RADON INHALATION EXPERIMENTS TO TEST RADON EXHALATION KINETICS.

Three experiments were conducted with a volunteer to test the kinetics of the 222Rn exhalation after a short-time exposure to an elevated 222Rn air concentration. Radon concentration in an exhaled air was measured, complemented by whole body counting of 222Rn decay products in a body. Exhaled activities are compared with the prediction of the recent ICRP biokinetic model for radon. While a rapid equilibration of the exhaled radon activity concentration with that in the air inhaled corresponded with the model, the measured 222Rn exhalation rate was significantly less than modelled. Five hours after termination of the inhalation phase, the radon concentration in the exhaled air decreased to levels expected for non-elevated indoor radon activity concentration. Whole body activities of the 222Rn decay products were found higher than expected. Inhalation of the unattached fraction or residual activity of decay products in the air inhaled may be the explanation.

THE NRPI MULTI-PURPOSE ON-LINE MONITORING STATION FOR MEASUREMENT OF NATURAL RADIOACTIVITY IN THE AMBIENT ATMOSPHERE AND IN THE SOIL.

During years 2010-12 an automated, on-line and wireless outdoor measurement station of atmospheric radon, gamma dose rate and meteorological parameters was realised at the National Radiation Protection Institute (NRPI) in Prague. At the turn of the year 2013 an expansion of the existing station was completed. Under the project funded by the Czech Technological Agency a new updated station was established, additionally equipped with modules for measurement of atmospheric radon/thoron short-lived decay products, radon in water and soil and radon exhalation rate from soil. After the introduction of the station updated key detection parameters and benefits, its use for atmospheric modelling and monitoring is demonstrated. There are summarised results from the 3-year measurement period in the NRPI outdoor area in Prague and from simultaneous annual measurement performed by another similar station located near uranium mud fields in DIAMO, state enterprise, Stráz pod Ralskem. Observed seasonal and diurnal variations of atmospheric radon concentrations and variability of the equilibrium factor, F, are illustrated and compared.

2014 ICHLNRRA intercomparison of radon/thoron gas and radon short-lived decay products measuring instruments in the NRPI Prague.

During the Eighth International Conference on High Levels of Natural Radiation and Radon Areas held in autumn 2014 at Prague, the third intercomparison of radon/thoron gas and radon short-lived decay products measurement instruments was organised by and held at the Natural Radiation Division of the National Radiation Protection Institute (NRPI; SÚRO v.v.i.) in Prague. The intercomparison was newly focussed also on continuous monitors with active sampling adapters capable to distinguish radon/thoron gas in their mix field.The results of radon gas measurements carried out in the big NRPI radon chamber indicated very well an average deviation of up to 5 % from the reference NRPI value for 80 % of all the exposed instruments. The results of equilibrium equivalent concentration continuous monitors indicated an average deviation of up to 5 % from the reference NRPI value for 40 % of all the exposed instruments and their ~8-10 % shift compared with the NRPI. The results of investigated ambient conditions upon response of exposed continuous monitors indicated influence of aerosol changes upon response of radon monitors with an active air sampling adapters through the filter, only. The exposures of both radon/thoron gas discriminative continuous monitors and passive detectors have been indicated inconsistent results: on one hand, their excellent agreement up to several per cent for both the gases, and on the other hand, systematic unsatisfactory differences up to 40 %. Additional radon/thoron exercises are recommended to improve both the instruments themselves and quality of their operators.

International intercomparison of measuring instruments for radon/thoron gas and radon short-lived daughter products in the NRPI Prague.

During the 7th European Conference on Protection Against Radon at Home and at Work held in the autumn of 2013 in Prague, the second intercomparison of measuring instruments for radon and its short-lived decay products and the first intercomparison of radon/thoron gas discriminative passive detectors in mix field of radon/thoron were organised by and held at the Natural Radiation Division of the National Radiation Protection Institute (NRPI) in Prague. In total, 14 laboratories from 11 different countries took part in the 2013 NRPI intercomparison. They submitted both continuous monitors for the measurement of radon gas and equivalent equilibrium radon concentration in a big NRPI chamber (48 m3) and sets of passive detectors including radon/thoron discriminative for the measurement of radon gas in the big chamber and thoron gas in a small thoron chamber (150 dm3).

Radon entry rate analyses using in situ tracer gas method application.

Recently, the role of energy savings in indoor air quality deterioration has been extensively emphasised, predominantly in the context of significant air exchange rate reduction as a result of home energy retrofits. In case of refurbishment of existing buildings, the effect of energy-efficient technologies on indoor radon concentration is considerably complex and has to be carefully evaluated with respect to radon entry rate (RER) and air exchange rate alteration. For the purpose of detailed analysis of radon entry pathways, the unique infiltration experiment has been carried out using the tracer gas (N2O) method application in field conditions. Significant amount of experimental works has been done to provide an independent assessment of RER and air-exchange rate facilitating the analysis of fundamental factors influencing the indoor radon variations (e.g. indoor-outdoor pressure difference induced by wind, stack effect, heating, ventilation and operation of air-conditioning systems).

Diurnal and seasonal variability of outdoor radon concentration in the area of the NRPI Prague.

In autumn 2010, an outdoor measuring station for measurement of atmospheric radon, gamma equivalent dose rate in the range of 100 nSv h(-1)-1 Sv h(-1) and proper meteorological parameters such as thermal air gradient, relative air humidity, wind speed and direction and solar radiation intensity was built in the area of the National Radiation Protection Institute vvi. The station was designed to be independent of an electrical network and enables on-line wireless transfer of all data. After introduction of the station, illustrations of its measurement properties and the results of measured diurnal and seasonal variability of atmospheric radon, based on annual continuous measurement using a high-volume scintillation cell at a height of 2.5 m above the ground, are presented.

Results of the 2010 National Radiation Protection Institute intercomparison of radon and its short-lived decay product continuous monitors.

During the Sixth European Conference on Protection Against Radon at Home and at Work held in autumn 2010 in Prague, the first intercomparison of continuous radon and its short-lived decay product monitors was organised and held by the Natural Radiation Division of the National Radiation Protection Institute (NRPI) in Prague. Eight laboratories submitted eight continuous radon monitors, two electronic monitors, three passive integral systems based on charcoal and three continuous radon short-lived decay product monitors. The intercomparison included exposures to both the radon gas concentration and equivalent equilibrium radon concentration (EEC) under different ambient conditions similar to the ones in dwellings. In particular, the influence of the equilibrium factor F, unattached fraction of EEC f(p) and absolute air humidity were investigated. The results of the radon gas measurements were performed on a calibration level of about 8  kBq m(-3). The results of all monitors were compared with the reference NRPI monitor.

Significance of independent radon entry rate and air exchange rate assessment for the purpose of radon mitigation effectiveness proper evaluation: case studies.

Two new single-family houses identified as insufficient with regard to existing radon barrier efficiency, have been selected for further examination. A complex set of radon diagnosis procedures has been applied in order to localise and quantify radon entry pathways into the indoor environment. Independent assessment of radon entry rate and air exchange rate has been carried out using the continuous indoor radon measurement and a specific tracer gas application. Simultaneous assessment of these key determining factors has turned out to be absolutely crucial in the context of major cause identification of elevated indoor radon concentration.

QA programme for radon and its short-lived progeny measuring instruments in NRPI Prague.

To subserve the institutional research and tasks coming out from the Czech National Radon Programme, a new QA programme to calibrate all the known types of devices that measure radon and its short-lived progeny was developed at the Department of Radon mobile group of the National Radiation Protection Institute (NRPI) at Prague. The programme also included calibration of instruments measuring a unique quantity of unattached and attached fractions of short- lived radon progeny Generally, NRPI declares estimation of radon concentration during all routine calibration measurements with an overall uncertainty <5% (one sigma) and of equilibrium-equivalent radon concentration with an overall uncertainty <10% (one sigma). The results of the comparative measurements of the unattached and attached fractions of each short-lived radon progeny carried out with a comparing continuous monitor Fritra 4 in the German reference radon chamber at PTB Braunschweig indicated an acceptable level of agreement, up to 10%.