Laser-induced damage growth of fused silica optics near growth threshold at 351 nm.

Laser-induced damage growth on the exit surface of fused silica optics triggered by nanosecond pulses at 351 nm is widely described with exponential dynamics. In this Letter, a particular experimental setup allowed us to study damage growth with a large beam and fluences near damage growth threshold for a high number of shots. This allowed us to observe and characterize a regime with a slow and linear growth dynamic not documented in the literature and yet fundamental for the operation of high-power laser installations.

Linear-to-circular polarization conversion with full-silica meta-optics to reduce nonlinear effects in high-energy lasers.

High-energy lasers have benefited from intense efforts to bring light-matter interactions to new standards and to achieve laser fusion ignition. One of the main issues to further increasing laser energy is the resistance of optical materials to high laser fluences, in particular at the final stage of the laser beamline where nonlinear Kerr effects can occur in optical materials and provoke laser filamentation. One promising way to mitigate this process is to reduce the nonlinear susceptibility of the material by switching the polarization from a linear to a circular state. Here, we report a significant reduction in the laser filamentation effect on glass by using a full-silica metamaterial waveplateable to switch the linear-to-circular polarization of high fluence laser beams. This result is achieved through the use of a large size full-silica meta-optics exhibiting nominal polarization conversion associated with an excellent transmission efficiency and wavefront quality, as well as a high laser damage resistance.

Impact of the multilayer dielectric design on the laser-induced damage threshold of pulse compression gratings for petawatt-class lasers.

The peak-power of petawatt-class lasers is limited by laser-induced damage to final optical components, especially on the pulse compression gratings. Multilayer dielectric (MLD) gratings are widely used in compressor systems because they exhibit a high diffraction efficiency and high damage threshold. It is now well established that the etching profile plays a key role in the electric field distribution, which influences the laser damage resistance of MLD gratings. However, less attention has been devoted to the influence of the multilayer design on the laser damage resistance of MLD gratings. In this Letter, we numerically and experimentally evidence the impact of the dielectric stack design on the electric field intensity (EFI) and the laser-induced damage threshold (LIDT). Three different MLD gratings are designed and manufactured to perform laser damage tests. On the basis of the expected EFIs and diffraction efficiencies, the measured LIDTs show how the multilayer design influences the laser resistance of the MLD gratings. This result highlights the impact of the multilayer dielectric design on the electric field distribution and shows how to further improve the laser-induced damage threshold of pulse compression gratings.

Influence of the multilayer dielectric mirror design on the laser damage growth in the sub-picosecond regime.

The peak power of high-power laser facilities is limited by the laser-induced damage to the final optical components. Also, when a damage site is generated, the damage growth phenomenon limits the lifetime of the component. Many studies have been performed to improve the laser-induced damage threshold of these components. The question now arises as to whether improvement of the initiation threshold leads to a reduction of the damage growth phenomenon. To address this question, we performed damage growth experiments on three different multilayer dielectric mirror designs exhibiting different damage thresholds. We used classical quarter-wave designs and optimized designs. The experiments were carried out with a spatial top-hat beam, spectrally centered at 1053 nm with a pulse duration of 0.8 ps in s- and p-polarization. The results showed the impact of design on the improvement of the damage growth thresholds and a reduction of the damage growth rates. A numerical model was used to simulate damage growth sequences. The results reveal similar trends to those observed experimentally. On the basis of these three cases, we have shown that improvement of the initiation threshold through a modification of the mirror design can lead to the reduction of the damage growth phenomenon.

Estimation of laser-induced damage depth from surface image features.

In laser damage experiments, damage initiation and growth are typically monitored by imaging the surface of the tested fused silica sample, ignoring their bulk morphology. The depth of a damage site in fused silica optics is considered to be proportional to its equivalent diameter. However, some damage sites experience phases with no diameter changes but growth in the bulk independently from their surface. A proportionality relationship with the damage diameter does not accurately describe the growth of such sites. In the following, an accurate estimator for damage depth is proposed, which is based on the hypothesis that the light intensity scattered by a damage site is proportional to its volume. Such an estimator, using the pixel intensity, describes the change of damage depth through successive laser irradiations, including phases in which depth and diameter variations are uncorrelated.

Full-scale optic designed for onsite study of damage growth at the Laser MegaJoule facility.

Large fusion scale laser facilities aim at delivering megajoules laser energy in the UV spectrum and nanosecond regime. Due to the extreme laser energies, the laser damage of final optics of such beamlines is an important issue that must be addressed. Once a damage site initiates, it grows at each laser shot which decreases the quality of the optical component and spoil laser performances. Operation at full energy and power of such laser facilities requires a perfect control of damage kinetics and laser parameters. Monitoring damage kinetics involves onsite observation, understanding of damage growth process and prediction of growth features. Facilities are equipped with cameras dedicated to the monitoring of damage site growth. Here we propose to design and manufacture a dedicated full size optical component to study damage growth at increased energy, on the beamline, i.e. in the real environment of the optics on a large laser facility. Used for the first time in 2021, the growth statistics acquired by this approach at the Laser MegaJoule (LMJ) facility provides a new calibration point at a fluence less than 5 J cm-2 and a flat-in-time pulse of 3 ns.

Investigation of the influence of a spatial beam profile on laser damage growth dynamics in multilayer dielectric mirrors in the near infrared sub-picosecond regime.

Laser-induced damage growth has often been studied with Gaussian beams in the sub-picosecond regime. However, beams generated by high-power laser facilities do not feature Gaussian profiles, a property that raises questions concerning the reliability of off-line laser-induced damage measurements. Here, we compare laser-induced damage growth dynamics as a function of beam profiles. Experiments on multilayer dielectric mirrors at 1053 nm have been carried out with squared top-hat and Gaussian beams. The results demonstrate that the laser-induced damage growth threshold does not depend on the incident beam profile. A higher damage growth rate, however, has been measured with the top-hat beam. In addition, three different regimes in the growth dynamics were identified above a given fluence. A numerical model has been developed to simulate a complete damage growth sequence for different beam profiles. The numerical results are in good agreement with the observations, three growth regimes were also revealed. These results demonstrate that a linear description of growth cannot be used for the whole growth domain.

Estimating and monitoring laser-induced damage size on glass windows with a deep-learning-based pipeline.

Laser-induced damage is a major issue in high power laser facilities such as the Laser MégaJoule (LMJ) and National Ignition Facility (NIF) since they lower the efficiency of optical components and may even require their replacement. This problem occurs mainly in the final stages of the laser beamlines and in particular in the glass windows through which laser beams enter the central vacuum chamber. Monitoring such damage sites in high energy laser facilities is, therefore, of major importance. However, the automatic monitoring of damage sites is challenging due to the small size of damage sites and to the low-resolution images provided by the onsite camera used to monitor their occurrence. A systematic approach based on a deep learning computer vision pipeline is introduced to estimate the dimensions of damage sites of the glass windows of the LMJ facility. The ability of the pipeline to specialize in the estimation of damage sites of a size less than the repair threshold is demonstrated by showing its higher efficiency than classical machine learning approaches in the specific case of damage site images. In addition, its performances on three datasets are evaluated to show both robustness and accuracy.

Polarization dependence of laser damage growth features on multilayer dielectric mirrors for petawatt-class lasers.

PETAL (Petawatt Aquitaine Laser) is an ultrahigh-power laser dedicated to academic research that delivers sub-picosecond pulses. One of the major issues of these facilities is the laser damage on optical components located at the final stage. Transport mirrors of the PETAL facility are illuminated under different polarization directions. This configuration motivates a thorough investigation of the dependency of the laser damage growth features (thresholds, dynamics, and damage site morphologies) on the incident polarization. Damage growth experiments were carried out in s- and p-polarization at 0.8 ps and 1053 nm on multilayer dielectric mirrors with a squared top-hat beam. Damage growth coefficients are determined by measuring the evolution of the damaged area for both polarizations. In this Letter, we report higher damage growth threshold in p-polarization together with higher damage initiation threshold in s-polarization. We also report faster damage growth dynamics in p-polarization. The damage site morphologies and their evolution under successive pulses are found to strongly depend on polarization. A numerical model in 3D was developed to assess experimental observations. This model shows the relative differences in damage growth threshold even if it is not able to reproduce the damage growth rate. Numerical results demonstrate that damage growth is mainly driven by the electric field distribution which depends on the polarization.

Sub-pixel detection of laser-induced damage and its growth on fused silica optics using registration residuals.

Fused silica optics are key components to manipulate high energy Inertial Confinement Fusion (ICF) laser beams but their optical properties can be degraded by laser-induced damage. The detection of laser damage sites is of major importance. The challenge is to monitor damage initiation and growth at sub-pixel scale with highly sensitive measurements. The damage diameter is a widely used indicator to quantify damage growth but its accuracy is strongly dependent on the available image resolution. More recently, it was shown that registration residual maps (i.e., gray level differences between two registered images) could also be used to monitor laser-induced damage. In this paper, the performance of both indicators are compared to detect laser damage initiation and growth at high and low image resolutions thanks to a highly instrumented laser setup. The results prove that registration residual maps are more efficient to detect sub-pixel laser damage growth than diameter measurements at a given image resolution. The registration residual maps are therefore a powerful indicator for monitoring laser-induced damage initiation and growth at sub-pixel scale either for laser damage metrology setups, for high energy laser facilities, or other situations where damage is suspected to occur. The accuracy of (laser-induced) damage laws may also be improved thanks to this tool.

Parametric study of laser-induced damage growth in fused silica optics with large beams at 351 nm. Part 1: stochastic approach.

Both the rate and probability of the growth of laser-induced damage sites in fused silica depend on several parameters. In this two-part paper, we investigate the impact of the laser parameters on damage growth. In Part I, we present statistical measurements of damage growth at different energy densities, pulse durations, and initial damage sizes. In Part II, we use fractal analysis to quantify the evolution of the damage morphology as a function of the laser energy density and pulse duration. Damage initiation is performed using phase masks. These phase masks allow for the initiation of evenly spaced damage sites that can then be exposed to the same laser beam, and, therefore, the same pulse duration. This configuration allowed the study of damage growth in a large population of more than 5000 damage sites. The results clearly indicate that both the probability and the rate at which a damage site will grow strongly depend on the laser pulse duration. These differences can be explained by hypotheses that we have developed from an observation of the bulk damage morphology. Such observations will be presented in detail in the second part of this article.

Parametric study of laser-induced damage growth in fused silica optics with large beams at 351 nm. Part 2: fractal analysis.

The impact of laser fluence and pulse duration on both the rate and probability of growth of laser-induced damage sites has been reported and analyzed statistically in a companion paper. In this paper, we report and analyze the volume morphology of damage sites during the growth process in fused silica optical components, at 351 nm, under various laser fluence and pulse durations. Fractal analysis has been used to quantify the bulk damage morphology. A clear link between the damage morphology and laser pulse duration has been observed. The results from fractal analysis allows for a better understanding of the results from the stochastic approach developed in our companion paper. More specifically, fractal analysis shows how the laser parameters such as fluence and pulse duration impact the phenomenology and the dynamics of the growth process.

Temporal dependency in the picosecond regime of laser damage growth.

Based on squared top-hat beam irradiations, we investigate how a change of the pulse duration in the picosecond regime affects the phenomenon of laser damage growth on dielectric mirrors. We first confirm two major previously reported experimental results with a Gaussian beam that are the existence of a growth threshold fluence smaller than the laser-induced damage threshold (LIDT) and the linear evolution, characterized by a growth coefficient, of the damage area with the number of irradiations when growth occurs. We then express the growth coefficient with the fluence and the growth threshold in particular. Changing the pulse duration ultimately allows us to refine this expression a step further which leads us to establish an empirical growth law for the damage area. The temporal dependency displayed within this law appears to be very close to the one found for the LIDT which evidences the deterministic nature of laser damage growth in short pulse regimes.

Large optics metrology for high-power lasers.

The Laser MégaJoule (LMJ) is a high-power laser dedicated to laser-plasma experiments. At the beginning of the project in the mid-1990s, an optical metrology laboratory was created at CEA to help accomplish all the steps in the construction of this laser. This paper proposes an overview of the capabilities of this metrology laboratory in four main fields: surface imperfections, photometry, laser damage measurement, and wavefront measurement. The specificities for high-power laser optics in each domain are highlighted as well as the specific features that make our instruments unique.

Wavelength dependence of the mechanisms governing the formation of nanosecond laser-induced damage in fused silica.

The influence of the wavelength on the morphology of nanosecond laser-induced damage on the exit surface of fused silica is investigated. A combination between the typical features of damage sites initiated at 1064 nm and 355 nm is observed at 532 nm, including ring patterns sporadically exhibited, in good agreement with calculations of the development of an electron avalanche at this wavelength. The associated ring appearance speed scales as the cube root of the laser intensity, and is ~10.5 km/s while it is ~20 km/s when initiated by infrared pulses. The whole set of results sheds light on the different wavelength-dependent mechanisms governing damage formation.

Nanosecond laser damage initiation at 0.35 µm in fused silica.

In nanosecond regime, the laser-induced damage density at the exit surface of fused silica optics at the wavelength of 0.35 µm shows a characteristic behavior: in a specific fluence range, the surface damage density begins to grow exponentially as a function of fluence and then tends to saturate at high fluences. Up to now, no satisfactory explanation of these peculiarities could be provided. We herein detail a statistical model based on laser-matter interaction, where two types of absorbing precursors are involved in the energy deposit: subsurface micro-cracks and surface impurities. We show that the reported model predicts this characteristic damage density for a large range of fluences and different polishing processes.

Laser-induced damage of fused silica optics at 355 nm due to backward stimulated Brillouin scattering: experimental and theoretical results.

Forward pump pulses with nanosecond duration are able to generate an acoustic wave via electrostriction through a few centimeters of bulk silica. Part of the incident energy is then scattered back on this sound wave, creating a backward Stokes pulse. This phenomenon known as stimulated Brillouin scattering (SBS) might induce first energy-loss, variable change of the temporal waveform depending on the location in the spatial profile making accurate metrology impossible, and moreover it might also initiate front surface damage making the optics unusable. Experiments performed on thick fused silica optics at 355 nm with single longitudinal mode pulses allowed us to detect, observe and quantify these backward pulses. Experimental results are first compared to theoretical calculations in order to strengthen our confidence in metrology. On this basis a phase-modulator has been implemented on the continuous-wave seeders of the lasers leading to pulses with a wide spectrum that suppress SBS and do not exhibit temporal overshoots that also reduce Kerr effects. The developed set-ups are used to check the reduction of the backward stimulated Brillouin scattering and they allow measuring with accuracy the rear surface damage of thick fused silica optics.

Impact of mechanical stress induced in silica vacuum windows on laser-induced damage.

At the interface between vacuum and air, optical windows must keep their optical properties, despite being subjected to mechanical stress. In this Letter, we investigate the impact of such stress on the laser-induced damage of fused silica windows at the wavelength of 351 nm in the nanosecond regime. Different stress values, from 1 to 30 MPa, both tensile and compressive, were applied. No effect of the stress on the laser-induced damage was evidenced.

Multi-wavelength growth of nanosecond laser-induced surface damage on fused silica gratings.

The nanosecond laser-induced damage growth phenomenon on the exit surface of fused silica grating is investigated at 1064 nm and 355 nm separately and also simultaneously. Experiments are first carried out on damage sites on a plane fused silica sample showing two different morphologies, and a damage type is selected for ensuring the repeatability of the subsequent tests. Comparing the mono-wavelength growth results on a grating and a plane fused silica sample, the periodic surface structure is found to be an aggravating factor for damage growth. This is highly supported by calculations of the enhancement of the optical electric field intensity thanks to Finite-Difference Time-Domain simulations. Finally, the mono-wavelength results enable us to quantify a coupling occurring in the multi-wavelength configuration, which could originate from the heating of the plasma (more likely produced in the ultraviolet) preferentially by the infrared pulse. This study provides interesting results about the involvement of the surface topography in damage growth, and paves the way towards the comprehension of this phenomenon at high-energy nanosecond laser facilities where fused silica gratings are simultaneously irradiated at several wavelengths.

Quantification of laser-induced damage growth using fractal analysis.

Lateral and longitudinal laser damage growth under subsequent irradiations at 351 nm in the nanosecond range from micrometric to millimetric scales is presented herein. Atypical behavior has been observed, showing the growth in the longitudinal direction, whereas the lateral growth does not evolve. We propose the use of fractal analysis to describe the evolution of the bulk damage morphology. The results indicate first a dependence between the damage fractal dimension and the laser parameters, such as the fluence and the pulse duration. Next, it seems from observations that the damage morphology modifications drive the growth rate changes.