Energy transfer driven brightening of MoS2 by ultrafast polariton relaxation in microcavity MoS2/hBN/WS2 heterostructures.

Energy transfer is a ubiquitous phenomenon that delivers energy from a blue-shifted emitter to a red-shifted absorber, facilitating wide photonic applications. Two-dimensional (2D) semiconductors provide unique opportunities for exploring novel energy transfer mechanisms in the atomic-scale limit. Herein, we have designed a planar optical microcavity-confined MoS2/hBN/WS2 heterojunction, which realizes the strong coupling among donor exciton, acceptor exciton, and cavity photon mode. This configuration demonstrates an unconventional energy transfer via polariton relaxation, brightening MoS2 with a record-high enhancement factor of ~440, i.e., two-order-of-magnitude higher than the data reported to date. The polariton relaxation features a short characteristic time of ~1.3 ps, resulting from the significantly enhanced intra- and inter-branch exciton-exciton scattering. The polariton relaxation dynamics is associated with Rabi energies in a phase diagram by combining experimental and theoretical results. This study opens a new direction of microcavity 2D semiconductor heterojunctions for high-brightness polaritonic light sources and ultrafast polariton carrier dynamics.

Limit cycles and chaos in the hybrid atom-optomechanics system.

We consider atoms in two different periodic potentials induced by different lasers, one of which is coupled to a mechanical membrane via radiation pressure force. The atoms are intrinsically two-level systems that can absorb or emit photons, but the dynamics of their position and momentum are treated classically. On the other hand, the membrane, the cavity field, and the intrinsic two-level atoms are treated quantum mechanically. We show that the mean excitation of the three systems can be stable, periodically oscillating, or in a chaotic state depending on the strength of the coupling between them. We define regular, limit cycle, and chaotic phases, and present a phase diagram where the three phases can be achieved by manipulating the field-membrane and field-atom coupling strengths. We also computed other observable quantities that can reflect the system's phase such as position, momentum, and correlation functions. Our proposal offers a new way to generate and tune the limit cycle and chaotic phases in a well-established atom-optomechanics system.

Electric Field Modulation of 2D Perovskite Excitonics.

Multiquantum-well (MQW) perovskite is one of the forerunners in high-efficiency perovskite LED (PeLEDs) research. Despite the rapid inroads, PeLEDs suffer from the pertinent issue of efficiency decrease with increasing brightness, commonly known as "efficiency roll-off". The underlying mechanisms are presently an open question. Herein, we explicate the E-field effects on the exciton states in the archetypal MQW perovskite (C6H5C2H4NH3)2PbI4, or PEPI, in a device-like architecture using field-assisted transient spectroscopy and theoretical modeling. The applied E-field results in a complex interplay of spectral blueshifts and enhancement/quenching of the different exciton modes. The former originates from the DC Stark shift, while the latter is attributed to the E-field modulation of the transfer rates between bright/dark exciton modes. Importantly, our findings uncover crucial insights into the photophysical processes under E-field modulation contributing to efficiency roll-off in MQW PeLEDs. Electrical modulation of exciton properties presents exciting possibilities for signal processing devices.

Creating and concentrating quantum resource states in noisy environments using a quantum neural network.

Quantum information processing tasks require exotic quantum states as a prerequisite. They are usually prepared with many different methods tailored to the specific resource state. Here we provide a versatile unified state preparation scheme based on a driven quantum network composed of randomly-coupled fermionic nodes. The output of such a system is then superposed with the help of linear mixing where weights and phases are trained in order to obtain desired output quantum states. We explicitly show that our method is robust and can be utilized to create almost perfect maximally entangled, NOON, W, cluster, and discorded states. Furthermore, the treatment includes energy decay in the system as well as dephasing and depolarization. Under these noisy conditions we show that the target states are achieved with high fidelity by tuning controllable parameters and providing sufficient strength to the driving of the quantum network. Finally, in very noisy systems, where noise is comparable to the driving strength, we show how to concentrate entanglement by mixing more states in a larger network.

Revealing Nonclassicality of Inaccessible Objects.

Some physical objects are hardly accessible to direct experimentation. It is then desirable to infer their properties based solely on the interactions they have with systems over which we have control. In this spirit, here we introduce schemes for assessing the nonclassicality of the inaccessible objects as characterized by quantum discord. We consider two probes individually interacting with the inaccessible object but not with each other. The schemes are based on monitoring entanglement dynamics between the probes. Our method is robust and experimentally friendly, as it allows the probes and the object to be open systems and makes no assumptions about the initial state, dimensionality of involved Hilbert spaces, and details of the probe-object Hamiltonian. We apply our scheme to a membrane-in-the-middle optomechanical system, to detect system-environment correlations in open system dynamics as well as nonclassicality of the environment, and we foresee potential benefits for the inference of the nonclassical nature of gravity.