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1.
ACS Photonics ; 11(4): 1673-1683, 2024 Apr 17.
Article in English | MEDLINE | ID: mdl-38645995

ABSTRACT

High-order harmonic generation (HHG) arising from the nonperturbative interaction of intense light fields with matter constitutes a well-established tabletop source of coherent extreme-ultraviolet and soft X-ray radiation, which is typically emitted as attosecond pulse trains. However, ultrafast applications increasingly demand isolated attosecond pulses (IAPs), which offer great promise for advancing precision control of electron dynamics. Yet, the direct generation of IAPs typically requires the synthesis of near-single-cycle intense driving fields, which is technologically challenging. In this work, we theoretically demonstrate a novel scheme for the straightforward and compact generation of IAPs from multicycle infrared drivers using hollow capillary fibers (HCFs). Starting from a standard, intense multicycle infrared pulse, a light transient is generated by extreme soliton self-compression in a HCF with decreasing pressure and is subsequently used to drive HHG in a gas target. Owing to the subcycle confinement of the HHG process, high-contrast IAPs are continuously emitted almost independently of the carrier-envelope phase (CEP) of the optimally self-compressed drivers. This results in a CEP-robust scheme which is also stable under macroscopic propagation of the high harmonics in a gas target. Our results open the way to a new generation of integrated all-fiber IAP sources, overcoming the efficiency limitations of usual gating techniques for multicycle drivers.

2.
Opt Express ; 29(2): 929-937, 2021 Jan 18.
Article in English | MEDLINE | ID: mdl-33726318

ABSTRACT

The generation of ultrashort visible energetic pulses is investigated numerically by the nonlinear propagation of infrared necklace beams in capillaries. We have developed a (3+1)D model that solves the nonlinear propagation equation, including the complete spatio-temporal dynamics and the azimuthal dependence of these structured beams. Due to their singular nonlinear propagation, the spectrum broadening inside the capillary extends to the visible region in a controlled way, despite the high nonlinearity, avoiding self-focusing. The results indicate that the features of these necklace beams enable the formation of visible pulses with pulse duration below 10 fs and energies of 50 µJ by soliton self-compression dynamics for different gas pressures inside the capillary.

3.
Opt Express ; 26(11): 14108, 2018 05 28.
Article in English | MEDLINE | ID: mdl-29877453

ABSTRACT

The first equation in [Opt. Express26, 6345 (2018)] contains an error and is corrected in this erratum.

4.
Opt Express ; 26(5): 6345-6350, 2018 Mar 05.
Article in English | MEDLINE | ID: mdl-29529826

ABSTRACT

Soliton self-compression is demonstrated during the propagation of high spatial modes in hollow core fibers in the near-infrared spectral region, taking advantage of their negative dispersion response. We have found that there is always an optimum spatial mode to observe this phenomenon, compressing the pulses down to the single-cycle regime without needing any external compression device and with a consequent increase in the output peak power. Our result is relevant for any ultrashort laser application in which few- or single-cycle pulses are crucial.

5.
Opt Lett ; 43(2): 337-340, 2018 Jan 15.
Article in English | MEDLINE | ID: mdl-29328280

ABSTRACT

Intense few- and single-cycle pulses are powerful tools in different fields of science Today, third- and higher-order terms in the remnant spectral phase of the pulses remain a major obstacle for obtaining high-quality few- and single-cycle pulses from in-line post-compression setups. In this Letter, we show how input pulse shaping can successfully be applied to standard post-compression setups to minimize the occurrence of high-order phase components during nonlinear propagation and to directly obtain pulses with durations down to 3 fs. Furthermore, by combining this pulse shaping of the input pulse with new-generation broadband chirped mirrors and material addition for remnant third-order phase correction, pulses down to 2.2 fs duration have been measured.

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