Quantum Dot Photoluminescence Enhancement in GaAs Nanopillar Oligomers Driven by Collective Magnetic Modes.

Single photon sources based on semiconductor quantum dots are one of the most prospective elements for optical quantum computing and cryptography. Such systems are often based on Bragg resonators, which provide several ways to control the emission of quantum dots. However, the fabrication of periodic structures with many thin layers is difficult. On the other hand, the coupling of single-photon sources with resonant nanoclusters made of high-index dielectric materials is known as a promising way for emission control. Our experiments and calculations show that the excitation of magnetic Mie-type resonance by linearly polarized light in a GaAs nanopillar oligomer with embedded InAs quantum dots leads to quantum emitters absorption efficiency enhancement. Moreover, the nanoresonator at the wavelength of magnetic dipole resonance also acts as a nanoantenna for a generated signal, allowing control over its radiation spatial profile. We experimentally demonstrated an order of magnitude emission enhancement and numerically reached forty times gain in comparison with unstructured film. These findings highlight the potential of quantum dots coupling with Mie-resonant oligomers collective modes for nanoscale single-photon sources development.

Toward Perfect Optical Diffusers: Dielectric Huygens' Metasurfaces with Critical Positional Disorder.

Conventional optical diffusers, such as thick volume scatterers (Rayleigh scattering) or microstructured surface scatterers (geometric scattering), lack the potential for on-chip integration and are thus incompatible with next-generation photonic devices. Dielectric Huygens' metasurfaces, on the other hand, consist of 2D arrangements of resonant dielectric nanoparticles and therefore constitute a promising material platform for ultrathin and highly efficient photonic devices. When the nanoparticles are arranged in a random but statistically specific fashion, diffusers with exceptional properties are expected to come within reach. This work explores how dielectric Huygens' metasurfaces can implement wavelength-selective diffusers with negligible absorption losses and nearly Lambertian scattering profiles that are largely independent of the angle and polarization of incident waves. The combination of tailored positional disorder with a carefully balanced electric and magnetic response of the nanoparticles is shown to be an integral requirement for the operation as a diffuser. The proposed metasurfaces' directional scattering performance is characterized both experimentally and numerically, and their usability in wavefront-shaping applications is highlighted. Since the metasurfaces operate on the principles of Mie scattering and are embedded in a glassy environment, they may easily be incorporated in integrated photonic devices, fiber optics, or mechanically robust augmented reality displays.

Enhanced Nonlinear Light Generation in Oligomers of Silicon Nanoparticles under Vector Beam Illumination.

All-dielectric nanoparticle oligomers have recently emerged as promising candidates for nonlinear optical applications. Their highly resonant collective modes, however, are difficult to access by linearly polarized beams due to symmetry restraints. In this paper, we propose a new way to increase the efficiency of nonlinear processes in all-dielectric oligomers by tightly focused azimuthally polarized cylindrical vector beam illumination. We demonstrate two orders enhancement of the third-harmonic generation signal, governed by a collective optical mode represented by out-of-plane magnetic dipoles. Crucially, the collective mode is characterized by strong electromagnetic field localization in the bulk of the nonlinear material. For comparison, we measure third-harmonic generation in the same oligomer pumped with linearly and radially polarized fundamental beams, which both show significantly lower harmonic output. We also provide numerical analysis to describe and characterize the observed effect. Our findings open a new route to enhance and modulate the third-harmonic generation efficiency of Mie-resonant isolated nanostructures by tailoring the polarization of the pump beam.