High-efficiency single-photon generation via large-scale active time multiplexing.

Deterministic generation of single- and multiphoton states is a key requirement for large-scale optical quantum information and communication applications. While heralded single-photon sources (HSPSs) using nonlinear optical processes have enabled proof-of-principle demonstrations in this area of research, they are not scalable as their probabilistic nature severely limits their generation efficiency. We overcome this limitation by demonstrating a substantial improvement in HSPS efficiency via large-scale time multiplexing. Using an ultra-low loss, adjustable optical delay to multiplex 40 conventional HSPS photon generation processes into each operation cycle, we have observed a factor of 9.7(5) enhancement in efficiency, yielding a 66.7(24)% probability of collecting a single photon with high indistinguishability (90%) into a single-mode fiber per cycle. We also experimentally investigate the trade-off between a high single-photon probability and unwanted multiphoton emission. Upgrading our time-multiplexed source with state-of-the-art HSPS and single-photon detector technologies will enable the generation of >30 coincident photons with unprecedented efficiency.

Detection-loophole-free test of quantum nonlocality, and applications.

We present a source of entangled photons that violates a Bell inequality free of the "fair-sampling" assumption, by over 7 standard deviations. This violation is the first reported experiment with photons to close the detection loophole, and we demonstrate enough "efficiency" overhead to eventually perform a fully loophole-free test of local realism. The entanglement quality is verified by maximally violating additional Bell tests, testing the upper limit of quantum correlations. Finally, we use the source to generate "device-independent" private quantum random numbers at rates over 4 orders of magnitude beyond previous experiments.

Hyperentanglement-enabled direct characterization of quantum dynamics.

We use hyperentangled photons to experimentally implement an entanglement-assisted quantum process tomography technique known as direct characterization of quantum dynamics. Specifically, hyperentanglement-assisted Bell-state analysis enabled us to characterize a variety of single-qubit quantum processes using far fewer experimental configurations than are required by standard quantum process tomography. Furthermore, we demonstrate how known errors in Bell-state measurement may be compensated for in the data analysis. Using these techniques, we have obtained single-qubit process fidelities over 98% but with one-third the number of experimental configurations required for standard quantum process tomography. Extensions of these techniques to multiqubit quantum processes are discussed.

Experimental methods for detecting entanglement.

Here we present experimental realizations of two new entanglement detection methods: a three-measurement Bell inequality inequivalent to the Clauser-Horne-Shimony-Holt inequality and a nonlinear Bell-type inequality based on the negativity measure. In addition, we provide an experimental and theoretical comparison between these new methods and several techniques already in use: the traditional Clauser-Horne-Shimony-Holt inequality, the entanglement witness, and complete state tomography.

Experimental investigation of a two-qubit decoherence-free subspace.

We thoroughly explore the phenomenon of a decoherence-free subspace (DFS) for two-qubit systems. Specifically, we both collectively and noncollectively decohere entangled polarization-encoded two-qubit states using thick birefringent crystals. These results characterize the basis-dependent effect of decoherence on the four Bell states, the robustness of the DFS state against perturbations in the assumption of collective decoherence, and the existence of a DFS for each type of stable noncollective decoherence. Finally, we investigate the effects of collective and noncollective dissipation.

Ancilla-assisted quantum process tomography.

Complete and precise characterization of a quantum dynamical process can be achieved via the method of quantum process tomography. Using a source of correlated photons, we have implemented several methods, each investigating a wide range of processes, e.g., unitary, decohering, and polarizing. One of these methods, ancilla-assisted process tomography (AAPT), makes use of an additional "ancilla system," and we have theoretically determined the conditions when AAPT is possible. Surprisingly, entanglement is not required. We present data obtained using both separable and entangled input states. The use of entanglement yields superior results, however.

Experimental entanglement distillation and 'hidden' non-locality.

Entangled states are central to quantum information processing, including quantum teleportation, efficient quantum computation and quantum cryptography. In general, these applications work best with pure, maximally entangled quantum states. However, owing to dissipation and decoherence, practically available states are likely to be non-maximally entangled, partially mixed (that is, not pure), or both. To counter this problem, various schemes of entanglement distillation, state purification and concentration have been proposed. Here we demonstrate experimentally the distillation of maximally entangled states from non-maximally entangled inputs. Using partial polarizers, we perform a filtering process to maximize the entanglement of pure polarization-entangled photon pairs generated by spontaneous parametric down-conversion. We have also applied our methods to initial states that are partially mixed. After filtering, the distilled states demonstrate certain non-local correlations, as evidenced by their violation of a form of Bell's inequality. Because the initial states do not have this property, they can be said to possess 'hidden' non-locality.

Experimental verification of decoherence-free subspaces.

Using spontaneous parametric down-conversion, we produce polarization-entangled states of two photons and characterize them using two-photon tomography to measure the density matrix. A controllable decoherence is imposed on the states by passing the photons through thick, adjustable birefringent elements. When the system is subject to collective decoherence, one particular entangled state is seen to be decoherence-free, as predicted by theory. Such decoherence-free systems may have an important role for the future of quantum computation and information processing.

Absolute efficiency and time-response measurement of single-photon detectors.

Using correlated photons from spontaneous parametric downconversion, we have measured both the absolute quantum efficiencies and the time responses of four single-photon detectors. Efficiencies as high as (76.4 ± 2.3)% (at 702 nm) were seen, which to our knowledge are the highest reported single-photon detection efficiencies. An auxiliary retroreflection mirror was found to increase the net detection efficiency by as much as a factor of 1.19. The narrowest time profile for coincidences between two detectors displays a peak with 300 ps FWHM. We also investigated the presence of afterpulses and the effects of saturation and varying device parameters.