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1.
Adv Mater ; 33(25): e2008528, 2021 Jun.
Article in English | MEDLINE | ID: mdl-33988861

ABSTRACT

Correlated topological phases (CTPs) with interplay between topology and electronic correlations have attracted tremendous interest in condensed matter physics. Therein, correlated Weyl semimetals (WSMs) are rare in nature and, thus, have so far been less investigated experimentally. In particular, the experimental realization of the interacting WSM state with logarithmic Fermi velocity renormalization has not been achieved yet. Here, experimental evidence of a correlated magnetic WSM state with logarithmic renormalization in strained pyrochlore iridate Pr2 Ir2 O7 (PIO) which is a paramagnetic Luttinger semimetal in bulk, is reported. Benefitting from epitaxial strain, "bulk-absent" all-in-all-out antiferromagnetic ordering can be stabilized in PIO film, which breaks time-reversal symmetry and leads to a magnetic WSM state. With further analysis of the experimental data and renormalization group calculations, an interacting Weyl liquid state with logarithmically renormalized Fermi velocity, similar to that in graphene, is found, dressed by long-range Coulomb interactions. This work highlights the interplay of strain, magnetism, and topology with electronic correlations, and paves the way for strain-engineering of CTPs in pyrochlore iridates.

2.
J Environ Radioact ; 217: 106191, 2020 Jun.
Article in English | MEDLINE | ID: mdl-32063555

ABSTRACT

In March 2011, an earthquake caused the shutdown of the active reactors at the Fukushima Daiichi Nuclear Power Plant (NPP), with the succeeding tsunami resulting in the release of radioactively contaminated water into the adjacent Japanese coastal waters. Marine biota selected from various trophic levels were collected in Korean coastal waters throughout 2014 and 2015 and their plutonium levels were measured to evaluate the radioactive contamination levels in the marine organisms that constitute the primary seafood diet in the Republic of Korea (ROK). The results showed that the activity concentrations of 239,240Pu in plankton, macroalgae, mollusks, crustaceans, and cephalopods ranged from 13 to 58, 0.64 to 0.80, 0.94 to 5.40, 0.06 to 0.50, and 0.26 mBq kg-1 of wet weight (w.w.), respectively. The activity concentrations of 239,240Pu measured in the muscles of fish varied from 0.09 to 0.30 mBq kg-1 (w.w.), relatively low values compared to those in other groups regardless of fish species, size, and sampling area. The concentration characteristics of 239,240Pu in the various organs in the respective marine products revealed that the internal organs showed higher concentrations than the muscle or skin (or exoskeleton). The highest concentration of 239,240Pu was measured in the viscera of an abalone, which had an activity concentration of 6.31 mBq kg-1 (w.w.). The concentration factors (CFs) in the >300-µm fraction of plankton and in anchovy, shrimp, and mackerel ranged 67-84% of the International Atomic Energy Agency (IAEA)-recommended values, although the CF in macroalgae was much lower at approximately 5% of IAEA values, suggesting a wide range of 239,240Pu CF in macroalgae. The mean transfer factor (TF) between macroalgae (0.6-0.8 mBq kg-1) and abalone (5.4 mBq kg-1) was estimated to be 7.5, implying that effective Pu transfer occurred between the two species. These figures equate to annual effective doses of 239,240Pu to Koreans through consumption of macroalgae, shellfish, and fish of 1.8 × 10-6, 1.4 × 10-6, and 7.1 × 10-7 mSv yr-1, respectively, and a total dose of 3.9 × 10-6 mSv yr-1, values that are negligible compared to the annual effective dose limit of 1 mSv yr-1.


Subject(s)
Fukushima Nuclear Accident , Radiation Monitoring , Animals , Cesium Radioisotopes , Japan , Nuclear Power Plants , Oceans and Seas , Plutonium , Republic of Korea , Water Pollutants, Radioactive
3.
Small ; 11(35): 4526-31, 2015 Sep 16.
Article in English | MEDLINE | ID: mdl-26081390

ABSTRACT

Nanoscale patterning with massively parallel 2D array tips is of significant interest in scanning probe lithography. A challenging task for tip-based large area nanolithography is maintaining parallel tip arrays at the same contact point with a sample substrate in order to pattern a uniform array. Here, polymer pen lithography is demonstrated with a novel leveling method to account for the magnitude and direction of the total applied force of tip arrays by a multipoint force sensing structure integrated into the tip holder. This high-precision approach results in a 0.001° slope of feature edge length variation over 1 cm wide tip arrays. The position sensitive leveling operates in a fully automated manner and is applicable to recently developed scanning probe lithography techniques of various kinds which can enable "desktop nanofabrication."

4.
Nano Lett ; 15(5): 3364-9, 2015 May 13.
Article in English | MEDLINE | ID: mdl-25909996

ABSTRACT

The chemical vapor deposition (CVD) of molybdenum disulfide (MoS2) single-layer films onto periodically poled lithium niobate is possible while maintaining the substrate polarization pattern. The MoS2 growth exhibits a preference for the ferroelectric domains polarized "up" with respect to the surface so that the MoS2 film may be templated by the substrate ferroelectric polarization pattern without the need for further lithography. MoS2 monolayers preserve the surface polarization of the "up" domains, while slightly quenching the surface polarization on the "down" domains as revealed by piezoresponse force microscopy. Electrical transport measurements suggest changes in the dominant carrier for CVD MoS2 under application of an external voltage, depending on the domain orientation of the ferroelectric substrate. Such sensitivity to ferroelectric substrate polarization opens the possibility for ferroelectric nonvolatile gating of transition metal dichalcogenides in scalable devices fabricated free of exfoliation and transfer.

5.
J Cardiovasc Ultrasound ; 22(3): 148-50, 2014 Sep.
Article in English | MEDLINE | ID: mdl-25309693

ABSTRACT

The differential diagnosis of cardiac mass is important in determining the therapeutic plan and avoiding unnecessary surgical intervention. Non-invasive imaging methods would be useful in the diagnosis of suspected cardiac mass, because they may provide earlier diagnosis and more accurate assessment of cardiac mass. Native aortic valve thrombosis is a rare disorder and difficult to differentiate from a tumor, and in particular, a papillary fibroelastoma. Thus, the clinical decision making with imaging modalities should be performed cautiously. We recently met a female patient who had a aortic valve mass resembling papillary fibroelastoma in normal native valve. The patient underwent a surgical resection and the pathologic finding showed an organized thrombus with no evidence of papillary fibroelastoma.

6.
Nano Lett ; 12(11): 5539-44, 2012 Nov 14.
Article in English | MEDLINE | ID: mdl-22963681

ABSTRACT

We report the observation of layer-breathing mode (LBM) vibrations in few-layer graphene (FLG) samples of thickness from two to six layers, exhibiting both Bernal (AB) and rhombohedral (ABC) stacking order. The LBM vibrations are identified using a Raman combination band lying around 1720 cm(-1). From double resonance theory, we assign the feature as the LO+ZO' combination mode of the out-of-plane LBM (ZO') and the in-plane longitudinal optical mode (LO). The LOZO' Raman band is found to exhibit multiple peaks with a unique line shape for each layer thickness and stacking order. These complex line shapes of the LOZO'-mode arise both from the material-dependent selection of different phonons in the double-resonance Raman process and from the detailed structure of the different branches of LBM in FLG.

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