Bi-Directional Full-Color Generation and Tri-Channel Information Encoding Based on a Plasmonic Metasurface.

Dynamic optical structural color is always desired in various display applications and usually involves active materials. Full-color generation, especially bi-directional full-color generation in both reflective and transmissive modes, without any active materials included, has rarely been investigated. Herein, we demonstrate a scheme of bi-directional full-color generation based on a plasmonic metasurface modulated by the rotation of the polarization angle of the incident light without varying the geometry and the optical properties of the materials and the environment where the metasurface resides. The metasurface unit cell consists of plasmonic modules aligning in three directions and is patterned in a square array. The metasurface structural color device is numerically confirmed to generate full colors in both reflection and transmission. Based on the proposed polarization-dependent structural color, the information encoding process is demonstrated for three multiplexed animal images and quick-responsive (QR) codes to verify the efficient information encoding and decoding of the proposed scheme. In the simulation, the animals can be seen under different polarization incidences, and the QR codes can be successfully decoded by the polarization rotation in transmission. The proposed bi-directional full-color generation metasurface has great potential in applications such as kaleidoscope generation, anti-counterfeiting, dynamic color display, and optical information encoding.

Broadband Absorption Based on Thin Refractory Titanium Nitride Patterned Film Metasurface.

In this paper, a thin metasurface perfect absorber based on refractory titanium nitride (TiN) is proposed. The size parameter of the metasurface is investigated based on the finite difference time domain method and transfer matrix method. With only a 15-nm-thick TiN layer inside the silica/TiN/silica stacks standing on the TiN substrate, the near-perfect absorption throughout the visible regime is realized. The cross-talk between the upper and lower dielectric layers enables the broadening of the absorption peak. After patterning the thin film into a nanodisk array, the resonances from the nanodisk array emerge to broaden the high absorption bandwidth. As a result, the proposed metasurface achieves perfect absorption in the waveband from 400 to 2000 nm with an average absorption of 95% and polarization-insensitivity under the normal incidence. The proposed metasurface maintains average absorbance of 90% up to 50-degree oblique incidence for unpolarized light. Our work shows promising potential in the application of solar energy harvesting and other applications requiring refractory metasurfaces.

Polarization-Dependent All-Dielectric Metasurface for Single-Shot Quantitative Phase Imaging.

Phase retrieval is a noninterferometric quantitative phase imaging technique that has become an essential tool in optical metrology and label-free microscopy. Phase retrieval techniques require multiple intensity measurements traditionally recorded by camera or sample translation, which limits their applicability mostly to static objects. In this work, we propose the use of a single polarization-dependent all-dielectric metasurface to facilitate the simultaneous recording of two images, which are utilized in phase calculation based on the transport-of-intensity equation. The metasurface acts as a multifunctional device that splits two orthogonal polarization components and adds a propagation phase shift onto one of them. As a proof-of-principle, we demonstrate the technique in the wavefront sensing of technical samples using a standard imaging setup. Our metasurface-based approach fosters a fast and compact configuration that can be integrated into commercial imaging systems.

Multi-frequency surface plasmons supported with a nanoscale non-uniform 2D electron gas formed due to a polar catastrophe at the oxide interface, dispersions, diffractions, and beyond.

Recently, 2D electron gases (2DEGs) formed at oxide interfaces are drawing increasing attention as they cause a myriad of intriguing phenomena. As ideal platforms in supporting surface plasmon polaritons (SPPs) without metallic constituents, such 2DEGs are favorable in non-linear plasmonics for ultra-low total Joule dissipation. Convincingly, an increase in the interfacial electron density (IIED) formed at the interface of indium-tin-oxide and LiNbO3 composite slab is responsible for a number of interesting phenomena, which are hardly explained with the conventional photorefractive theoretical framework but can be satisfactorily elucidated via SPP excitation and resultant colossal non-linear effects. Since the polar-catastrophe-led IIED is universal to all combinations of highly polar ferroelectric oxides (FOs) and less polar transparent conducting oxides (TCOs), a systematic theoretical treatment of an FO/TCO system is pivotal to a variety of promising applications. In this study, the nanometer scale 2DEG at the FO/TCO interface is illustrated theoretically with the Thomas-Fermi screening picture, by taking into account the spontaneous polarization, along with related boundary conditions. The local plasma frequency of 2DEGs can be increased up to the UV regime for the composite slabs discussed, which are suitable for highly desirable visible applications. The SPP dispersion relationship was given for the 2DEG layer sandwiched between the FO slab and the unmodified TCO layer. To further take the non-uniform nature of IIED into account, dramatic dispersions of dielectric permittivity and index of refraction were simulated with a very broad range, hinting at different ways for meeting phase matching conditions and slowing the light for non-linear plasmonic applications, which are confirmed experimentally.

Accumulation-layer hybridized surface plasmon polaritions at an ITO/LiNbO3 interface.

To circumvent the hindrance to broad practical applications associated with uses of highly lossy metals in plasmonics, electrostatic modification-based low-loss structures are conceived and demonstrated in supporting surface plasmon polaritions (SPPs). Pairing a highly polar LiNbO3 (LN) slab with a nonpolar indium-tin-oxide (ITO) thin film, a subnanometer ITO layer was modified into visible SPPs supportive owing to electrostatic screening; yet a theoretical treatment of a sandwiched structure with a sub-nanometer interlayer and an anisotropic substrate is still missing. In this Letter, a hybridized SPP supporting picture was drawn in the ITO/LN system, which agrees well with the 2D diffraction patterns observed out of phase gratings written with two coherent laser beams either of pure-extraordinary, pure-ordinary, or mixed polarizations. This platform of ITO/LN is promising in designing hybridized SPP-based devices in which the parasitic scattering of surface waves may be suppressed greatly.

Broadband Perfect Absorber Based on TiN-Nanocone Metasurface.

Based on an integrated array of refractory titanium nitride (TiN), a metasurface perfect absorber (MPA) in the visible-to-near infrared (NIR) band is reported. The systematic and detailed simulation study of the absorption of the MPA is performed with the finite-different time-domain (FDTD) method. Tailoring the structure, the MPA realizes as high an average as 99.6% broadband absorption, ranging from 400 nm to 1500 nm. The broadband perfect absorption can be attributed to localized surface plasmonic resonance (LSPR), excited by the continuous diameter evolution from the apex to the base of the nanocone, and the gap plasmons excited among the nanocones, as well as in the spacer layer at longer wavelengths. Particularly, the coupling of the resonances is essentially behind the broadening of the absorption spectrum. We also evaluated the electric field intensity and polarization-dependence of the nanocone MPA to offer further physical insight into light trapping capability. The MPA shows about 90% average absorption even at an oblique incidence up to 50°, which improves the acceptance capability of light-harvesting system applications. This unique design with the TiN nanocone array/aluminium oxide (Al2O3)/TiN structure shows potential in imminent applications in light trapping and thermophotovoltaics.

Broadband Perfect Absorber with Monolayer MoS2 and Hexagonal Titanium Nitride Nano-disk Array.

A broadband metamaterial absorber (MA) composed of hexagonal-arranged single-sized titanium nitride (TiN) nano-disk array and monolayer molybdenum disulfide (MoS2) is studied using finite-difference time-domain (FDTD) simulations. The structure of TiN nano-disk array/dielectric silica (SiO2)/aluminum (Al) is adopted in our design. By optimizing the dimension parameters of the structure, an average absorption of 96.1% is achieved from 400 to 850 nm. In addition, by inserting a monolayer MoS2 which has high absorption at the short wavelength side underneath the TiN nano-disk array, an average absorption of 98.1% over the entire visible regime from 400 to 850 nm was achieved, with a peak absorption near 100% and absorption over 99% from 475 to 772 nm. Moreover, the absorber presented in this paper is polarization insensitive. This compact and unique design with TiN nano-disk/monolayer MoS2/ SiO2/Al structure may have great potential for applications in photovoltaics and light trapping.