Highly efficient graphene terahertz modulator with tunable electromagnetically induced transparency-like transmission.

Graphene-based optical modulators have been extensively studied owing to the high mobility and tunable permittivity of graphene. However, weak graphene-light interactions make it difficult to achieve a high modulation depth with low energy consumption. Here, we propose a high-performance graphene-based optical modulator consisting of a photonic crystal structure and a waveguide with graphene that exhibits an electromagnetically-induced-transparency-like (EIT-like) transmission spectrum at terahertz frequency. The high quality-factor guiding mode to generate the EIT-like transmission enhances light-graphene interaction, and the designed modulator achieves a high modulation depth of 98% with a significantly small Fermi level shift of 0.05 eV. The proposed scheme can be utilized in active optical devices that require low power consumption.

Terahertz radiation from propagating acoustic phonons based on deformation potential coupling.

We report on new THz electromagnetic emission mechanism from deformational coupling of acoustic (AC) phonons with electrons in the propagation medium of non-polar Si. The epicenters of the AC phonon pulses are the surface and interface of a GaP transducer layer whose thickness (d) is varied in nanoscale from 16 to 45 nm. The propagating AC pulses locally modulate the bandgap, which in turn generates a train of electric field pulses, inducing an abrupt drift motion at the depletion edge of Si. The fairly time-delayed THz bursts, centered at different times (t1T H z, t2T H z, and t3T H z), are concurrently emitted only when a series of AC pulses reach the point of the depletion edge of Si, even without any piezoelectricity. The analysis on the observed peak emission amplitudes is consistent with calculations based on the combined effects of mobile charge carrier density and AC-phonon-induced local deformation, which recapitulates the role of deformational potential coupling in THz wave emission in a formulatively distinct manner from piezoelectric counterpart.

Graphene-based fine tuning of Fano resonance transmission of quasi-bound states in the continuum.

Quasi-bound state in the continuum (BIC) has significant potential because it supports an ultra-high quality factor (Q-factor). Here, we propose a graphene-embedded subwavelength grating that supports quasi-BIC for tuning very sharp Fano resonance transmission. The strongly enhanced light-graphene interaction from the quasi-BIC enables fine variation of the transmission at the resonant wavelength. The Q-factor of quasi-BIC significantly decreases as the Fermi level of graphene increases. We also propose a low-energy consumption THz-wave modulator using this scheme. The designed modulator shows approximately 100% modulation depth with a Fermi level shift of only EF = 90 meV.

Creation of Fano resonances and bound states in the continuum in metallic metasurface superlattices.

A perfect metal film with a periodic arrangement of cut-through slits, an anisotropic metallic metamaterial film, mimics a dielectric slab and supports guided electromagnetic waves in the direction perpendicular to the slits. Since the guided Bloch modes exist only below the light line, conventional metallic metamaterial films do not exhibit interesting leaky-wave effects, such as bound states in the continuum and Fano resonances. Here, we introduce metallic metasurface superlattices that include multiple slits in a period and demonstrate that the superlattices support the Fano resonances and bound states in the continuum. We show that the number of Fano resonances and bound states depend on the number of slits in a period of superlattices through rigorous finite element method simulations. Experimental results in microwave region also support the creation of Fano resonance and bound states in the continuum by the increment of the number of slits in a period of superlattices.

Metasurfaces with Bound States in the Continuum Enabled by Eliminating First Fourier Harmonic Component in Lattice Parameters.

Conventional photonic lattices, such as metamaterials and photonic crystals, exhibit various interesting physical properties that are attributed to periodic modulations in lattice parameters. In this study, we introduce novel types of photonic lattices, namely Fourier-component-engineered metasurfaces, that do not possess the first Fourier harmonic component in the lattice parameters. We demonstrate that these metasurfaces support the continuous high-Q bound states near second stop bands. The concept of engineering Fourier harmonic components in periodic modulations provides a new method to manipulate electromagnetic waves in artificial periodic structures.

Polarization-differentiated band dynamics of resonant leaky modes at the lattice Γ point.

In the physical description of photonic lattices, leaky-mode resonance and bound states in the continuum are central concepts. Understanding of their existence conditions and dependence on lattice parameters is of fundamental interest. Primary leaky-wave effects are associated with the second stop band at the photonic lattice Γ point. The pertinent band gap is defined by the frequency difference between the leaky-mode band edge and the bound-state edge. This paper address the polarization properties of the band gaps resident in laterally periodic one-dimensional photonic lattices. We show that the band gaps pertinent to TM and TE leaky modes exhibit significantly differentiated evolution as the lattice parameters vary. This is because the TM band gap is governed by a surface effect due to the discontinuity of the dielectric constant at the interfaces of the photonic lattice as well as by a Bragg effect due to the periodic in-plane dielectric constant modulation. We find that when the lattice is thin (thick), the surface (Bragg) effect dominates the Bragg (surface) effect in the formation of the TM band. This leads to complex TM band dynamics with multiple band closures possible under parametric variation. In complete contrast, the TE band gap is governed only by the Bragg effect thus exhibiting simpler band dynamics. This research elucidates the important effect of polarization on resonant leaky-mode band dynamics whose explanation has heretofore not been available.

Strong Linear Correlation between CH3NH2 Molecular Defect and THz-Wave Absorption in CH3NH3PbI3 Hybrid Perovskite Thin Film.

To control the density of a CH3NH2 molecular defect, which strongly contributed to a significant THz-wave absorption property in the CH3NH3PbI3 hybrid perovskite thin film formed by the sequential vacuum evaporation method, we performed post-annealing processes with various temperatures and times. In the thin film after post-annealing at 110 °C for 45 min, the density of the CH3NH2 molecular defect was minimized, and CH3NH3I and PbI2 disappeared in the thin film after the post-annealing process at 150 °C for 30 min. However, the density of the CH3NH2 molecular defect increased. Moreover, the THz-wave absorption property for each thin film was obtained using a THz time-domain spectroscopy to understand the correlation between the density of a molecular defect and the THz-wave oscillation strength at 1.6 THz, which originated in the molecular defect-incorporated hybrid perovskite structure. There is a strong linear correlation between the oscillator strength of a significant THz-wave absorption at 1.6 THz and the CH3NH2 molecular defect density.

Scalable terahertz generation by large-area optical rectification at 80 TW laser power.

We demonstrate high-energy terahertz generation from a large-aperture (75-mm diameter) lithium niobate wafer by using a femtosecond laser with energy up to 2 J. This scheme utilizes optical rectification in a bulk lithium niobate crystal, where most terahertz energy is emitted from a thin layer of the rear surface. Despite its simple setup, this scheme can yield 0.19 mJ of terahertz energy with laser-to-terahertz conversion efficiencies of ∼10-4, about 3 times better than ZnTe when pumped at 800 nm. The experimental setup is upscalable for multimillijoule terahertz generation with petawatt laser pumping.

Significant THz absorption in CH3NH2 molecular defect-incorporated organic-inorganic hybrid perovskite thin film.

The valid strong THz absorption at 1.58 THz was probed in the organic-inorganic hybrid perovskite thin film, CH3NH3PbI3, fabricated by sequential vacuum evaporation method. In usual solution-based methods such as 2-step solution and antisolvent, we observed the relatively weak two main absorption peaks at 0.95 and 1.87 THz. The measured absorption spectrum is analyzed by density-functional theory calculations. The modes at 0.95 and 1.87 THz are assigned to the Pb-I vibrations of the inorganic components in the tetragonal phase. By contrast, the origin of the 1.58 THz absorption is due to the structural deformation of Pb-I bonding at the grain boundary incorporated with a CH3NH2 molecular defect.

Theoretical study of photonic bands of one-dimensional photonic crystals containing epsilon-near-zero metamaterials.

The photonic bands of a one-dimensional photonic crystal containing epsilon-near-zero metamaterials are investigated both theoretically and numerically. A theoretical expression of the edge frequencies of the photonic bands derived from the dispersion relation of the photonic crystal is in excellent agreement with the edge frequencies of the photonic bands calculated using the plane wave expansion method. These results are also confirmed using the transmittance obtained from the transfer matrix method. The theoretical expression of the band edge frequencies indicates that the magnitude of the bandgap increases as the frequency increases in the lower bands and becomes saturated in the higher bands. This is because the bands become flat in the higher frequency range.

Trilayer hybrid structures for highly efficient THz modulation.

We demonstrate a novel technique to achieve a highly efficient terahertz (THz) modulation based on hybrid structures of organic layers (fullerene derivative [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) and 6,13-bis(triisopropylsilylethynyl) pentacene (TIPS-pentacene) fabricated on both sides of a silicon (Si) substrate. The organic layer generating an optically induced electron (or hole) transfer is deposited on the back (or front) side of the Si substrate. The spatial charge separation improved owing to the transferred photo-excited electrons or holes at both interfaces of PCBM/Si and TIPS-pentacene/Si, enables a highly efficient THz wave modulation. The photoexcitation on the hole-transfer organic layer (TIPS-pentacene/Si) further improves the modulation efficiency, as the diffusion of electrons through the Si substrate is faster than that of photo-excited holes.

Strong polarization-dependent terahertz modulation of aligned Ag nanowires on Si substrate.

Optically tunable, strong polarization-dependent transmission of terahertz pulses through aligned Ag nanowires on a Si substrate is demonstrated. Terahertz pulses primarily pass through the Ag nanowires and the transmittance is weakly dependent on the angle between the direction of polarization of the terahertz pulse and the direction of nanowire alignment. However, the transmission of a terahertz pulse through optically excited materials strongly depends on the polarization direction. The extinction ratio increases as the power of the pumping laser increases. The enhanced polarization dependency is explained by the redistribution of photocarriers, which accelerates the sintering effect along the direction of alignment of the Ag nanowires. The photocarrier redistribution effect is examined by the enhancement of terahertz emission from the sample. Oblique metal nanowires on Si could be utilized for designing optically tunable terahertz polarization modulators.

High refractive index metamaterials using corrugated metallic slots.

We report on a method for realizing high refractive index metamaterials using corrugated metallic slot structures at terahertz frequencies. The effective refractive index and peak index frequency can be controlled by varying the width of the air gap in the corrugated slot arrays. The phenomenon occurs because of the secondary resonance effect due to the fundamental inductive-capacitive resonance, which generates a red-shift of the fundamental resonance determined by twice the length of the corrugated metallic slots. In addition, multiple gaps in the corrugated slots act as plasmonic hotspots which have the properties of three-dimensional subwavelength confinement due to extremely strong enhancement of the terahertz waves. The versatile characteristics of the structures may have many potential applications in designing compact optical devices incorporating various functionalities and in developing highly sensitive spectroscopic/imaging systems.

Evolution of the surface state in Bi2Se2Te thin films during phase transition.

Topological insulators, a new quantum state of matter, have created exciting opportunities for studies in topological quantum physics and for exploring spintronics applications due to their gapless helical metallic surface states. In this study, thin films composed of alternate layers of Bi and Se (Te) ({Bi(3 Å)Te(9 Å)}n/{Bi(3 Å)Se(9 Å)}n) were fabricated by controlling the layer thickness within the atomic scale using thermal evaporation techniques. The high-purity growth of uniform Bi2Se2Te1 thin films has not yet been achieved using a thermal evaporation method. However, as a result of a self-ordering process during annealing, an as-grown amorphous film with p-type polarity could transform into single crystalline Bi2Se2Te1 with n-type polarity. Using THz-time domain spectroscopy (THz-TDS) and ultraviolet photoemission spectroscopy (UPS), we concluded that the conductivity is dominated by the Drude contribution, suggesting the presence of a quantum well state and surface states. Moreover we demonstrated that the emission of terahertz waves from the (001) surface of the single crystalline Bi2Se2Te1 thin film would be possible under the excitation of 790 nm femtosecond optical pulses, indicating the presence of a Dirac-fermion, a photo-Dember effect at the surface state and the transient current within the surface depletion region. The results reported herein provide useful information regarding a valuable deposition method that can be useful in studies of the evolution of surface state electrons in topological insulators.

Fano resonance of self-collimated beams in two-dimensional photonic crystals.

We report that the Fano resonance of self-collimated beams can be achieved in a two-dimensional photonic crystal by introducing a Fano resonator that is composed of zigzag line defects. An asymmetric Fano line shape in a transmission spectrum is generated by the interference between radiated light beams from the resonator and self-collimated beams that directly pass through the resonator without resonance. It is shown that the Fano profile increases in sharpness as the number of zigzag line defects increases because the phase values of the radiated light beams change more rapidly when the number of defects increases. The Fano resonance of self-collimated beams could provide an efficient approach to manipulate light propagation and increase the possibility of application of self-collimated beams.

Monopole resonators in planar plasmonic metamaterials.

We first present a new phenomenon: the quarter-wavelength resonance of an electromagnetic field in planar plasmonic metamaterials consisting of asymmetrically coupled air-slot arrays, which is essential for a monopole resonator. The anti-nodal electric field intensity of the quarter-wavelength fundamental mode is formed by strong charge concentrations at the sharp metallic edges of the crossing position of the air-slots, and the nodal point of the electric field intensity naturally occurs at the other end of the air-slot. By tuning the structural asymmetry, the quarter-wavelength resonances were successfully split from the half-wavelength resonance, experimentally and numerically.

Propagation of spoof surface plasmon on metallic square lattice: bending and splitting of self-collimated beams.

The propagation characteristics of spoof surface plasmon modes are studied in both real and reciprocal spaces. From the metallic square lattice, we obtain constant frequency contours by directly measuring electric fields in the microwave frequency regime. The anisotropy of the measured constant frequency contour supports the presence of the negative refraction and the self-collimation which are confirmed from measured electric fields. Additionally, we demonstrate the spoof surface plasmon beam splitter in which the splitting ratio of the self-collimated beam is controlled by varying the height of rods.

Grating-induced omnidirectional refraction of self-collimated beams at a photonic crystal surface.

We report that self-collimated beams from a photonic crystal can be refracted to any direction in air by introducing an additional layer composed of dielectric rods at a photonic crystal surface. The refraction angle can be tuned from negative to positive value by adjusting the period of the additional layer. The refracted beam power can be also controllable by varying the radii of rods in the layer and the distance between the layer and the surface. The grating-induced omnidirectional refraction of self-collimated beams could provide an efficient way to manipulate light propagation and increase the possibility of application of self-collimated beams.

Resonant transmission of self-collimated beams through coupled zigzag-box resonators: slow self-collimated beams in a photonic crystal.

The resonant transmission of self-collimated beams through zigzag-box resonators is demonstrated experimentally and numerically. Numerical simulations show that the flat-wavefront and the width of the beam are well maintained after passing through zigzag-box resonators because the up and the down zigzag-sides prevent the beam from spreading out and the wavefront is perfectly reconstructed by the output zigzag-side of the resonator. Measured split resonant frequencies of two- and three-coupled zigzag-box resonators are well agreed with those predicted by a tight binding model to consider optical coupling between the nearest resonators. Slowing down the speed of self-collimated beams is also demonstrated by using a twelve-coupled zigzag-box resonator in simulations. Our work could be useful in implementing devices to manipulate self-collimated beams in time domain.

Terahertz band gaps induced by metal grooves inside parallel-plate waveguides.

We report experimental and finite-difference time-domain simulation studies on terahertz (THz) characteristics of band gaps by using metal grooves which are located inside the flare parallel-plate waveguide. The vertically localized standing-wave cavity mode (SWCM) between the upper waveguide surface and groove bottom, and the horizontally localized SWCM between two groove side walls (groove cavity) are observed. The E field intensity of the horizontally localized SWCM in grooves is very strongly enchanced which is three order higher than that of the input THz. The 4 band gaps except the Bragg band gap are caused by the π radian delay (out of phase) between the reflected THz field by grooves and the propagated THz field through the air gap. The measurement and simulation results agree well.