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1.
Phys Rev E ; 104(1-1): 014133, 2021 Jul.
Article in English | MEDLINE | ID: mdl-34412266

ABSTRACT

We consider the motion of a Brownian particle in a sawtooth potential dichotomously modulated by a spatially harmonic perturbation. An explicit expression for the Laplace transform of the Green function of an extremely asymmetric sawtooth potential is obtained. With this result, within the approximation of small potential-energy fluctuations, the integration of the relations for the average particle velocity is performed in elementary terms. The obtained analytical result, its high-temperature, low-frequency, and high-frequency asymptotics, as well as numerical calculations performed for a sawtooth potential of an arbitrary symmetry, indicate that in such a system, the frequency-temperature controlling the magnitude and direction of the ratchet velocity becomes possible. We clarify the mechanism of the appearance of additional regions of nonmonotonicity in the frequency dependence of the average velocity, which leads to the appearance of additional ratchet stopping points. This mechanism is a consequence of the competition between the sliding time along the steep slope of the highly asymmetric sawtooth potential and the correlation time of the dichotomous noise.

2.
Phys Rev E Stat Nonlin Soft Matter Phys ; 83(5 Pt 1): 051120, 2011 May.
Article in English | MEDLINE | ID: mdl-21728503

ABSTRACT

A Brownian motor is considered which operates due to asymmetric dichotomic fluctuations of the spatially periodic asymmetric potential energy. As shown, the motion direction and stopping points of this motor are dictated by the competition between the spatial and temporal asymmetry of the potential energy (or solely by temporal asymmetry in the case that the potential energy sign fluctuates). For an asymmetric sawtooth potential, the Brownian-particle average velocity is calculated numerically as a function of certain parameters of the model, whereas the low-frequency and low-energy approximations allow the corresponding analytical relationships to be derived for an arbitrarily shaped potential profile. It is shown that temporal asymmetry is not necessary for stopping point occurrence provided that the potential profile fluctuates not only in amplitude but in shape as well. This inference is illustrated by photoinduced fluctuations of the potential energy for a number of substituted arylpyrene molecules on a substrate with symmetrically distributed charge density.

3.
Phys Rev E Stat Nonlin Soft Matter Phys ; 77(6 Pt 1): 061111, 2008 Jun.
Article in English | MEDLINE | ID: mdl-18643221

ABSTRACT

The study addresses the azimuthal jumping motion of an adsorbed polar molecule in a periodic n -well potential under the action of an external alternating electric field. Starting from the perturbation theory of the Pauli equation with respect to the weak field intensity, explicit analytical expressions have been derived for the time dependence of the average dipole moment as well as the frequency dependences of polarizability and the average angular velocity, the three quantities exhibiting conspicuous stochastic resonance. As shown, unidirectional rotation can arise only provided simultaneous modulation of the minima and maxima of the potential by an external alternating field. For a symmetric potential of hindered rotation, the average angular velocity, if calculated by the second-order perturbation theory with respect to the field intensity, has a nonzero value only at n=2 , i.e., when two azimuthal wells specify a selected axis in the system. Particular consideration is given to the effect caused by the asymmetry of the two-well potential on the dielectric loss spectrum and other Brownian motion parameters. When the asymmetric potential in a system of dipole rotators arises from the average local fields induced by an orientational phase transition, the characteristics concerned show certain peculiarities which enable detection of the phase transition and determination of its parameters.

4.
Phys Rev E Stat Nonlin Soft Matter Phys ; 75(6 Pt 1): 061115, 2007 Jun.
Article in English | MEDLINE | ID: mdl-17677228

ABSTRACT

We consider two basic types of Brownian motors which generate directed motion in a periodic asymmetric piecewise-linear potential as a result of random half-period shifts of the potential relief (flashing ratchets) or due to a temporally asymmetric unbiased force applied to the system (rocking ratchets). Analytical relationships have been derived which enable the comparison of the upper limits for the conventional and generalized energy conversion efficiencies in these motors. As found, the increasing amplitude of a sawtooth potential (or the decreasing temperature) makes the conventional efficiency tend to the unity limit faster for a rocking ratchet (in the absence of temporal asymmetry) than for a flashing ratchet. The inverse is true for the generalized efficiency. The potential amplitude being the same, the generalized efficiency is always less than the conventional efficiency. A decreased asymmetry of the potential always results in the reduction of both efficiencies. The temporal asymmetry of an unbiased force has an opposite effect on the conventional and generalized efficiencies: the former rises and the latter drops as the positive signal component becomes shorter in time and larger in amplitude.

5.
Phys Rev E Stat Nonlin Soft Matter Phys ; 71(4 Pt 1): 041102, 2005 Apr.
Article in English | MEDLINE | ID: mdl-15903652

ABSTRACT

For a flashing ratchet with periodic potentials fluctuating via random shifts of one-half period, a high efficiency is shown to result from two mechanisms. The previously reported one [Yu. A. Makhnovskii, Phys. Rev. E 69, 021102 (2004); V. M. Rozenbaum, JETP Lett. 79, 388 (2004)] is realized in the near-equilibrium region and implies, first, the presence of a high barrier V0 blocking the reverse movement of a Brownian particle and, second, identical, though energy-shifted, portions of the asymmetric flat potential profile on both half periods. We report another mechanism acting far from equilibrium, typical of strongly asymmetric potentials which are shaped identically on both half periods with a large energetic shift DeltaV . The two mechanisms exhibit radically different limiting behavior of the maximum possible efficiency: eta(m) approximately 1-exp (-beta V0 /2) for the former and eta(m) approximately 1-ln (2betaDeltaV) /betaDeltaV for the latter ( beta being the reciprocal temperature in energy units). The flux and the efficiency for a Brownian motor with a piecewise-linear potential are calculated using the transfer matrix method; an exact analytical solution can thus be obtained for an extremely asymmetric sawtooth potential, the simplest example of the second high-efficiency mechanism. As demonstrated, the mechanisms considered are also characteristic of a two-well periodic potential treated in terms of the kinetic approach.


Subject(s)
Biological Clocks/physiology , Models, Biological , Models, Chemical , Molecular Motor Proteins/chemistry , Molecular Motor Proteins/physiology , Movement/physiology , Algorithms , Computer Simulation , Energy Transfer/physiology , Stress, Mechanical
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