High purcell factor due to coupling of a single emitter to a dielectric slot waveguide.

We demonstrate an all-dielectric quantum electrodynamical nanowire-slab system with a single emitter that concentrates the extremely intense light at the scale of 10 × 75 nm(2). The quantum dot exhibits a record high 31-fold spontaneous decay rate enhancement, its optical saturation and blinking are strongly suppressed, and 80% of emission couples into a waveguide mode.

Strongly enhanced molecular fluorescence inside a nanoscale waveguide gap.

We experimentally demonstrate dramatically enhanced light-matter interaction for molecules placed inside the nanometer scale gap of a plasmonic waveguide. We observe spontaneous emission rate enhancements of up to about 60 times due to strong optical localization in two dimensions. This rate enhancement is a nonresonant nature of the plasmonic waveguide under study overcoming the fundamental bandwidth limitation of conventional devices. Moreover, we show that about 85% of molecular emission couples into the waveguide highlighting the dominance of the nanoscale optical mode in competing with quenching processes. Such optics at molecular length scales paves the way toward integrated on-chip photon source, rapid transfer of quantum information, and efficient light extraction for solid-state-lighting devices.

Nonlinear quantum optics in a waveguide: distinct single photons strongly interacting at the single atom level.

We propose a waveguide-QED system where two single photons of distinct frequency or polarization interact strongly. The system consists of a single ladder-type three level atom coupled to a waveguide. When both optical transitions are coupled strongly to the waveguide's mode, we show that a control photon tuned to the upper transition induces a π phase shift and tunneling of a probe photon tuned to the otherwise reflective lower transition. Furthermore, the system exhibits single photon scattering by a classical control beam. Waveguide-QED schemes could be an alternative to high quality cavities or dense atomic ensembles in quantum information processing.

Electro-optic modulation of single photons.

We use the Stokes photon of a biphoton pair to set the time origin for electro-optic modulation of the wave function of the anti-Stokes photon thereby allowing arbitrary phase and amplitude modulation. We demonstrate conditional single-photon wave functions composed of several pulses, or instead, having Gaussian or exponential shapes.

Observation of optical precursors at the biphoton level.

We describe the observation of a sharp leading-edge spike in a biphoton wave packet that is produced using slow light and measured by two-photon correlation. Using the stationary-phase approximation we characterize this spike as a Sommerfeld-Brillouin precursor resulting from the interference of low- and high-frequency spectral components.

Subnatural linewidth biphotons with controllable temporal length.

This Letter describes the generation of biphotons with a temporal length that can be varied over the range of 50-900 ns, with an estimated subnatural linewidth as small as 0.75 MHz. We make use of electromagnetically induced transparency and slow light in a two-dimensional magneto-optical trap with an optical depth as high as 62. We report a sharp leading edge spike that is a Sommerfeld-Brillouin precursor, as observed at the biphoton level.

Generation of narrow-bandwidth paired photons: use of a single driving laser.

We describe a generator of narrow-band paired photons. A single retroreflected Ti:sapphire laser is used to cool, render transparent, and parametrically pump a cloud of (87)Rb atoms. We attain a paired-photon generation rate into opposing fibers of 600 counts/s with an intensity correlation function that has a width of 5 ns, and violates the Cauchy-Schwartz criteria by a factor of 2000.

Generation of paired photons with controllable waveforms.

We describe experiments and theory showing the generation of counterpropagating paired photons with coherence times of about 50 ns and waveforms that are controllable at a rudimentary level. Using cw lasers, electromagnetically induced transparency and cold 87Rb atoms we generate paired photons into opposing single-mode optical fibers at a rate of approximately 12 000 pairs per second.