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1.
J Vis Exp ; (68)2012 Oct 09.
Article in English | MEDLINE | ID: mdl-23093178

ABSTRACT

The physical properties of a material are defined by its electronic structure. Electrons in solids are characterized by energy (ω) and momentum (k) and the probability to find them in a particular state with given ω and k is described by the spectral function A(k, ω). This function can be directly measured in an experiment based on the well-known photoelectric effect, for the explanation of which Albert Einstein received the Nobel Prize back in 1921. In the photoelectric effect the light shone on a surface ejects electrons from the material. According to Einstein, energy conservation allows one to determine the energy of an electron inside the sample, provided the energy of the light photon and kinetic energy of the outgoing photoelectron are known. Momentum conservation makes it also possible to estimate k relating it to the momentum of the photoelectron by measuring the angle at which the photoelectron left the surface. The modern version of this technique is called Angle-Resolved Photoemission Spectroscopy (ARPES) and exploits both conservation laws in order to determine the electronic structure, i.e. energy and momentum of electrons inside the solid. In order to resolve the details crucial for understanding the topical problems of condensed matter physics, three quantities need to be minimized: uncertainty* in photon energy, uncertainty in kinetic energy of photoelectrons and temperature of the sample. In our approach we combine three recent achievements in the field of synchrotron radiation, surface science and cryogenics. We use synchrotron radiation with tunable photon energy contributing an uncertainty of the order of 1 meV, an electron energy analyzer which detects the kinetic energies with a precision of the order of 1 meV and a He(3) cryostat which allows us to keep the temperature of the sample below 1 K. We discuss the exemplary results obtained on single crystals of Sr2RuO4 and some other materials. The electronic structure of this material can be determined with an unprecedented clarity.


Subject(s)
Photoelectron Spectroscopy/instrumentation , Photoelectron Spectroscopy/methods , Cold Temperature , Ruthenium Compounds/chemistry , Strontium/chemistry
2.
Nature ; 431(7004): 1 p following 39, 2004 Sep 02.
Article in English | MEDLINE | ID: mdl-15346602

ABSTRACT

One of the mysteries of modern condensed-matter physics is the nature of the pseudogap state of the superconducting cuprates. Kaminski et al. claim to have observed signatures of time-reversal symmetry breaking in the pseudogap regime in underdoped Bi2Sr2CaCu2O8+delta (Bi2212). Here we argue that the observed circular dichroism is due to the 51 superstructure replica of the electronic bands and therefore cannot be considered as evidence for spontaneous time-reversal symmetry breaking in cuprates.

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