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1.
Adv Mater ; 28(17): 3406-10, 2016 05.
Article in English | MEDLINE | ID: mdl-26932458

ABSTRACT

The density of trap states within the bandgap of methylammonium lead iodide single crystals is investigated. Defect states close to both the conduction and valence bands are probed. Additionally, a comprehensive electronic characterization of crystals is carried out, including measurements of the electron and hole mobility, and the energy landscape (band diagram) at the surface.

2.
Adv Mater ; 27(1): 116-21, 2015 Jan 07.
Article in English | MEDLINE | ID: mdl-25382752

ABSTRACT

A colloidal quantum dot solar cell is fabricated by spray-coating under ambient conditions. By developing a room-temperature spray-coating technique and implementing a fully automated process with near monolayer control-an approach termed as sprayLD-an electronic defect is eliminated resulting in solar cell performance and statistical distribution superior to prior batch-processed methods along with a hero performance of 8.1%.


Subject(s)
Colloids/chemistry , Electric Power Supplies , Quantum Dots/chemistry , Solar Energy , Automation/methods , Elastic Modulus , Equipment Design , Microscopy, Atomic Force , Microscopy, Electron, Scanning , Microscopy, Electron, Transmission , Nebulizers and Vaporizers , Spectroscopy, Electron Energy-Loss , Surface Properties , Temperature
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