ABSTRACT
Recent advances in metasurfaces and optical nanostructures have enabled complex control of incident light with optically thin devices. However, it has thus far been unclear whether it is possible to achieve complete linear control of coherent light transmission, that is, independent control of polarization, amplitude, and phase for both input polarization states, with just a single, thin nanostructure array. Here, it is proved possible, and a universal metasurface is proposed, a bilayer array of high-index elliptic cylinders that possesses a complete degree of optical freedom with fully designable chirality and anisotropy. The completeness of achievable light control is mathematically shown with corresponding Jones matrices, new types of 3D holographic schemes that were formerly impossible are experimentally demonstrated, and a systematic way of realizing any input-state-sensitive vector linear optical device is presented. The results unlock previously inaccessible degrees of freedom in light transmission control.
ABSTRACT
In optical nanostructures used as artificial resonance-based color filters, there is unfortunate universal trade-off between spectral sharpness and angular tolerance as well as maximum extinction. We rigorously derive the maximum performance bounds of wavelength-rejection filters realized by single-layer plasmonic metasurfaces with a dominant resonance and weak near-field coupling, and propose a multi-layer approach to overcome these single-layer limits and trade-offs. We also present a realistic example that has a narrow full-width-at-half-maximum bandwidth of 24 nm with 10 dB extinction at 532 nm with good angular tolerance up to 60°. The performance of the proposed metasurface is close to the general theoretical bound.
ABSTRACT
Metasurfaces, or two-dimensional arrays of subwavelength-scale structures, can exhibit extraordinary optical properties. However, typical metasurfaces have a bumpy surface morphology that may restrict their practical applications. Here, we propose and demonstrate an optical metasurface that is composed of a thin metallic film, with hidden dielectric structures underneath, and a metal back mirror layer. Exploiting the large difference between the Thomas-Fermi screening length for longitudinal electric fields and the skin depth for transverse electromagnetic fields, the near-atomically flat top surface of the proposed structure can appear homogeneous chemically and electrically but highly inhomogenous optically. The size and shape of the hidden dielectric structures as well as the thickness of the top metallic layer can be tailored to acquire desired optical properties. We performed both theoretical and experimental studies of the proposed metasurface, finding a good agreement between them. This work provides a new platform for ultra-flat optical devices, such as a wavelength selective electrode, diffusive back reflector, meta-lens, and plasmonically enhanced optical biosensors.
ABSTRACT
Effective surface enhancement of Raman scattering (SERS) requires strong near-field enhancement as well as effective light collection of plasmonic structures. To this end, plasmonic nanoparticle (NP) arrays with narrow gaps or sharp tips have been suggested as desirable structures. We present a highly dense and uniform Au nanoscale gap array enabled by the customized design of NP shape and arrangement employing block copolymer self-assembly. Block copolymer self-assembly in thin films offers uniform hexagonally packed nanopost template arrays over the entire surface of a 2 in. wafer. Conventional evaporative metal deposition over the nanotemplate surface allows precise geometric control and positional arrangement of metal NPs, constituting tunable, strong plasmonic near-field enhancement particularly at the "hot spots" near interparticular nanoscale gaps. Underlying field distribution has been investigated by a finite-difference time-domain simulation. In the detection of thiophenol, our Au nanogap array shows a remarkable enhancement of Raman intensity greater than â¼104, a standard deviation as small as 12.3% compared to that of the planar Au thin film. In addition, adenine biomolecules can be detected with a detection limit as low as 100 nM. Our approach proposes highly sensitive and reliable SERS on the basis of a scalable, low-cost bottom-up strategy.
