the random orientation of molecules in the gas phase. We show that three-dimensional structural information can be retrieved from multiple electron diffraction patterns of aligned molecules. The molecules are aligned impulsively with a femtosecond laser pulse and probed with a femtosecond electron pulse two picoseconds later, when the degree of alignment reaches a maximum.

Highly-efficient coupling of linearly- and radially-polarized femtosecond pulses in hollow-core photonic band-gap fibers.

We demonstrate extremely efficient excitation of linearly-, radially-, and azimuthally-polarized modes in a hollow-core photonic band-gap fiber with femtosecond laser pulses. We achieve coupling efficiencies as high as 98% with linearly polarized input Gaussian beams and with high-power pulses we obtain peak intensities greater than 10(14) W/cm(2) inside and transmitted through the fiber. With radially polarized pulses, we achieve 91% total transmission through the fiber while maintaining the polarization state. Alternatively with azimuthally-polarized pulses, the mode is degraded in the fiber, and the pure polarization state is not maintained.

Silica-glass contribution to the effective nonlinearity of hollow-core photonic band-gap fibers.

We measure the effective nonlinearity of various hollow-core photonic band-gap fibers. Our findings indicate that differences of tens of nanometers in the fiber structure result in significant changes to the power propagating in the silica glass and thus in the effective nonlinearity of the fiber. These results show that it is possible to engineer the nonlinear response of these fibers via small changes to the glass structure.