VERTICAL MIXING NEAR THE SEA SURFACE OBSERVED BY SHORT-LIVED NATURAL RADIONUCLIDES ( 214PB AND 214BI).

I performed continuous gamma-ray measurements in seawater to observe the temporal variation of radon progenies ( 214Pb and 214Bi) derived from atmospheric precipitation. Underwater gamma-ray measurements using two NaI(Tl) detectors at different installation depths (1 and 4 m) were recorded from July to November 2011 at the marine observation buoy. An increase in the concentration of 214Pb + 214Bi in seawater was observed due to precipitation when the wind velocity was <2 m s-1. However, this increase was only detected at 1 m depth and a downward spread of 214Pb + 214Bi was not observed. In contrast, at a wind velocity of >8 m s-1, the 214Pb + 214Bi concentration ratio at 4 m/1 m was almost constant (0.6-0.7) for most of the measurement irrespective of precipitation intensity. Assuming one-dimensional diffusion in the water column, the apparent vertical diffusion coefficient estimated from the temporal variation of 214Pb + 214Bi concentrations at 4 m/1 m varied from <10 to 500 cm2 s-1 depending on the wind velocity.

Preliminary investigation of 222Rn in the Yakumo Wind-hole, an algific talus deposits, from Izumo, southwest Honshu, Japan.

The Yakumo Wind-hole in southwest Japan formed by landslip, and it is known as a cold air blowhole. This wind-hole consists of two parts, which have complementary relationships in regard to the flow of air, namely, topographically upper and lower holes that can be characterized as a warm wind-hole (WWH) and cold wind-hole (CWH), respectively. We carried out a preliminary investigation of radon behavior in the Yakumo Wind-hole. The data showed remarkable seasonal change from high 222Rn concentrations reaching to 7.6 ±â€¯0.1 kBq/m3 in the warm season (mid-May to October) to low 222Rn concentrations in the cold season (December to early May) at the CWH. The threshold in the regional atmospheric temperature was estimated as 16.2 °C for the beginning and 17.1 °C for the ending periods of air blow with higher 222Rn concentrations. These seasonal changes in 222Rn were not only associated with the dynamic convection caused by temperature differences in and out of the talus, but were also related to the relative humidity of air that is blown out. High 222Rn concentrations were formed in the high humidity environment, and the humidity may possibly be associated with melting ice. According to the known information on 222Rn behavior in relation to humidity, a radon trap in the growing ice in spring and in the melted water in summer are suggested. This study revealed that 222Rn measurements are a useful tool to understand the air dynamics in the talus.

Vertical profiles of Fukushima Dai-ichi NPP-derived radiocesium concentrations in the waters of the southwestern Okhotsk Sea (2011-2017).

We examined the vertical 134Cs and 137Cs concentration profiles in the southwestern Okhotsk Sea in 2011, 2013, and 2017. In June 2011, atmospheric deposition-derived 134Cs from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) was detected at depths of 0-200 m (0.06-0.6 mBq/L). In July 2013, 134Cs detected at depths of 100-200 m (∼0.05 mBq/L) was ascribed to the transport of low-level 134Cs-contaminated water and/or the convection of radioactive depositions (<0.03 mBq/L at depths of 0-50 m). In July 2017, 134Cs was detected in water samples at depths above 300 m (0.03-0.05 mBq/L), and the inventory, decay-corrected to the FDNPP accident date, exhibited its maximum value (85 Bq/m2) during this period. Combining temperature-salinity data with the concentrations of global fallout-derived 137Cs led to a plausible explanation for this observation, which is a consequence of re-entry of FDNPP-derived radiocesium through the Kuril Strait from the northwestern North Pacific Ocean to the Okhotsk Sea and subsequent mixing with the south Okhotsk subsurface layer until 2017.

Temporal variations in (134)Cs and (137)Cs concentrations in seawater along the Shimokita Peninsula and the northern Sanriku coast in northeastern Japan, one year after the Fukushima Dai-ichi Nuclear Power Plant accident.

Ninety-six seawater samples were collected between May 2011 and March 2012 at 6 sites along the Shimokita Peninsula and the northern Sanriku coast, 250-450 km north of the Fukushima Dai-ichi Nuclear Power Plant (FDNPP). Cesium-134 and (137)Cs concentrations were determined by low-background γ-spectrometry. During May-June 2011, (134)Cs and (137)Cs concentrations in surface waters decreased from 1.0-2.8 to 0.7-1.5 mBq/L and from 2.1-3.9 to 1.9-3.0 mBq/L, respectively. These decreases were due to diffusion and advection in the ocean after atmospheric input of the FDNPP-derived radionuclides. However, in July-August 2011, the concentrations of both radionuclides in the water samples collected on the Pacific side of the Shimokita Peninsula and the northern Sanriku coast exhibited 30-50-fold increases (∼40 mBq/L for (134)Cs and ∼50 mBq/L for (137)Cs) over concentrations observed at these sampling sites in June 2011 in contrast to the gradual decreases in the concentrations on the Tsugaru Strait side of the Shimokita Peninsula. These results suggest that radiocesium-contaminated waters offshore in the Pacific Ocean were transported to coastal regions along the Pacific side of the Shimokita Peninsula and the northern Sanriku coast by ocean currents.

Opening of the closed water area and consequent changes of ²²8Ra/²²6Ra activity ratios in coastal lagoon Nakaumi, southwest Japan.

In Lake Nakaumi, the second largest coastal lagoon in Japan, artificially closed (Honjyo) area, which was left untouched for 28 years, was partly opened in May, 2009. (228)Ra/(226)Ra ratio of waters in Honjyo area and Lake Nakaumi showed a well-tuned seasonal variation exhibiting high value in summer. After the opening event, however, the (228)Ra/(226)Ra ratios in the Honjyo water showed an unclear seasonal variation in both surface and deep water. This opening event caused the change of active movement of lake and marine water.

Spatial variations of low levels of ¹³4Cs and ¹³7Cs in seawaters within the Sea of Japan after the Fukushima Dai-ichi Nuclear Power Plant accident.

Our method based on low background γ-spectrometry enabled the measurement of low radiocesium concentrations in only 20 L of seawater. In May 2011 after deposition of radiocesium, (134)Cs concentration in surface water within the Sea of Japan was confirmed to be significantly small (<0.1-1 mBq/L) by the method. The concentration was not detected (<0.1 mBq/L) below 50 m depth. The Fukushima-derived radiocesium migrated from the surface water of the Sea of Japan without advection to below the thermocline.

Spatial variations of 226Ra, 228Ra, 137Cs, and 228Th activities in the southwestern Okhotsk Sea.

We collected 14 water column seawater samples in the southwestern Okhotsk Sea and 7 surface samples around the northern area of Hokkaido Island, Northern Japan, and employed low-background γ-spectrometry with convenient minimal radiochemical processing to determine the activities of (226)Ra (half-life t(1/2)=1600 y), (228)Ra (5.75 y), (137)Cs (30.2 y), and (228)Th (1.91 y) in the samples. Activities of (226)Ra (~2.3 mBq/L), (228)Ra (~0.7 mBq/L), and (137)Cs (~1 mBq/L) of surface waters on the Okhotsk Sea side show notable differences from those on the Japan Sea side (Soya Warm Current Water; SWCW) (~1.5 mBq/L; 1.5-2 mBq/L; 1.4-1.6 mBq/L), indicating their different origins and lateral mixing patterns. All of these nuclides exhibit unique vertical profiles; activities of soluble (226)Ra, (228)Ra, (137)Cs, and reactive (228)Th exhibit small variations from 50 to 500 m depth ((226)Ra, ~2.2 mBq/L; (228)Ra, ~0.4 mBq/L; (137)Cs, ~1 mBq/L; (228)Th, ~0.13 mBq/L). These profiles can be explained by the convective mixing of surface water such as the East Sakhalin Current Water (ESCW) to this layer.