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1.
Nat Commun ; 10(1): 738, 2019 02 13.
Article in English | MEDLINE | ID: mdl-30760712

ABSTRACT

Studies on quantum critical points (QCP) have focused on magnetic QCPs to date. Remarkable phenomena such as superconductivity due to avoided criticality have been discovered, but we focus here on the non-magnetic counterpart, i.e., the superconductivity of SrTiO3 regarded as being close to a ferroelectric QCP. Here we prepare high-quality Sr1-xLaxTi(16O1-z18Oz)3 single crystals without localisation at low temperatures, which allow us to systematically investigate the La substitution of Sr as an alternative to introducing oxygen vacancies. Analysis of our data based on a theoretical model predicts an appearance of the ferroelectric QCP around 3 × 1018 cm-3. Because of the QCP, the superconducting dome of Sr1-xLaxTiO3 can be raised upwards. Furthermore, remarkable enhancement of Tc (~0.6 K) is achieved by 18O exchange on the Sr1-xLaxTiO3 crystals. These findings provide a new knob for observing intriguing physics around the ferroelectric QCP.

2.
Sci Rep ; 6: 25789, 2016 05 12.
Article in English | MEDLINE | ID: mdl-27174141

ABSTRACT

Electrostatic carrier accumulation on an insulating (100) surface of SrTiO3 by fabricating a field effect transistor with Parylene-C (6 nm)/HfO2 (20 nm) bilayer gate insulator has revealed a mystifying phenomenon: sheet carrier density is about 10 times as large as ( is the sheet capacitance of the gate insulator, VG is the gate voltage, and e is the elementary charge). The channel is so clean to exhibit small subthreshod swing of 170 mV/decade and large mobility of 11 cm(2)/Vs for of 1 × 10(14) cm(-2) at room temperature. Since does not depend on either VG nor time duration, beyond is solely ascribed to negative charge compressibility of the carriers, which was in general considered as due to exchange interactions among electrons in the small limit. However, the observed is too large to be naively understood by the framework. Alternative ideas are proposed in this work.

3.
Adv Mater ; 25(15): 2158-61, 2013 Apr 18.
Article in English | MEDLINE | ID: mdl-23382006

ABSTRACT

A Mott transistor that exhibits a large switching ratio of more than two orders at room temperature is demonstrated by using the electric double layer of an ionic liquid for gating on a strongly correlated electron system SmCoO3. From the thickness dependence of the on-state channel current, we estimate the screening length of the SmCoO3 to be ∼5 nm. The good carrier confinement within the Thomas-Fermi screening length demonstrates that the SmCoO3-channel electric double layer transistor is the first candidate for a two-dimensional Mott transistor.

4.
Adv Mater ; 23(48): 5822-7, 2011 Dec 22.
Article in English | MEDLINE | ID: mdl-22105844

ABSTRACT

A prototype Mott transistor, the electric double layer transistor with a strained CaMnO(3) thin film, is fabricated. As predicted by the strain phase diagram of electron-doped manganite films, the device with the compressively strained CaMnO(3) exhibits an immense conductivity modulation upon applying a tiny gate voltage of 2 V.


Subject(s)
Manganese Compounds/chemistry , Electrolytes , Electronics , Electrons , Equipment Design , Magnetics , Materials Testing , Metals/chemistry , Microscopy, Atomic Force/methods , Nanotechnology/instrumentation , Pressure , Temperature , Transistors, Electronic , X-Ray Diffraction
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