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1.
Nano Lett ; 13(12): 5797-802, 2013.
Article in English | MEDLINE | ID: mdl-24228733

ABSTRACT

The recent focus on topological insulators is due to the scientific interest in the new state of quantum matter as well as the technology potential for a new generation of THz optoelectronics, spintronics and quantum computations. It is important to elucidate the dynamics of the Dirac fermions in the topologically protected surface state. Hence we utilized a novel ultrafast optical pump mid-infrared probe to explore the dynamics of Dirac fermions near the Dirac point. The femtosecond snapshots of the relaxation process were revealed by the ultrafast optics. Specifically, the Dirac fermion-phonon coupling strength in the Dirac cone was found to increase from 0.08 to 0.19 while Dirac fermions were away from the Dirac point into higher energy states. Further, the energy-resolved transient reflectivity spectra disclosed the energy loss rate of Dirac fermions at room temperature was about 1 meV/ps. These results are crucial to the design of Dirac fermion devices.


Subject(s)
Nanostructures/chemistry , Nanotechnology , Optics and Photonics , Quantum Theory , Semiconductors , Spectrophotometry, Infrared
2.
Opt Express ; 21(12): 13930-7, 2013 Jun 17.
Article in English | MEDLINE | ID: mdl-23787582

ABSTRACT

This study systematically investigates the influence of free carriers on the generation of THz in ZnTe crystals, over a wide range of pumping fluences. As the pumping fluence is increased (< 6.36 mJ/cm(2)), the concentration of free carriers gradually increases and the THz output power is saturated, as clearly demonstrated by the time delay in the THz temporal waveforms, the changes in the THz spectral weight and the red-shift in the PL spectra. For high pumping fluences (> 6.36 mJ/cm(2)), spectacularly, there is a significant quadratic increase in the THz output power when the pumping fluence is increased, as well as at low pumping fluences of < 0.58 mJ/cm(2), because of the saturation of free carriers.


Subject(s)
Tellurium/chemistry , Tellurium/radiation effects , Zinc/chemistry , Zinc/radiation effects , Crystallization , Electron Transport , Materials Testing , Scattering, Radiation , Terahertz Radiation
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