ABSTRACT
The evolution of the magnetic excitation spectrum of the heavy fermion superconductor PrOs(4)Sb(12) was studied by inelastic neutron scattering on crossing the critical field H(c2) for superconductivity at low temperature. The peak positions in energy and the peak intensities of the modes of the triplet split by magnetic field confirm the known crystal field parameters for PrOs(4)Sb(12) in T(h) symmetry. A selective broadening of the lineshape occurs on increasing the magnetic field: the linewidth of the upper mode of the triplet increases while the one of the middle mode does not.
ABSTRACT
We report inelastic neutron scattering experiments performed to investigate the low energy magnetic excitations on single crystals of the heavy-fermion superconductor PrOs(4)Sb(12). The observed excitation clearly softens at a wave vector Q=(1,0,0), which is the same as the modulation vector of the field-induced antiferro-quadrupolar ordering, and its intensity at Q=(1,0,0) is smaller than that around the zone center. This result directly evidences that this excitonic behavior is derived mainly from nonmagnetic quadrupolar interactions. Furthermore, the narrowing of the linewidths of the excitations below the superconducting transition temperature indicates the close connection between the superconductivity and the excitons.
ABSTRACT
The magnetic structure of the localized-5f uranium intermetallic compound U3Pd20Si6 has been determined by means of a neutron diffraction experiment. Our data demonstrate that this compound has a collinear coupling of the sublattice ordering of the uranium spins on the 4a and 8c sites. We conclude that higher-order exchange and/or quadrupole interactions are necessary to stabilize this unique collinear structure. We discovered a new type of spin-flop transition against the uniaxial anisotropy induced by this collinear coupling.
ABSTRACT
Inelastic neutron scattering measurements of magnetic excitations in the charge-ordered state of Yb4As3 have been performed under magnetic field up to about 6 T. By applying a magnetic field, the spectrum at the one-dimensional wave vector q = 1 [ pi/d] changes drastically from a broad one corresponding to the spinon excitation continuum of the one-dimensional S = 1 / 2 spin system to a sharp one at a finite energy, indicating the opening of an energy gap in the system. The magnetic field dependence of the gap is well fitted by the power law H2/3. The experimental result gives strong evidence for the existence of a staggered field alternating along Yb3+ chains induced by the Dzyaloshinsky-Moriya interaction.
